Single-photon sources based on spontaneous photon-pair generation have enabled pioneering experiments in quantum physics. However, next-generation photonic quantum technologies require higher generation probabilities of photons in well-controlled pure states capable of high-visibility interference. We have harnessed bespoke fiber technology to develop virtually alignment-free sources that deliver high-purity heralded single photons in telecoms single-mode fiber. The resulting access to low-loss optical delay enabled us to actively route the heralded output from two almost identical sources to enhance the delivery probability of single photons relative to one individual source. Our results indicate how the scale of photonic quantum technologies might be increased via guided-wave multiplexing of high-purity photons.
Single-photon sources based on spontaneous photon-pair generation have enabled pioneering experiments in quantum physics. However, next-generation photonic quantum technologies require higher generation probabilities of photons in well-controlled pure states capable of high-visibility interference. We have harnessed bespoke fiber technology to develop virtually alignment-free sources that deliver high-purity heralded single photons in telecoms single-mode fiber. The resulting access to low-loss optical delay enabled us to actively route the heralded output from two almost identical sources to enhance the delivery probability of single photons relative to one individual source. Our results indicate how the scale of photonic quantum technologies might be increased via guided-wave multiplexing of high-purity photons.
Single photon sources based on spontaneous photon-pair generation have enabled pioneering experiments in quantum optics. However, their non-determinism presents a bottleneck to scaling up photonic and hybrid quantum-enhanced technologies. Furthermore, photon pairs are typically emitted into many correlated frequency modes, producing an undesirable mixed state on heralding. Here we present a complete fibre-integrated heralded single photon source that addresses both these difficulties simultaneously. We use active switching to provide a path to deterministic operation by multiplexing separate spontaneous sources, and dispersion engineering to minimise frequency correlation for high-purity single photon generation. All the essential elements -- nonlinear material with dispersion control, wavelength isolation, optical delay, and fast switching -- are incorporated in a low-loss alignment-free package that heralds photons in telecoms single-mode fibre. Our results demonstrate a scalable approach to delivering pure single photons directly into guided-wave photonic devices.
The field of quantum optics offers the intriguing possibility of developing new, potentially ground-breaking technologies based on the laws of quantum physics. Single quanta of light, called photons, are at the heart of many such quantum optical technologies. They can serve, for example, as information carriers in quantum cryptography and in quantum-information processing. If such applications are to fulfill their enormous potential, it is essential to have sources available that provide photons in the required quantum states. An established way of generating states of single photons is based on photon-pair sources. In this approach, the detection of one photon of a pair heralds the presence of the partner photon, which can then be further processed. However, to generate heralded photons in pure quantum states, specific conditions have to be met, making the design and implementation of such sources challenging. This thesis presents two new photon-pair sources that allow the heralded generation of single photons with high purity. Both sources are based on optical fiber, which allows high collection efficiencies for the generated states and opens the possibility of easy integration into modern-day fiber networks. Chapter 1 provides an introduction to quantum optical technologies and gives a short overview of current approaches to generate pure single photons. Chapter 2 presents the basic theory on which the experimental work presented in Chapters 3 and 4 is based. It explains the concept of a spectrally broad single photon and how photon purity can be tested using Hong-Ou-Mandel (HOM) interference. Subsequently, the properties of photon-pair states and the heralded generation of single photons from such states are discussed. It is shown that for a heralded photon to be pure, the original photon pair has to be in a factorable state, that is, free of any correlations. The introduced theory is then applied to spontaneous four-wave mixing (SFWM) in optical fibers, a nonlinear process that allows the generation of photon pairs. It is shown how the factorability of the created pairs depends on the fiber's dispersion properties, and the necessary conditions for the generation of factorable states are derived. The chapter concludes with an analysis of the photon statistics of the four-wave mixing process, explaining how statistics and the g(2) correlation function can be used to evaluate the factorability of the SFWM output state. Chapters 3 and 4 contain the main results of this thesis. Chapter 3 presents the first spectrally decorrelated photon-pair source bridging the visible and telecommunication wavelength ranges. The photon pairs are generated by SFWM in a photonic crystal fiber (PCF). The chapter documents the procedure of how the PCF source was designed and fabricated, as well as its characterization based on spectral measurements and photon statistics. One photon of the pair state is generated in the visible at 513.5 nm, where it can be efficiently detected with silicon-based single-photon detectors. It serves as a herald for its broadband partner photon, which is emitted in the telecom wavelength range at 1547 nm. A spectral coincidence measurement shows that the heralded photon exhibits a purity of up to 0.82. At increased pump powers, even the heralded generation of higher photon-number states in the telecom band becomes feasible. In Chapter 4, we use commercial birefringent fiber to herald high-purity photons of picosecond duration at 848 nm. The presented two-source HOM interference experiment shows that the heralded unfiltered state has a purity of at least 0.73. This value is increased to 0.84 with the application of wavelength filters suppressing low-intensity side peaks in the spectrum. The heralded photons are coupled into a single-mode fiber with an efficiency of 85%, the highest reported value to date for factorable sources. It is also shown that a commercial polarization controller can be used to fine-tune the generated wavelengths. This facilitates matching photons from multiple sources, as required for optical quantum computing schemes. Chapter 5 summarizes all results and provides an outlook toward potential future projects.
