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Manipulation and characterisation of two photon spectral correlation states in nonlinear devices

Iman Jizan

Published Jun 29, 2016• 0 citations
OpenAlex

Abstract

In quantum photonics, the requirement for photon pairs with specific quantum states has led to a demand for a fast, high resolution and accurate characterisation of photon pair sources. However, current quantum methods of characterisation suffer from limited accuracy and resolution, and only consist of intensity measurements that prevent access to phase-sensitive measurement photon pairs. A promising tool that addresses these challenges, uses the classical analogue of nonlinear processes to stimulate photon generation, yielding much higher count rates that allows for a higher resolution and accurate photon pair source characterisation. Furthermore, this classical measurement allows for an innovative method to perform full phase-sensitive quantum tomography of photon pair sources that was previous thought to be experimentally challenging to obtain. This thesis examines and compares the quantum and classical method of characterisation of spectral correlations in χ^3 nonlinear devices; namely two integrated silicon nanowires, and a highly nonlinear fibre. In the first study, we use stimulated nonlinear process to confirm the speed-up of characterisation of photon pairs and demonstrate that additional resolution is gained when compared to the traditional coincidence measurements with no increase in measurement time. By applying this technique with phase-sensitive amplification to another identical silicon nanowire, the first phase sensitive measurements are presented showing details that are otherwise hidden in traditional intensity measurements. Furthermore, phase-sensitive measurement of a highly nonlinear fibre shows that phase-sensitive measurements have excellent sensitivity to small features when compared to the traditional intensity measurements.

