Quantum information science has vast potential for revolutionary technologies such as communi-cation, computation and precision measurements. One approach in realising these goals is to use single photons, the indivisible quanta of light particles. However, to date, the majority of optical quantum experiments use bulk optical components, and the physical size of these components limit the complexity and stability of those experiments. Recently, there has been a trend to integrate op-tical quantum experiments into monolithic photonic integrated circuits, usually with footprints in the order of centimetres or smaller. One of the challenges is the miniaturisation of non-classical quan-tum light sources, suitable for the on-chip integration with other devices. In in thesis, I will give an overview to the development of quantum optics and integrated photonics, and subsequently discuss different chalcogenide glass and silicon photonic nanostructures for on-chip single-photon generation.
Quantum information science has vast potential for revolutionary technologies such as communi-cation, computation and precision measurements. One approach in realising these goals is to use single photons, the indivisible quanta of light particles. However, to date, the majority of optical quantum experiments use bulk optical components, and the physical size of these components limit the complexity and stability of those experiments. Recently, there has been a trend to integrate op-tical quantum experiments into monolithic photonic integrated circuits, usually with footprints in the order of centimetres or smaller. One of the challenges is the miniaturisation of non-classical quan-tum light sources, suitable for the on-chip integration with other devices. In in thesis, I will give an overview to the development of quantum optics and integrated photonics, and subsequently discuss different chalcogenide glass and silicon photonic nanostructures for on-chip single-photon generation.
Single photons are the smallest indivisible quanta of light, canonically described by quantum mechanics. By carefully controlling the interaction of single photons, exquisite non-classical phenomena can be observed. Mature photonic chip technology has recently emerged as an ideal platform for quantum information processing using single photons. However, generating single photons efficiently on-chip remains a fundamental challenge. One solution is to harness the intrinsic nonlinearity available in certain photonic materials for nonlinear photon generation directly in on-chip waveguides themselves. This work examines nonlinear photon generation in two key material platforms. The first is chalcogenide glass. Chalcogenide, while highly nonlinear, is amorphous and thus has broadband Raman noise. In this study the Raman noise is characterised at the single-photon level to find an intrinsic minima, which is then targeted for low-noise photon generation using an engineered waveguide. The second platform is silicon. As silicon is complementary metal-oxide-semiconductor (CMOS) fabrication compatible, it is congruent with mass production. Thus, in this study, photon-pair generation is first shown in a compact photonic crystal, before combining two monolithic sources using active multiplexing. This thesis presents significant progress towards a key goal of the field – on- demand photon generation in a fully integrated photonic quantum processor.
In the past decades quantum optics has been at the forefront of quantum innovative technologies. For practical applications, scalable platforms for implementation of quantum optical circuits are vital. This thesis presents two new platforms for scalable implementation of quantum optical circuits, namely, modular approach and monolithic integration. Here, we take the first steps towards the integration of three main elements of every quantum optics circuits: Single-photon emitters, single-photon detectors, and quantum logics. Until now, most quantum optical circuits used separate platforms for single-photon generation and detection. The main challenge in the integration of these technologies, which have different requirements, has slowed down the research in the field. Here, we integrate sources and detectors by first fabricating the devices on their own platform and then transferring and combining them together. Plasma enhanced chemical vapor deposition of silicon nitride followed by etching optical waveguides connect these elements. Removing the Poissonian optical excitation field from the quantum circuit is necessary for integration. Classical optical excitation can be avoided if the sources are electrically pumped. However, fabrication of high-quality electrically pumped sources, suitable for integration, has been limited. The experiments described in chapter 4 are our first step towards addressing the mentioned problem. Defect-free nanowires are grown on <100> direction and their optoelectronic performance are characterized. Nanowire quantum dots, thanks to their waveguiding, purity, coherence and their potentials for deterministic integration with other optical circuits, are promising single-photon sources for on-chip quantum optics. However, precise control of the emission energy of the quantum dots by growth has not become possible yet. Chapter 5 describes a method for on-chip tuning of emission energy of nanowire quantum dots using strain fields. We show the emission energy of independent nanowire quantum dots can be brought into degeneracy without affecting their single-photon emission properties. The quantum optical components have to be routed and connected together to form functional circuits. On a chip, this is usually carried out using optical waveguides. Moreover, manipulation of single photons has to be done in a scalable fashion. Again optical waveguides and ring resonators are very good candidates for this task. Therefore, understanding the behavior of these circuits such as their losses, polarization dependence, and temperature behavior is important. The experiment described in chapter 6 studies the behavior of plasma enhanced silicon nitride waveguides in cryogenic temperatures. We concluded in this chapter that due to weak thermo-optic sensitivity of silicon nitride at cryogenic temperatures, the available thermal budget on the system should be carefully considered. An important step in achieving a scalable platform for quantum optical circuits is deterministic and efficient integration of single-photon sources. In chapter 7, we demonstrate successful integration of III-V nanowire quantum dots with silicon nitride waveguides. The nanowires are deterministically selected and transferred from the original growth chip to the new substrate where they are integrated with low-loss silicon nitride waveguides. Our measurements show that the integrated sources preserve their high quality emission properties. In chapter 8, we describe an alternative approach: amodular method for scalable quantum optics. The proposed technique is based on coupling the single-photon from sources into optical fibers where the photons can be processed and then fed into the single-photon detectors. This approach has high flexibility and is easier to implement but as described in the chapter, at the moment, losses in the interfaces between optical fibers and single-photon sources are a major limiting factor. We conclude the thesis with some possible future directions and exciting new results on integration of single-photon detectors with sources and waveguides. Finally, primary results on on-chip single-photon filtering and removal of the optical excitation field are demonstrated.
