Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Oxford University Press eBooks

Real-time monitoring of a fluctuating condensate in high-temperature superconductors

L. Perfetti, Bruno Sciolla, Giulio Biroli, Tobias Kampfrath

Published Jun 23, 2016• 0 citations
Publisher

Abstract

This chapter investigates the critical behavior of high-temperature superconductors that are suddenly driven far from equilibrium conditions. Bi2Sr2CaCu2O8+δ is excited with a femtosecond laser pulse, and the subsequent nonequilibrium dynamics of the mid-infrared conductivity is monitored. The collected data allow discrimination of temperature regimes where superconductivity is coherent, fluctuating, or vanishingly small. Above the transition temperature Tc, the recovery to equilibrium conditions displays power-law behavior and scaling properties. Partial agreement is found between the scaling law of the optimal doped sample and the time-dependent Ginzburg–Landau (TDGL) model. Inherent limits of TDGL call for nonequilibrium field theories treating fluctuations, mode coupling, and fast degrees of freedom on an equal footing. These results open a timely connection between superconducting condensates and Bose–Einstein condensates of ultracold atoms.

DOI
10.1093/acprof:oso/9780198768166.003.0009

Related papers

Dynamics of fluctuations in high temperature superconductors far from equilibrium conditions

L. Perfetti, Bruno Sciolla, Giulio Biroli +4 more

Despite extensive work on high-temperature superconductors, the critical behavior of an incipient condensate has so far been studied exclusively under equilibrium conditions. Here, we excite Bi2Sr2CaCu2O8+d with a femtosecond laser pulse and monitor the subsequent nonequilibrium dynamics of the mid-infrared conductivity. Our data allow us to discriminate temperature regimes where superconductivity is either coherent, fluctuating or vanishingly small. Above the transition temperature Tc, we make the striking observation that the relaxation to equilibrium exhibits power-law dynamics and scaling behavior, both for optimally and underdoped superconductors. Our findings can in part be modeled using time-dependent Ginzburg-Landau theory and provide strong indication of universality in systems far from equilibrium.

•Jul 29, 2014•0 citations

Ultrafast Dynamics of Fluctuations in High-Temperature Superconductors Far from Equilibrium

L. Perfetti, Bruno Sciolla, Giulio Biroli +4 more

Despite extensive work on high-temperature superconductors, the critical behavior of an incipient condensate has so far been studied exclusively under equilibrium conditions. Here, we excite Bi(2)Sr(2)CaCu(2)O(8+δ) with a femtosecond laser pulse and monitor the subsequent nonequilibrium dynamics of the midinfrared conductivity. Our data allow us to discriminate temperature regimes where superconductivity is either coherent, fluctuating or vanishingly small. Above the transition temperature T(c), we make the striking observation that the relaxation to equilibrium exhibits power-law dynamics and scaling behavior, both for optimally and underdoped superconductors. Our findings can in part be modeled using time-dependent Ginzburg-Landau theory, and they provide strong indication of universality in systems far from equilibrium.

arXiv:1407.7689•Physical Review Letters•Feb 12, 2015•29 citations

Novel Non–Equilibrium Dynamics in Superconductors: Induced Superconductivity and Higgs Modes

Nikolaj Bittner

This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.

•Jan 1, 2017•0 citations

Nature of the superconducting fluctuations in photoexcited systems

Ryuta Iwazaki, Naoto Tsuji, Shintaro Hoshino

The photoexcited state associated with superconducting fluctuations above the superconducting critical temperature ${T}_{c}$ is studied based on the time-dependent Ginzburg-Landau approach. The excited state is created by an electric-field pulse and is probed by a weak secondary external field, which is treated by the linear response theory mimicking pump-probe spectroscopy experiments. The behavior is basically controlled by two relaxation rates: one is ${\ensuremath{\gamma}}_{1}$ proportional to the temperature measured from the critical point $T\ensuremath{-}{T}_{c}$, and the other is ${\ensuremath{\gamma}}_{2}$ proportional to the excitation intensity of the pump pulse. The excited state approaches the equilibrium state exponentially in a long time $t\ensuremath{\gg}{\ensuremath{\gamma}}_{1}^{\ensuremath{-}1}$, while in the intermediate-time domain we find a power-law or logarithmic decay with different exponents for $t\ensuremath{\ll}{\ensuremath{\gamma}}_{2}^{\ensuremath{-}1}$ and ${\ensuremath{\gamma}}_{2}^{\ensuremath{-}1}\ensuremath{\ll}t\ensuremath{\ll}{\ensuremath{\gamma}}_{1}^{\ensuremath{-}1}$, even though the system is located away from the critical point. This is interpreted as the critical point in equilibrium being extended to a finite region in the excited situation. The parameter dependences on both the pump and probe currents are also systematically studied in all dimensions.

