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Quantum device applications of mesoscopic superconductivity

Mika E. T. Sillanpää

Published Apr 1, 2005• 2 citations
OpenAlex

Abstract

The work involves a study of physical phenomena that take place at very small length scales, below one micro-meter. At temperatures roughly below one degree Kelvin, quantum-mechanical effects may rule in electronic transport. Macroscopic quantum-coherent effects that occur in metallic superconducting microstructures, are particularly intriguing. Large-scale quantum information processing is widely believed to be attainable utilizing such physical systems. This work concentrates on answering the question of how the described quantum-mechanical systems may be used as sensitive measuring devices. Considerable attention is paid to energy-storing metallic microstructures whose electrical properties resemble those of the familiar inductor or capacitor. This research involves primarily experimental investigations conducted around temperatures of 0.1 Kelvin. Methods both at low and at radio frequencies have been used. The experimental findings have been modelled theoretically, and theoretical concepts for new physical phenomena have been introduced. An inductively measured radio-frequency Cooper-pair transistor, the L-SET, has been developed and experimentally verified in this work. Being highly sensitive, fast, and non-invasive, the L-SET appears to be the most promising method for measuring electric charge. Sensitivity in charge measurements of 20 millionths of the electron charge (micro-e) within one second, and an input bandwidth of 100 MHz, have been demonstrated. It has been shown theoretically that the ultimate measurement accuracy is about 0.1 micro-e within a second. A new phase detector based on the Cooper-pair transistor has been proposed. This system has also been shown to be potentially usable as a quantum bit. A new type of radio-frequency single-electron transistor built using a multi-walled carbon nanotube has been fabricated and operated. Technologies have been developed in order to make the physical nano- or microstructures. A method has been presented to fabricate non-superconducting tunnel junctions. Consequences of the inverse superconducting proximity effect on the studied superconducting structures were considered. Measurement procedures were investigated for a new low-noise nanoamplifier, the Bloch-oscillating transistor. Single superconducting tunnel junctions were tested as detectors of energy states of the environment, or of noise.

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In this work four different mesoscopic superconducting devices have been experimentally studied: an ammeter based on a hysteretic Josephson junction switching from the superconducting state to the normal state, a conventional Cooper pair pump (CPP) based on two superconducting islands separated by tunnel junctions, a novel flux assisted Cooper pair pump and a thermometer based on a tunnel junction between a superconductor and a normal metal. These devices make use of phenomena related to superconductivity and are also benefiting from some properties of small structures, e.g., of quantum mechanical tunneling and of transport of single electrons. The present research focused on investigating performance limitations of these devices and the aim was to improve their performance. A hysteretic Josephson junction switching can be used as a sensitive current threshold detector. For many purposes, a smaller critical current Ic of the detecting junction would yield a higher current sensitivity. It was found in this Thesis that the main limitation of the ammeter is that with increasing sensitivity the negative effects due to dissipation start to dominate. In this Thesis the Josephson junction was also demonstrated as a shot-noise detector, and it was concluded that this kind of a device could probably be made into an absolute on-chip detector of Fano-factors and noise in general. A charge pump is a device which can periodically transfer a discrete amount of charge Q through an electrical circuit. The measured double island CPP introduced a frequency dependent current with a value close to the expected one at low pumping frequencies. The drawback in the measurements was that the direction of the pumped current was set by the bias voltage. The results of the measurement on flux assisted pumping were indeed very promising and the studied device was able to produce sufficiently high pumped currents of around 0.1 nA with reasonable accuracy. Thermometer based on NIS (Normal metal - Insulator - Superconductor) tunnel junctions is a very promising temperature sensor for bolometric radiation sensor applications. This work showed that it can be used as a sensitive thermometer up to MHz frequencies range and that its response time is limited by the electron-phonon scattering rate.