Nonclassical states of light are an essential resource for many emerging quantum technologies and applications ranging from information processing, encrypted communications, and networking to sensing, metrology, and imaging. Nonlinear optical processes in solid-state materials are widely used for generating quantum light, including single photons, entangled-photon pairs, and quadrature-squeezed states. Recent advances in nonlinear photonics have enabled the functionality of benchtop nonlinear instruments to be scaled down to a single chip without sacrificing efficiency or degrading the key performance metrics. The dramatic improvement in the size, weight, power, cost, and stability enabled by photonic integrated circuits has been essential for enabling the chip-scale generation, manipulation, and detection of quantum light at a steadily increasing degree of complexity and scale. Within the last decade, the authors have seen the progression from few-component photonic circuits operating on two photons to arrays of 18 identical heralded single-photon sources and reconfigurable devices operating with more than 650 components for multidimensional entanglement and arbitrary two-photon quantum gates. In this review, the authors summarize the history and recent key technological developments of chip-scale nonlinear quantum light generation based on integrated nonlinear photonics, recent advances in heterogeneous integrated methods, and approaches for system-level integration and demonstrated applications.
The capability of realizing quantum photonics implementations on-chip will have a strong impact on several aspects of quantum computation and information processing. The implementation of large scale integrated quantum photonic technologies requires on-chip reconfigurable waveguide circuits as well as single-photon sources and detectors. Many successes have been made in recent years to demonstrate complex quantum circuits in many material platforms. Among all these platforms, the Silicon-on-Insulator (SOI) platform is outstanding as it is well developed for classical applications and therefore deploys a high component density, mature fabrication techniques and compatibility with the telecom regime and the complementary metal-oxide-semiconductor (CMOS) technology. However, the lack of on-demand non-classical light sources, directly incorporated in silicon chips, forces the use of nonlinear processes to generate non-classical light states: the probabilistic nature of the emission process sets a limit in the maximally achievable experimental complexity. The use of on-demand sources will have a strong impact on the device’s scalability.
Quantum information science aims to harness uniquely quantum mechanical properties to enhance measurement and information technologies, and to explore fundamental aspects of quantum physics. Of the various approaches to quantum computing [1], photons are particularly appealing for their low-noise properties and ease of manipulation at the single qubit level [2]. Encoding quantum information in photons is also an appealing approach to quantum communication, metrology (eg. [3]), measurement (eg. [4]) and other quantum technologies [5]. However, the implementation of optical quantum circuits with bulk optics has reached practical limits. We have developed an integrated waveguide approach to photonic quantum circuits for high performance, miniaturisation and scalability [6]. Here we report high-fidelity silica-on-silicon integrated optical realisations of key quantum photonic circuits, including two-photon quantum interference and a controlled-NOT logic gate [7]. We have demonstrated controlled manipulation of up to four photons on-chip, including high-fidelity single qubit operations, using a lithographically patterned resistive phase shifter [8]. We have used this architecture to implement a small-scale compiled version of Shorʼs quantum factoring algorithm [9] and demonstrated heralded generation of tuneable four photon entangled states from a six photon input [10]. We have combined waveguide photonic circuits with superconducting single photon detectors [11]. We describe complex quantum interference behaviour in multi-mode interference devices with up to eight inputs and outputs [12], and quantum walks of correlated particles in arrays of coupled waveguides [13]. Finally, we give an overview of our recent work on fundamental aspects of quantum measurement [14,15] and single photon sources [16,17].
Very recently, the interest for quantum technologies by the scientific community and industry has strongly increased. Different types of implementations have been proposed as a practical implementation for a quantum bit as trapped atoms, superconducting qubits and single photons. In particular, we are interested in using single photons and single spins in solid state host matrices such as diamond (nanodiamonds or membranes). Integration of nanosources of light is currently a major bottleneck preventing the realisation of all-photonic chips for quantum technologies and nanophotonics applications. Nanophotonics and integrated optics are vast growing fields with huge market potentials in particular for quantum technologies. Ideally, one needs optical circuitry, on-chip photodetection and on-chip generation of quantum states of light (single photons, entangled photons…). We want to present our recent work on using integrated optics that can offer an easier and robust way to create fixed and compact quantum circuits that can be on chip and scalable. In this context, the coupling between waveguides and single photon emitters is critical. The goal of our research is to efficiently couple single photon emitters with a new platform made of optical glass waveguides. To achieve this goal, several paths are undertaken such as the use of dielectric and plasmonic structuration in order to increase the light interaction with the waveguide or to develop fabrication techniques to insert the emitters directly inside the guide (for nanodiamonds). We will show what is our current state of the art for placing single emitters at the right place on our optical waveguides made of ion-exchange in glass and in particular what can be done to improve our first promising results in order to get near unity coupling between the optical bus and single photon emitters. We will show first results with semiconductor nanocrystals (NCs) but also using nitrogen-vacancy defects in diamond either under nanodiamond form or in thin membranes.