arXiv:1904.05820•Physical review. B./Physical review. B•Sep 20, 2019•5 citations

Disorder Effects on AC Fluctuation Conductivity in High-Tc Superconductors

Bo Zhou

For High-Tc superconductors the fluctuation regime is much wider than conventional superconductors due to the short coherence length and high transition temperature. AC measurements can probe the conductivity at a wide range of frequencies, and therefore provide a test of the scaling properties predicted from theory. The measured critical exponents and width of the fluctuation peak are sample dependent, which suggests that the sample inhomogeneities may play an important role in the critical region. In this thesis we study the effects of disorder on the fluctuation conductivity in the critical regime of zero-field normal-superconducting transition by the time-dependent Ginzburg-Landau theory. We set up a discretized model of the superconductor and calculate the two-dimensional and three-dimensional scaling function without disorder above Tc. The result of the discretized model deviates slightly from previous theoretical studies of the continuous model, which can be explained by a finite short wavelength cutoff in Ginzburg-Landau theory. Our results agree well with other theoretical investigations on cutoff effects from an analytical approach. Disorder in a superconductor is modeled by a distribution of Tc's at the lattice sites. We add random disorder to a two-dimensional lattice and calculate the scaling functions averaged over 1000 disorder configurations. When disorder is weak, the scaling functions are increased when T is close Tc . At strong disorder anomalous behavior may occur at the region close to Tc.

•Jan 1, 2005•0 citations

Quench–drive spectroscopy of cuprates

Matteo Ballerini Puviani, Dirk Manske

Cuprates are d-wave superconductors which exhibit a rich phase diagram: they are characterized by superconducting fluctuations even above the critical temperature, and thermal disorder can reduce or suppress the phase coherence. However, photoexcitation can have the opposite effect: recent experiments have shown an increasing phase coherence in optimally doped BSCCO with mid-infrared driving. Time-resolved terahertz spectroscopies are powerful techniques to excite and probe the non-equilibrium states of superconductors, directly addressing collective modes, such as amplitude (Higgs) oscillations. In this work, we calculate the full time evolution of the current generated by a cuprate with a quench-drive spectroscopy setup. Analyzing the response in Fourier space with respect to both the real time and the quench-drive delay time, we look for the signature of a transient modulation of higher harmonics, as well as the Higgs mode, in order to characterize the ground state phase. In particular, this approach can provide a smoking gun for induced or increased phase coherence when applied to the pseudogap phase. These results can pave the way for future experimental schemes to characterize and study superconductors alongside incoherent phases and phase transitions, including induced and transient superconductivity.