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•Jan 1, 2018•0 citations
In quantum photonics, the requirement for photon pairs with specific quantum states has led to a demand for a fast, high resolution and accurate characterisation of photon pair sources. However, current quantum methods of characterisation suffer from limited accuracy and resolution, and only consist of intensity measurements that prevent access to phase-sensitive measurement photon pairs. A promising tool that addresses these challenges, uses the classical analogue of nonlinear processes to stimulate photon generation, yielding much higher count rates that allows for a higher resolution and accurate photon pair source characterisation. Furthermore, this classical measurement allows for an innovative method to perform full phase-sensitive quantum tomography of photon pair sources that was previous thought to be experimentally challenging to obtain. This thesis examines and compares the quantum and classical method of characterisation of spectral correlations in χ^3 nonlinear devices; namely two integrated silicon nanowires, and a highly nonlinear fibre. In the first study, we use stimulated nonlinear process to confirm the speed-up of characterisation of photon pairs and demonstrate that additional resolution is gained when compared to the traditional coincidence measurements with no increase in measurement time. By applying this technique with phase-sensitive amplification to another identical silicon nanowire, the first phase sensitive measurements are presented showing details that are otherwise hidden in traditional intensity measurements. Furthermore, phase-sensitive measurement of a highly nonlinear fibre shows that phase-sensitive measurements have excellent sensitivity to small features when compared to the traditional intensity measurements.
The growing requirement for photon pairs with specific spectral correlations in quantum optics experiments has created a demand for fast, high resolution and accurate source characterisation. A promising tool for such characterisation uses classical stimulated processes, in which an additional seed laser stimulates photon generation yielding much higher count rates, as recently demonstrated for a χ(2) integrated source in A. Eckstein et al. Laser Photon. Rev. 8, L76 (2014). In this work we extend these results to χ(3) integrated sources, directly measuring for the first time the relation between spectral correlation measurements via stimulated and spontaneous four wave mixing in an integrated optical waveguide, a silicon nanowire. We directly confirm the speed-up due to higher count rates and demonstrate that this allows additional resolution to be gained when compared to traditional coincidence measurements without any increase in measurement time. As the pump pulse duration can influence the degree of spectral correlation, all of our measurements are taken for two different pump pulse widths. This allows us to confirm that the classical stimulated process correctly captures the degree of spectral correlation regardless of pump pulse duration, and cements its place as an essential characterisation method for the development of future quantum integrated devices.
Non-classical light sources are a fundamental building block of quantum photonic technologies. As these photonic technologies require higher numbers of sources and more specific source properties, it becomes increasingly important to characterize and manipulate these sources effectively. This thesis consists of three main projects, all relating to non-classical sources of light. First, we present a method for the rapid measurement of the joint spectral intensity of fiber-based photon pair sources. This method extends the concept of Stimulated Emission Tomography, using a chirped, broadband seed beam to stimulate the four wave mixing interaction. The use of the broadband seed, generated through supercontinuum generation, allows for measurements on the few second timescale and requires only a single pump laser to achieve high resolution joint spectra. In the second project, we use this characterization tool to test a variety of different fiber-based photon pair sources. We use three different modification approaches (bending, squeezing, and tapering) to induce changes in the joint spectral properties of the photon pair sources. We show that each of these modifications has some impact on the joint spectra measured. The resulting joint spectra are very complex, highlighting the importance of performing measurements rather than relying on calculations alone. Lastly, we demonstrate a fast switch for the manipulation of single photons. The switch uses the optical Kerr effect to rotate the polarization state of single photons at ultrafast timescales. The implementation of this switch is experimentally straightforward, using a commercial, single mode fiber as the Kerr medium and nJ level pump powers. We operate at an 80 MHz repetition rate and measure 97% switching efficiency, picosecond level switching speed, and approximately 800:1 signal to noise ratio from the operation.
Quantum optics plays a central role in the study of fundamental concepts in quantum mechanics, and in the development of new technological applications. Typical experiments employ sources of photon pairs generated by parametric processes such as spontaneous parametric down-conversion and spontaneous four-wave-mixing. The standard characterization of these sources relies on detecting the pairs themselves and thus requires single photon detectors, which limit both measurement speed and accuracy. Here it is shown that the two-photon quantum state that would be generated by parametric fluorescence can be characterised with unprecedented spectral resolution by performing a classical experiment. This streamlined technique gives access to hitherto unexplored features of two-photon states and has the potential to speed up design and testing of massively parallel integrated nonlinear sources by providing a fast and reliable quality control procedure. Additionally, it allows for the engineering of quantum light states at a significantly higher level of spectral detail, powering future quantum optical applications based on time-energy photon correlations.
We present a novel measurement technique to perform full phase-sensitive tomography on the joint spectrum of photon pair sources, using stimulated four-wave mixing and phase-sensitive amplification. Applying this method to an integrated silicon nanowire source with a frequency chirped pump laser, we are able to observe a corresponding phase change in the spectral amplitude that would otherwise be hidden in standard intensity measurements. With a highly nonlinear fiber source, we show that phase-sensitive measurements have superior sensitivity to small spectral features when compared to intensity measurements. This technique enables more complete characterization of photon pair sources based on nonlinear photonics.
Quantum physics holds promise to revolutionise a number of technologies by enabling performance beyond what is feasible with classical resources, such as secure communications, precision measurement and high-speed simulation and computation. To realise this, quantum information must be encoded into one of the physical degrees of freedom of light. The time-frequency (TF) domain provides a infinite-dimensional space which is naturally compatible with integrated optical platforms. Additionally, future quantum networks will require coherent coupling of quantum systems that do not necessarily exhibit TF mode overlap. The ability to generate, coherently control and measure a variety of TF states of quantum light is therefore a necessary step towards implementing optical quantum technologies. Developing the building blocks for future optical quantum applications calls for an assortment of methods for measuring the properties of TF states of quantum light. Whilst much progress has been made towards this goal recently, deficiencies with existing methods remain. Efficient spectrally-resolved detection away from the telecoms wavelength range and a robust approach to single-photon state characterisation that is sensitive to the spectral phase have so far proven challenging. Additionally, accessing quantum advantages requires measurements that are sensitive to the nonclassical correlations that can exist between separate subsystems. However, until now a flexible approach to determining the full quantum state of systems of multiple time/frequency entangled photons has been lacking. Here we develop a toolbox of techniques for the measurement of TF quantum states of light for few-photon systems, and apply these to the task of precision measurement. Firstly, we propose, construct and demonstrate efficient single-photon spectrometers based on dispersive time-to-frequency mapping, using chirped fibre Bragg gratings to apply the necessary group delay dispersion. We use two such devices operating in coincidence to realise a full phase-sensitive reconstruction of the TF state of a single photon, by spectrally resolving the output of a nonclassical interference process with an external reference. We also demonstrate a complementary, optical reference-free method. This characterisation tool, an implementation of electro-optic spectral shearing interferometry with coincident spectrally-resolved single-photon detection, melds techniques from ultrafast metrology and quantum optics. We proceed to demonstrate the flexibility of this device by reconstructing a wide range of test pulses generated with a pulse shaper. By implementing this technique in conjunction with spectrally-resolved detection of a second photon, we realise complete characterisation of the TF wave function of a spectrally-entangled broadband photon pair. This method is robust to a wide range of inputs and is generalisable to spectrally mixed states and across a wide range of wavelengths, including to spectrally non-degenerate photon pairs. To demonstrate, we generate an entangled photon pair with controllable TF entanglement and perform a full reconstruction. Lastly, we present a new technique for using TF entangled photon pairs to realise quantum-enhanced measurement of a time delay in a quantum channel in the presence of environmental noise. This scheme is based on entanglement-enhanced rejection of background light. A simple experiment demonstrating the feasibility of such a measurement is presented.