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The work involves a study of physical phenomena that take place at very small length scales, below one micro-meter. At temperatures roughly below one degree Kelvin, quantum-mechanical effects may rule in electronic transport. Macroscopic quantum-coherent effects that occur in metallic superconducting microstructures, are particularly intriguing. Large-scale quantum information processing is widely believed to be attainable utilizing such physical systems. This work concentrates on answering the question of how the described quantum-mechanical systems may be used as sensitive measuring devices. Considerable attention is paid to energy-storing metallic microstructures whose electrical properties resemble those of the familiar inductor or capacitor. This research involves primarily experimental investigations conducted around temperatures of 0.1 Kelvin. Methods both at low and at radio frequencies have been used. The experimental findings have been modelled theoretically, and theoretical concepts for new physical phenomena have been introduced. An inductively measured radio-frequency Cooper-pair transistor, the L-SET, has been developed and experimentally verified in this work. Being highly sensitive, fast, and non-invasive, the L-SET appears to be the most promising method for measuring electric charge. Sensitivity in charge measurements of 20 millionths of the electron charge (micro-e) within one second, and an input bandwidth of 100 MHz, have been demonstrated. It has been shown theoretically that the ultimate measurement accuracy is about 0.1 micro-e within a second. A new phase detector based on the Cooper-pair transistor has been proposed. This system has also been shown to be potentially usable as a quantum bit. A new type of radio-frequency single-electron transistor built using a multi-walled carbon nanotube has been fabricated and operated. Technologies have been developed in order to make the physical nano- or microstructures. A method has been presented to fabricate non-superconducting tunnel junctions. Consequences of the inverse superconducting proximity effect on the studied superconducting structures were considered. Measurement procedures were investigated for a new low-noise nanoamplifier, the Bloch-oscillating transistor. Single superconducting tunnel junctions were tested as detectors of energy states of the environment, or of noise.
In this work four different mesoscopic superconducting devices have been experimentally studied: an ammeter based on a hysteretic Josephson junction switching from the superconducting state to the normal state, a conventional Cooper pair pump (CPP) based on two superconducting islands separated by tunnel junctions, a novel flux assisted Cooper pair pump and a thermometer based on a tunnel junction between a superconductor and a normal metal. These devices make use of phenomena related to superconductivity and are also benefiting from some properties of small structures, e.g., of quantum mechanical tunneling and of transport of single electrons. The present research focused on investigating performance limitations of these devices and the aim was to improve their performance. A hysteretic Josephson junction switching can be used as a sensitive current threshold detector. For many purposes, a smaller critical current Ic of the detecting junction would yield a higher current sensitivity. It was found in this Thesis that the main limitation of the ammeter is that with increasing sensitivity the negative effects due to dissipation start to dominate. In this Thesis the Josephson junction was also demonstrated as a shot-noise detector, and it was concluded that this kind of a device could probably be made into an absolute on-chip detector of Fano-factors and noise in general. A charge pump is a device which can periodically transfer a discrete amount of charge Q through an electrical circuit. The measured double island CPP introduced a frequency dependent current with a value close to the expected one at low pumping frequencies. The drawback in the measurements was that the direction of the pumped current was set by the bias voltage. The results of the measurement on flux assisted pumping were indeed very promising and the studied device was able to produce sufficiently high pumped currents of around 0.1 nA with reasonable accuracy. Thermometer based on NIS (Normal metal - Insulator - Superconductor) tunnel junctions is a very promising temperature sensor for bolometric radiation sensor applications. This work showed that it can be used as a sensitive thermometer up to MHz frequencies range and that its response time is limited by the electron-phonon scattering rate.