arXiv:2203.01242•Faraday Discussions•Jan 1, 2022•6 citations
This chapter investigates the critical behavior of high-temperature superconductors that are suddenly driven far from equilibrium conditions. Bi2Sr2CaCu2O8+δ is excited with a femtosecond laser pulse, and the subsequent nonequilibrium dynamics of the mid-infrared conductivity is monitored. The collected data allow discrimination of temperature regimes where superconductivity is coherent, fluctuating, or vanishingly small. Above the transition temperature Tc, the recovery to equilibrium conditions displays power-law behavior and scaling properties. Partial agreement is found between the scaling law of the optimal doped sample and the time-dependent Ginzburg–Landau (TDGL) model. Inherent limits of TDGL call for nonequilibrium field theories treating fluctuations, mode coupling, and fast degrees of freedom on an equal footing. These results open a timely connection between superconducting condensates and Bose–Einstein condensates of ultracold atoms.
Despite extensive work on high-temperature superconductors, the critical behavior of an incipient condensate has so far been studied exclusively under equilibrium conditions. Here, we excite Bi2Sr2CaCu2O8+d with a femtosecond laser pulse and monitor the subsequent nonequilibrium dynamics of the mid-infrared conductivity. Our data allow us to discriminate temperature regimes where superconductivity is either coherent, fluctuating or vanishingly small. Above the transition temperature Tc, we make the striking observation that the relaxation to equilibrium exhibits power-law dynamics and scaling behavior, both for optimally and underdoped superconductors. Our findings can in part be modeled using time-dependent Ginzburg-Landau theory and provide strong indication of universality in systems far from equilibrium.
Despite extensive work on high-temperature superconductors, the critical behavior of an incipient condensate has so far been studied exclusively under equilibrium conditions. Here, we excite Bi(2)Sr(2)CaCu(2)O(8+δ) with a femtosecond laser pulse and monitor the subsequent nonequilibrium dynamics of the midinfrared conductivity. Our data allow us to discriminate temperature regimes where superconductivity is either coherent, fluctuating or vanishingly small. Above the transition temperature T(c), we make the striking observation that the relaxation to equilibrium exhibits power-law dynamics and scaling behavior, both for optimally and underdoped superconductors. Our findings can in part be modeled using time-dependent Ginzburg-Landau theory, and they provide strong indication of universality in systems far from equilibrium.
This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.
The photoexcited state associated with superconducting fluctuations above the superconducting critical temperature Tc{T}_{c}Tc​ is studied based on the time-dependent Ginzburg-Landau approach. The excited state is created by an electric-field pulse and is probed by a weak secondary external field, which is treated by the linear response theory mimicking pump-probe spectroscopy experiments. The behavior is basically controlled by two relaxation rates: one is ${\ensuremath{\gamma}}_{1}$ proportional to the temperature measured from the critical point $T\ensuremath{-}{T}_{c}$, and the other is ${\ensuremath{\gamma}}_{2}$ proportional to the excitation intensity of the pump pulse. The excited state approaches the equilibrium state exponentially in a long time $t\ensuremath{\gg}{\ensuremath{\gamma}}_{1}^{\ensuremath{-}1}$, while in the intermediate-time domain we find a power-law or logarithmic decay with different exponents for $t\ensuremath{\ll}{\ensuremath{\gamma}}_{2}^{\ensuremath{-}1}$ and ${\ensuremath{\gamma}}_{2}^{\ensuremath{-}1}\ensuremath{\ll}t\ensuremath{\ll}{\ensuremath{\gamma}}_{1}^{\ensuremath{-}1}$, even though the system is located away from the critical point. This is interpreted as the critical point in equilibrium being extended to a finite region in the excited situation. The parameter dependences on both the pump and probe currents are also systematically studied in all dimensions.
For High-Tc superconductors the fluctuation regime is much wider than conventional superconductors due to the short coherence length and high transition temperature. AC measurements can probe the conductivity at a wide range of frequencies, and therefore provide a test of the scaling properties predicted from theory. The measured critical exponents and width of the fluctuation peak are sample dependent, which suggests that the sample inhomogeneities may play an important role in the critical region. In this thesis we study the effects of disorder on the fluctuation conductivity in the critical regime of zero-field normal-superconducting transition by the time-dependent Ginzburg-Landau theory. We set up a discretized model of the superconductor and calculate the two-dimensional and three-dimensional scaling function without disorder above Tc. The result of the discretized model deviates slightly from previous theoretical studies of the continuous model, which can be explained by a finite short wavelength cutoff in Ginzburg-Landau theory. Our results agree well with other theoretical investigations on cutoff effects from an analytical approach. Disorder in a superconductor is modeled by a distribution of Tc's at the lattice sites. We add random disorder to a two-dimensional lattice and calculate the scaling functions averaged over 1000 disorder configurations. When disorder is weak, the scaling functions are increased when T is close Tc . At strong disorder anomalous behavior may occur at the region close to Tc.
Cuprates are d-wave superconductors which exhibit a rich phase diagram: they are characterized by superconducting fluctuations even above the critical temperature, and thermal disorder can reduce or suppress the phase coherence. However, photoexcitation can have the opposite effect: recent experiments have shown an increasing phase coherence in optimally doped BSCCO with mid-infrared driving. Time-resolved terahertz spectroscopies are powerful techniques to excite and probe the non-equilibrium states of superconductors, directly addressing collective modes, such as amplitude (Higgs) oscillations. In this work, we calculate the full time evolution of the current generated by a cuprate with a quench-drive spectroscopy setup. Analyzing the response in Fourier space with respect to both the real time and the quench-drive delay time, we look for the signature of a transient modulation of higher harmonics, as well as the Higgs mode, in order to characterize the ground state phase. In particular, this approach can provide a smoking gun for induced or increased phase coherence when applied to the pseudogap phase. These results can pave the way for future experimental schemes to characterize and study superconductors alongside incoherent phases and phase transitions, including induced and transient superconductivity.