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Physical Review A

Radio-frequency-assisted electromagnetically induced transparency

Carl Basler, Jonas Grzesiak, Hanspeter Helm

Published Jul 7, 2015• 13 citations
Publisher

Abstract

A near-resonant rf field pumping the hyperfine transition between the two ground states of a $\mathrm{\ensuremath{\Lambda}}$-shaped dark resonance leads to a resonance tripling, each component displaying electromagnetically induced transparency (EIT). We investigate the three resonances under high spectral and temporal resolution. The triplet formation is analogous to that of the Mollow triplet but distinct in that the role played by the spontaneous emission rate is now taken by the one-photon scattering rate of the optical Raman transition. Complex phase relations exist between the three em fields under EIT conditions. We explain our observations using numerical solutions of the quantum master equation as well as a simple analytical dressed-state model.

DOI
10.1103/physreva.92.013809

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•Jan 1, 2011•5 citations
A near-resonant rf field pumping the hyperfine transition between the two ground states of a \ensuremathΛ\mathrm{\ensuremath{\Lambda}}\ensuremathΛ-shaped dark resonance leads to a resonance tripling, each component displaying electromagnetically induced transparency (EIT). We investigate the three resonances under high spectral and temporal resolution. The triplet formation is analogous to that of the Mollow triplet but distinct in that the role played by the spontaneous emission rate is now taken by the one-photon scattering rate of the optical Raman transition. Complex phase relations exist between the three em fields under EIT conditions. We explain our observations using numerical solutions of the quantum master equation as well as a simple analytical dressed-state model.
In this paper we study the nonlinear behavior of an electromagnetically induced transparency (EIT) resonance subject to a coherent driving field. The EIT is associated with a $\ensuremath{\Lambda}$ three-level system where two hyperfine levels within an electronic ground state are coupled to a common excited state level by a coupling field and a probe field. In addition there is an radio-frequency (rf) field driving a hyperfine transition within the ground state. The paper contrasts two different situations. In one case the rf-driven transition shares a common level with the probed transition and in the second case it shares a common level with the coupled transition. In both cases the EIT resonance is split into a doublet and the characteristics of the EIT doublet are determined by the strength and frequency of the rf-driving field. The doublet splitting originates from the rf-field induced dynamic Stark effect and has close analogy with the Autler-Townes effect observed in three-level pump-probe spectroscopy study. The situation changes when the rf field is strong and the two cases are very different. One is analogous to two $\ensuremath{\Lambda}$ three-level systems with EIT resonance associated with each. The other corresponds to a doubly driven three-level system with rf-field-induced electromagnetically induced absorption resonance. The two situations are modeled using numerical solutions of the relevant equation of motion of density matrix. In addition a physical account of their behaviors is given in terms of a dressed state picture.
The transparency and absorption of the Λ-type three-level scheme driven by two coupling fields were investigated.Mollow profile was obtained in a two-level scheme where a strong coupling field and a probing field were applied on the same optical transition between excited state and ground state.There was another coupling field which drived excited state to another ground states hyperfine level in this paper.The Λ-type three-level scheme driven by two coupling fields was introduced,and some new quantum coherent phenomena were given.It can be seen that there is superposition of Mollow profile and electromagnetically induced transparency(EIT) or electromagnetically induced absorption(EIA).The dependence of the position of EIT or EIA on Rabi frequencies and frequency detunings of two coupling fields is investigated.The results can be explained by dressed-state formalism.
Electromagnetically induced transparency (EIT) resonance is obtained in a well-studied lambda three level system where an optical coupling field and a probing field interact with two optical transitions. However, both electromagnetically induced absorption (EIA) and EIT can be obtained in a modified quasi-lambda four level system consisting of an optical-radio two-photon coupling field and a probing field. By solving the density matrix equation of motion, a physical account of EIA and EIT is given in terms of a dressed state picture. It can be seen that the optical coupling field in this quasi-lambda four level system has a crucial effect on the forming of EIA and EIT. An EIA is observed under a resonant optical coupling and it evolves into an EIT when there is a detuning. Furthermore, the width of EIA or EIT increases as the optical coupling Rabi frequency increases.
Summary form only given. Electromagnetically induced transparency (EIT) is a process by which a normally absorbing material is made transparent by application of electromagnetic radiation. It has a number of applications, including lasing without inversion and slow light. We see that the EIT resonances corresponding to the hyperfine levels are either inhibited, or enhanced depending on the position of the hyperfine transitions in relation to the applied rf field. We discuss the role of level splitting (destruction of EIT) and three photon resonance peaks in the resulting spectra. A 2 cm rubidium cell, heated to approximated 60 C is probed with a 780 nm laser.
Electromagnetically induced transparency (EIT) resonance in a $\ensuremath{\Lambda}$ configuration is obtained when the frequencies of two fields are close to resonance with two of the transitions and their frequency difference matches the frequency of the third transition. In this situation the spectrum of one swept field as a probe gives a simple transparency feature. However, when an additional field drives the third transition the EIT feature associated with the probe is split. This perturbed EIT is illustrated for both single and bichromatic driving fields. In the single-driving-field case a density matrix treatment is shown to be in reasonable agreement with experiment, and in both single and bichromatic cases the structure in the spectrum can be explained using the dressed-state formalism. The dressed states can also be used to account for subharmonic resonances observed in the strong-probe regime.
We initially discuss the theory of three-level systems using the dressed state formalism. One of the dressed states, containing a ground state and a Rydberg state, does not couple with the probe laser; thus, the medium becomes transparent to the latter. This phenomenon is known as electro- magnetically induced transparency (EIT) and this dressed state is known as a Rydberg dark state. We show that EIT can be used to extract the reduced dipole matrix element for transitions to a Rydberg state. However, a prob- lem with three-level Rydberg EIT in a vapour cell is the occurrence of space charges caused by photoelectric ionisation of Rb metal deposited inside the cell. To avoid this problem, we consider adding a third laser resonant with a fourth level. This is to avoid using the laser whose wavelength is less than the threshold wavelength. In cold atoms, the effect of the third laser is to split the usual EIT resonance into a doublet. In thermal atoms, we observe narrow features due to electromagnetically induced absorption and electro- magnetically induced transparency in the Doppler-free configuration. Next we consider the action of a far off-resonance radio frequency (rf) field in the three-level system. We demonstrate the formation of rf-dressed EIT reso- nances in a thermal Rb vapour and show that such states exhibit enhanced sensitivity to dc electric fields compared to their bare counterparts. Fitting the corresponding EIT profile enables precise measurements of the dc field in- dependent of laser frequency fluctuations. We further investigate the theory of rf-dressed Rydberg EIT using the Floquet approach in order to understand the formation of the sideband structure of the Rydberg state. We find that if the time scale of the rf interaction is much shorter than that of the system evolution and decoherence, the sideband structure is well resolved. We also show that the intermediate state exhibits a sideband structure, induced by the Rydberg state, when the Rabi frequency of coupling laser is larger than twice the modulation frequency. Finally we consider resonant microwave cou- pling between the Rydberg states which leads to an Autler-Townes splitting of the EIT resonance in cold atoms. This splitting can be employed to vary the group index by ±10^5 allowing independent control of the absorptive and dispersive properties of the medium, i.e., one can switch the transparency of the medium or control the group velocity of a pulse propagation by tuning on and off the microwave field.