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Optics and Spectroscopy

Observation of parametric nonadiabatic excitation of collective resonances under femtosecond optical pumping of a dense resonant extended medium without population inversion under the conditions of strong light-matter coupling

Sergei N Bagaev, V. S. Egorov, A. A. Pastor, Д. Ю. Преображенский, A. A. Preobrazhenskaya, Pavel Yu. Serdobintsev, Чехонин Игорь Анатольевич, M A Chekhonin

Published Sep 1, 2016• 3 citations
Publisher

Abstract

We experimentally studied the superradiance of the resonant line of rubidium under femtosecond optical pumping of a dense extended medium without population inversion under conditions of strong lightmatter coupling. Substantial self-splitting of superradiance components is observed.
DOI
10.1134/s0030400x16090034

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We experimentally and theoretically study the interaction of broadband polychromatic laser pulses with an optically dense resonant extended medium without population inversion. Experimental (probe field-pumping beam) measurements of the transmission and amplification spectra were carried out in the plasma of a positive neon glow-discharge column containing a large number of metastable atoms. The strong coupling in the field-matter system and the collective behavior of the atomic system in a resonant field were attributable to a high (∼10 12 cm −3 ) density of atoms at the lower (metastable) level of the optical transitions under consideration and to a relatively low intensity of the interacting laser beams. We observed a broadband weakening of the probe field in the absence of pumping and its strengthening in the line wings in the presence of a strong field. We develop a theoretical model for the parametric amplification of collective interactions in dense extended media based on the solution of the semiclassical Maxwell-Bloch equations for conditions under which the pumping field does not destroy the dipole interaction between atoms through probe-field photons.
The nonstationary pump-probe interaction between short laser pulses propagating in a resonant optically dense coherent medium is considered. Special attention is paid to the case where the density of two-level particles is high enough that a considerable part of the energy of relatively weak external laser fields can be coherently absorbed and reemitted by the medium. Thus, the field of the medium reaction plays a key role in the interaction processes, which leads to collective behavior of an atomic ensemble in the strongly coupled light-matter system. Such behavior results in fast excitation interchanges between the field and a medium in the form of optical ringing, which is analogous to polariton beating in solid-state optics. This collective oscillating response, which can be treated as successive beats between light wave packets of different group velocities, is shown to significantly affect the propagation and amplification of the probe field under its nonlinear interaction with a nearly copropagating pump pulse. Depending on the probe-pump time delay, the probe transmission spectra show the appearance of either a specific doublet or coherent dip. The widths of these features are determined by the density-dependent field-matter coupling coefficient and increase during the propagation. Besides that, the widths of the coherent features, which appear close to resonance in the broadband probe spectrum, exceed the absorption-line width, since under the strong-coupling regime, the frequency of optical ringing exceeds the rate of incoherent relaxation. Contrary to stationary strong-field effects, the density- and coordinate-dependent transmission spectra of the probe manifest the importance of collective oscillations and cannot be obtained in the framework of a single-atom model.
Experimental and theoretical investigation of the coherent propagation and amplification of polychromatic broadband laser pulses in optically dense resonant media without population inversion was carried out for the cases of plasma in a Ne glow discharge and a pulse discharge in Hg-Ar mixture. High density of Ne and Hg atoms in the metastable state (about 1012 cm-3), which was chosen to be the ground state of the two-level system under consideration, leads to the collective behavior of the atomic system in resonant electromagnetic field. The broadband probe field attenuation and the sideband amplification of the probe under the action of the coherent pump were observed. The amplification dependence on the pump intensity was obtained. The model of the parametrically enhanced collective interactions was developed and comparison the experimental data was made.
An experimental and theoretical study of the two-wave interaction (of a probe wave and a pumping wave) of wide-band multimode laser pulses with an optically dense extended resonant medium (metastable neon atoms in a positive glow-discharge column) is presented. Depending on the pumping power and characteristics of the medium, various regimes of interaction between the field and the matter, leading to qualitatively different types of amplification spectra, are realized: a cooperative interaction regime at low pumping powers corresponds to amplification spectra consisting of two peaks, which lie on both sides of the absorption line; in the regime of nonstationary Rabi oscillations (Rabi flopping), the amplification appears in the form of an isolated peak at a frequency close to the resonance in the substance; under certain interaction conditions, a dispersive shape of amplification spectra is observed. A significant gain in the probe field (by several times at a length of 10 cm) is obtained as a result of a nonstationary population inversion upon rotation of the Bloch vector of the resonant medium under the action of a strong pumping field in the course of propagation of the two waves.
Abstract For the first time, it is demonstrated that the magnitude and sign of the effect of “spectral condensation” of a laser pulse at the resonant-transition frequency of a dense medium can be controlled by changing the driving-pulse parameters (chirp, pulse width, and pulse amplitude). In the process of this, importantly, the driving-pulse energy and spectrum remain unchanged. Direct time-resolved measurements revealed an oscillatory character of the induced superradiance of rubidium vapors representing a long train of decaying short pulses. The width and repetition rate of the pulses in the train are determined by atomic density N0 of the medium, while the width of an entire superradiance pulse (10 ps) is considerably larger than that of the driving laser pulse (50 fs).