We investigate the problem of arbitrary photonic-Fock-state scattering in a waveguide-QED system which consists of a one-dimensional waveguide coupled to a two-level system. By imposing the open boundary conditions that directly describe the physical settings, we construct a complete set of eigenstates of the system, and elucidate the mathematical structures of the eigenstates. In particular, we show that the eigenstates include a set of multiphoton extended states and multiphoton bound states, formed by all possible partitions of the photon number $N$. The total number of the eigenstates is exactly described by the integer number partition function $Z(N)$. Using the set of eigenstates, we form the scattering matrix, which facilitates the calculations of the scattered photon states, for the scattering processes. With the scattered photon states, we compute the photon correlation functions that manifestly exhibit the bunching and antibunching behaviors in the scattered photon states. As a concrete example, we discuss in detail with a focus on the three-photon Fock state. Such a capability to generate photonic entanglement from unentangled Fock states will have broad applications in quantum information processing.
We investigate the problem of arbitrary photonic-Fock-state scattering in a waveguide-QED system which consists of a one-dimensional waveguide coupled to a two-level system. By imposing the open boundary conditions that directly describe the physical settings, we construct a complete set of eigenstates of the system, and elucidate the mathematical structures of the eigenstates. In particular, we show that the eigenstates include a set of multiphoton extended states and multiphoton bound states, formed by all possible partitions of the photon number N. The total number of the eigenstates is exactly described by the integer number partition function Z(N). Using the set of eigenstates, we form the scattering matrix, which facilitates the calculations of the scattered photon states, for the scattering processes. With the scattered photon states, we compute the photon correlation functions that manifestly exhibit the bunching and antibunching behaviors in the scattered photon states. As a concrete example, we discuss in detail with a focus on the three-photon Fock state. Such a capability to generate photonic entanglement from unentangled Fock states will have broad applications in quantum information processing.
Strong coupling between a two-level system (TLS) and bosonic modes produces dramatic quantum optics effects. We consider a one-dimensional continuum of bosons coupled to a single localized TLS, a system which may be realized in a variety of plasmonic, photonic, or electronic contexts. We present the exact many-body scattering eigenstate obtained by imposing open boundary conditions. Multiphoton bound states appear in the scattering of two or more photons due to the coupling between the photons and the TLS. Such bound states are shown to have a large effect on scattering of both Fock- and coherent-state wave packets, especially in the intermediate coupling-strength regime. We compare the statistics of the transmitted light with a coherent state having the same mean photon number: as the interaction strength increases, the one-photon probability is suppressed rapidly, and the two- and three-photon probabilities are greatly enhanced due to the many-body bound states. This results in non-Poissonian light.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
We give an exposure to diagrammatic techniques in waveguide quantum electrodynamics (QED) systems. A particular emphasis is placed on the systems with delayed coherent quantum feedback. Specifically, we show that the N-photon scattering matrices in single-qubit waveguide QED systems, within the rotating wave approximation, admit for a parametrization in terms of ($N\ensuremath{-}1$)-photon effective vertex functions and provide a detailed derivation of a closed hierarchy of generalized Bethe-Salpeter equations satisfied by these vertex functions. The advantage of this method is that the above-mentioned integral equations hold independently of the number of radiation channels, their bandwidth, the dispersion of the modes they are supporting, and the structure of the radiation-qubit coupling interaction, thus enabling one to study multiphoton scattering problems beyond the Born-Markov approximation. Further, we generalize the diagrammatic techniques to the systems containing more than a single emitter by presenting an exact set of equations governing the generic two- and three-photon scattering operators. The above-described theoretical machinery is then showcased on the example of a three-photon scattering on a giant acoustic atom, recently studied experimentally [G. Andersson et al., Nat. Phys. 15, 1123 (2019)].
Waveguide quantum electrodynamics (waveguide QED) describes the interaction between an electromagnetic field confined to a one-dimensional waveguide with atom-like quantum emitters close by. The characteristics of these kinds of systems are the possibility for strong and even ultrastrong interactions between the photonic and atom-like systems, and practically infinite range interactions between the emitters. These properties are valuable for a wide range of quantum optical applications, like quantum communication, quantum networks and quantum metrology. In this thesis we focus on two challenges in quantum optics, namely the generation and scattering of multiphoton states. In the first part of this thesis we demonstrate how waveguide QED systems can be exploited for the generation of multiphoton states, in particular of single-mode Fock states and superpositions thereof as well as multi-mode photonic states with metrological applications. The basic setup for this goal is an ensemble of quantum emitters coupled to a waveguide. In the so-called atomic mirror configuration symmetric Dicke states (or a superposition thereof) decay superradiantly to the ground state and emit the desired multiphoton state, which can be efficiently collected at the ends of the waveguide. We propose various protocols for the preparation of these Dicke states in waveguide QED systems and characterize the emitted photonic state. It turns out that in the low excitation regime, that is, if the number of photons is much lower than the ensemble size, the photonic state is emitted into a single mode. This single-mode structure is fundamental to current proposals for applications in quantum metrology with optical interferometers. Outside the low excitation regime, a multi-mode photonic state is generated, for which the metrological capabilities were unknown. We were able to show that these states still lead to quantum-enhanced optical interferometry. In the second part of this thesis we demonstrate how the scattering of multiphoton states on a single quantum emitter coupled to the waveguide can be used for testing the limits of the light-matter interaction strength. In particular, we investigate systems in the so-called ultrastrong coupling regime, where the coupling strength between the photonic and atom-like system is of the order of the emitter's transition energy. In this regime, many methods and approximations used in quantum optics, especially the Rotating Wave Approximation, break down and one needs to develop new analytical and numerical methods to study these systems. One approach is the so-called polaron Transformation. We show how this transformation can be applied for predicting the scattering amplitude of few photons scattering on the emitter. The comparison of these results with numerical simulations using matrix product states shows a good agreement for moderate coupling strengths. Both parts together show that waveguide QED systems are promising candidates for the generation of multiphoton states as well as for the investigation of fundamental limits probed through the scattering of multiphoton states. The latter also finds application in the implementation of photon-photon nonlinearities induced by the interaction with the quantum emitters. Apart from these and many other theoretical predictions, waveguide QED systems are also undergoing rapid progress in experiments. Therefore, we expect these kinds of systems to bring forth several advances in the field of quantum optics.
We present an exact dissipation model for correlated photon transport in waveguide QED systems. This model rigorously incorporates the infinitely many degrees of freedom of the full three-dimensional photonic scattering channels in the non-excitable ambient environment. We show that the photon leakages to the scattering channels can be accounted for by a reduced Hamiltonian and a restricted eigen-state, with a resultant atomic dissipation. This model is valid for arbitrary photonic Fock and coherent states.
We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.