Properties of weak links between two superconductors, or Josephson junctions, make them interesting for fundamental physics research. Since their discovery over four decades ago, they have provided a unique way to study the behavior of the superconducting quantum phase. More recently, ultra small, or mesoscopic, Josephson junctions with substantial single Cooper pair charging energy have gained interest due to their behavior as macroscopic quantum objects. In addition to the theoretical interest, Josephson junctions can be used as active elements in circuit applications. Particularly, in this Thesis we study two different devices. We develop the required theoretical treatments, derive device properties, and compare the results with experimental data. The first application is a Josephson voltage standard based on externally damped Superconductor - Insulator - Superconductor junctions. It consists of an array of large Josephson junctions connected in series and irradiated with a 70 GHz microwave signal. Phase locking the Josephson dynamics into the signal leads to the quantization of the voltage. This is utilized in metrology. We introduce a new circuit solution based on frequency dependent damping of the junctions. Optimization and some designs for practical arrays are presented. The purpose is to find such a design that the array is fast, has low power consumption and is as stable as possible. Arrays able to generate DC voltages of order 1 volt with metrological accuracy are demonstrated experimentally and their applicability in AC voltage calibrations is analyzed. The second application is the Bloch Oscillating Transistor (BOT). The BOT is based on controlling the Cooper pair current in an ultra small Josephson junction by means of quasiparticles tunneling through a normal junction. As part of the thesis work, the principle of operation is first demonstrated computationally. The model is then refined to yield quantitative predictions of the characteristics. Finally, an analytic theory for the device is developed and the properties as an amplifier are derived.
The Single Electron Transistor (SET), especially its variation the radio frequency single electron transistor (RF-SET), is a fast and ultra-sensitive electrometer working in the vicinity of the quantum limit. In this thesis, the theory and techniques related to the SET in the normal state and the superconducting state are introduced The thesis focuses especially on our efforts of improving the sensitivity of superconducting RF-SET, including: the design and fabrication of an all superconducting near loss-less matching network for improving the RF modulation, our early investigation of the sensitivity and linearity of a superconducting SET (S-SET) subject to quantum fluctuations of quasiparticles and Cooper pairs under different tunneling mechanisms, and our recent work approaching the quantum sensitivity limit using a double Josephson quasiparticle (DJQP) cycle of a S-SET. Using an effective bath description, we have found that the S-SET provides damping of the resonator modes proportional to its differential conductance, and has an effective temperature that can be well below both the ambient temperature and the energy scale of the bias voltage. In the region of negative differential conductance (NDC), the S-SET shows negative damping and a negative temperature. In the final part of the thesis, I have demonstrated our first application of an RF-SET for real-time detection of electron tunneling through a quantum dot.
This thesis presents measurements of quantum coherence in a single Cooper pair box, where quantum oscillations of charge between a reservoir and a small superconducting island have been observed. The single Cooper pair box (SCB) consists of a small metallic island which is connected to a reservoir via a tunnel junction. In the superconducting state, Cooper pairs are free to tunnel to and from the island, whose potential can be controlled by a gate voltage. A graded gap method was used to prevent quasiparticles from tunneling onto the island. For this purpose, a magnetic field suppressed the superconducting gap in the SCB leads more than in the island. This created an additional energy barrier for quasiparticles to tunnel to the island, making the gate voltage modulation periodic in Cooper pair charge. For a limited range of gate voltage, the SCB was found to behave as a model two-level quantum mechanical system. A non-adiabatic change in the induced island charge was used to bring two charge states into resonance. The resulting time evolution showed clear charge oscillations between the ground and excited state, with a frequency given by the energy level separation divided by Planck's constant. These oscillations had a longest coherence time of T2=9 ns at a point where the pure charge states are degenerate. The coherence time at this point was found to be limited by the relaxation rate, ?1. Away from this point, the coherence time was limited by the dephasing rate, ??. Away from the charge degeneracy, the dependence of T2 on gate charge suggested that low frequency fluctuators were the main source of dephasing. The charge of the Cooper pair box was measured by coupling the SCB capacitively to a radio frequency single electron transistor (RF-SET). The RF-SET was used as an electrometer by measuring the amount of reflection from a resonant microwave circuit in which a single electron transistor (SET) was embedded. A best charge sensitivity of 2.3·10-6 e/sqrt(Hz) and a 7 MHz bandwidth was reached in an improved setup. Another part of this thesis concerns an investigation of electrical filters for use in single electronics experiments. The characteristics of seven different types of cryogenic filters were evaluated.