Heralded single photon sources, based on probabilistic non-linear interactions, currently serve as the de-facto standard for performing multi-photon quantum interference experiments. Already, interesting phenomena may be explored with a handful of such sources [1], whilst in the future, large arrays of identical sources could be multiplexed with a switching network to achieve a truly scalable, near-deterministic emission [2]. However, fabricating such a large number of indistinguishable, pure, heralded single photon sources, operating with low-loss, remains an open challenge. Spontaneous four-wave mixing (SFWM) in a silica waveguide is a promising route to building such a source. The low-loss and excellent mode-matching to optical fibre of silica waveguides allows high preparation efficiency. Guided-wave photonics also allows the precise control of the optical modes needed to engineer emission of photons into a single pair of Schmidt modes: allowing heralded photons of high purity without narrowband filtering [3].
Abstract : Single photons sources are desired for many potential quantum information applications. One common method to produce single photons is based on a heralding protocol, which involves generating a pair of photons in an optical nonlinear medium and then detecting one photon in the pair to announce the existence of the other photon of the pair. Compared to other schemes, such a method offers several significant advantages. A major challenge to overcome which is inherent to this method, however, is that the photon pairs are created stochastically in the optical nonlinear medium. Thus, in order to ensure high purity levels for the single photons generated via heralding, sources of this type must be operated at low photon-pair production rates in order to keep the probability for simultaneous creation of multiple photon-pairs to an acceptably low level. A direct result of this restriction is a low heralding rate of single photons. A potential solution for achieving high-rate, high-purity, single-photon generation combines several heralding single-photon sources which are actively multiplexed to act as one source. The overall goal of this project is to develop methods to perform such multiplexing based on the use of a low loss high speed fiber optical switch.
A key obstacle to the experimental realization of many photonic quantum-enhanced technologies is the lack of low-loss sources of single photons in pure quantum states. We demonstrate a promising solution: generation of heralded single photons in a silica photonic chip by spontaneous four-wave mixing. A heralding efficiency of 40%, corresponding to a preparation efficiency of 80% accounting for detector performance, is achieved due to efficient coupling of the low-loss source to optical fibers. A single photon purity of 0.86 is measured from the source number statistics without narrow spectral filtering, and confirmed by direct measurement of the joint spectral intensity. We calculate that similar high-heralded-purity output can be obtained from visible to telecom spectral regions using this approach. On-chip silica sources can have immediate application in a wide range of single-photon quantum optics applications which employ silica photonics.
High-quality quantum sources are of paramount importance for the implementation of quantum technologies. We present here a heralded single-photon source based on commercial-grade polarization-maintaining optical fiber. The heralded photons exhibit a purity of at least 0.84 and an unprecedented heralding efficiency into a single-mode fiber of 85. The birefringent phase-matching condition of the underlying four-wave mixing process can be controlled mechanically to optimize the wavelength tuning needed for interfacing multiple sources, as is required for large-scale entanglement generation.