In this thesis the single Cooper pair box (SCB) is investigated with a radio frequency single electron transistor (RF-SET). The RF-SET is used as an electrometer to detect the charge of the SCB. The SCB can be regarded as a quantum two-level system and could therefore be a possible qubit. Both the SCB and the RF-SET have been fabricated with e-beam lithography followed by two-angle shadow evaporation of aluminium. The system has been measured in a dilution refrigerator at temperatures of ~30 mK. A charge sensitivity of 2.3 μe/square root of Hz was measured for an optimized RF-SET with a bandwidth of 7 MHz, operated in the superconducting state. In a phase sensitive measurement of the RF-SET reflected signal, the gate dependence of the quantum capacitance, due to avoided level crossing, was detected in a superconducting SET. Coulomb staircases for the SCB were obtained by changing the charge of the SCB by ramping a gate voltage and continuously measuring the charge with the RF-SET. To prevent quasiparticle poisoning of the SCB island, we have used a method of graded gaps. Here we exploit the greater reduction of the superconducting gap for the connecting leads with an external magnetic field applied, resulting in a higher gap for the island. This creates an effective barrier against quasiparticle tunnelling. The charging energy and the Josephson coupling energy of the SCB were measured with microwave spectroscopy. The SCBs were fabricated in a SQUID geometry, which made it possible to tune the Josephson coupling energy of the box. This tuning was verified through microwave spectroscopy. The effect of tuning could also be seen in the pure 2e Coulomb staircase, as a predicted smearing of the staircase, which was in excellent agreement with the independent spectroscopy data. Coherent quantum oscillation of the SCB charge state was measured by applying nonadiabatic DC-pulses to the SCB gate. The measured amplitude of the charge oscillations was higher than 70%. The deviation from 100% can be explained by the initial charge state purity and the finite rise time of the pulses. The longest decoherence time of the charge oscillations was T2 = 9 ns at the charge degeneracy point. It was found to be limited by relaxation. Away from the degeneracy point the decoherence time was limited by pure dephasing, due to low frequency charge fluctuators.
This Thesis studies opportunities to create a quantum standard for the electric current with the help of tunnel junctions. We use two types of tunnel junctions: superconducting Josephson junctions, and NIS junctions where one of the electrodes is normal (N) and the other one superconducting (S). In both cases, tunnel junctions are employed in a single-electron transistor (SET) structure, which is used to transfer a controlled number k of electrons (e) with the repetition frequency f. The magnitude of the resulting current is thus I = kef. First, we study the Cooper pair sluice, where Josephson junctions are connected as two superconducting quantum interference devices (SQUID). A gate electrode is used to control the charge state of the superconducting island formed between the SQUIDs. The sluice is based on tuning the tunneling rates through the SQUIDs with local magnetic fluxes, which allows to control the direction of the charge transfer. Weak traces of current quantization can be observed up to above 1 nA, which is large enough current for many metrological purposes. However, the accuracy of the current is still far from what is required in metrology. We study also a new type of SQUID structure, the balanced SQUID, which could be used to improve the accuracy of the sluice or in, e.g., some quantum computing applications. Second, we employ NIS junctions in the hybrid (SINIS) single-electron transistor with superconducting leads and a normal-metal island. This structure can be used as the SINIS turnstile which lets electrons to flow one by one in the direction determined by the bias voltage. We report the first experimental results on the SINIS turnstile and two methods to improve the accuracy of the current: increasing the charging energy of the island or connecting the turnstile in a resistive environment. We also show that the SINIS turnstile can be used as an electronic radio-frequency refrigerator where tunneling processes cool the electron temperature of the normal-metal island.