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New Journal of Physics

Multimode theory of single-photon subtraction

Valentin Averchenko, Clément Jacquard, Valérian Thiel, Claude Fabre, Nicolas Treps

Published Aug 25, 2016• 47 citations
Publisher

Abstract

We develop a general theory to describe the manipulation of a multimode quantum state of light via the subtraction of a single photon. The theory is applicable for various types of subtraction schemes independent of the physical nature of the light modes, their number or the embedded quantum states. We show that different subtraction schemes can be described in a unified approach through the characterization of their intrinsic subtraction modes. The conditional state of the multimode quantum light after the photon subtraction is defined by the number of subtraction modes and their matching with the light modes. We propose the manipulation of light states by controlling the subtraction modes. Performing a photon subtraction on a multimode quantum resource is promising for the implementation of a number of quantum information protocols in all-optical, multiplexed and scalable way.

DOI
10.1088/1367-2630/18/8/083042

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We develop a general theory to describe the manipulation of a multimode quantum state of light via the subtraction of a single photon. The theory is applicable for various types of subtraction schemes independent of the physical nature of the light modes, their number or the embedded quantum states. We show that different subtraction schemes can be described in a unified approach through the characterization of their intrinsic subtraction modes. The conditional state of the multimode quantum light after the photon subtraction is defined by the number of subtraction modes and their matching with the light modes. We propose the manipulation of light states by controlling the subtraction modes. Performing a photon subtraction on a multimode quantum resource is promising for the implementation of a number of quantum information protocols in all-optical, multiplexed and scalable way.
The subtraction of a single photon from a multimode quantum field is analyzed as the conditional evolution of an open quantum system. We develop a theory describing different subtraction schemes in a unified approach and we introduce the concept of subtraction modes intrinsic to the process. The matching between the subtraction modes and the modes of the field defines different possible scenarios for the photon subtraction. In particular, our framework identifies: the conditions of pure photon subtraction, the quantum states of the field modes conditioned to the photon subtraction, the mode with the highest fidelity with a single-photon state when the subtraction is performed on multimode squeezed light. We use our theory to analyze the photon subtraction from a highly multimode quantum resource - a train of quantum squeezed or correlated optical pulses. Performing the photon subtraction optimally on various multimode light field has the potential to implement a number of quantum information protocols in a multiplexed and scalable way.
During this thesis, we have built and characterized a single-photon subtractor to engineer the quantum states of light. The aim is to perform a pure and spectrally selective photon subtraction on a multimode resource in the spectral domain. This subtractor consists in a parametric sum-frequency interaction between a signal beam and a control beam within a non-linear medium. The optical spectrum of the control beam is shaped using ultrafast pulse shaping. The up-converted photon is filtered and detected by a single-photon detector. The subtractor is therefore the combination of all these successive elements. We have developed a theoretical framework to describe the multimode subtraction of a single photon and showed that it can be summed up by a subtraction matrix in a modal basis independently of the physical implementation. Thanks to this formalism, we have shown that the process can be characterized without measuring the transformed signal beam but simply by using a probe beam whose pulses are also shaped. We carried out a process tomography at the single-photon level for a wide range of different control beams. Our results are correctly described by the theory we developed and demonstrates the purity of the process as well as the agility of the technique we used.
This paper establishes a versatile theoretical framework that explicitly describes single-photon subtraction from multimode quantum light in the context of non-Gaussian state generation and manipulation. The treatment focuses on easy-to-implement configurations in which no mode-selective operation is available and evaluates features and advantages of schemes where only simple filtering stages are employed on the experiments. Such configuration, by considerably reducing the experimental overheads, makes experiments involving single-photon subtraction easier to be implemented. The obtained theoretical framework allows retrieving, given a multimode input state, optimal conditions required to herald and then to detect non-Gaussian states, providing a practical and powerful toolbox for experiments' design. The application of the proposed approach to the case study of Schr\"odinger cat state preparation starting from a frequency multimode squeezed state illustrates the impact of the derived theoretical tools.
Single-photon subtraction plays important roles in optical quantum information processing as it provides a non-Gaussian characteristic in continuous-variable quantum information.While the conventional way of implementing single-photon subtraction based on a low-reflectance beam splitter works properly for a single-mode quantum state, it is unsuitable for a multimode quantum state because a single photon is subtracted from all multiple modes without maintaining their mode coherence.Here, we experimentally implement and characterize a mode-tunable coherent single-photon subtractor based on sum-frequency generation.It can subtract a single photon exclusively from one desired time-frequency mode of light or from a coherent superposition of multiple time-frequency modes.To experimentally characterize the time-frequency modes of the single-photon subtractor, we employ quantum process tomography based on coherent states.The mode-tunable coherent single-photon subtractor will be an essential element for realizing non-Gaussian quantum networks necessary to get a quantum advantage in information processing.
Multimode photon subtraction provides an experimentally feasible option to construct large non-Gaussian quantum states in continuous variable quantum optics. The non-Gaussian features of the state can lead towards the more exotic aspects of quantum theory, such as negativity of the Wigner function. However, the payoff for states with such delicate quantum properties is their sensitivity to decoherence. In this paper, we present a general model that treats the most important source of decoherence in a purely optical setting: losses. We use the framework of open quantum systems and master equations to describe losses in nnn-photon-subtracted multimode states, where each photon can be subtracted in an arbitrary mode. As a main result, we find that mode-dependent losses and photon subtraction generally do not commute. In particular, the losses do not only reduce the purity of the state, they also change the modal structure of its non-Gaussian features. We then conduct a detailed study of single-photon subtraction from a multimode Gaussian state, which is a setting that lies within the reach of present-day experiments.
The nature of a quantum network, in particular in the continuous variable regime, is governed not only by the light quantum state but also by the measurement process. It can then be chosen after the light source has been generated. Multimode entanglement is not anymore an intrinsic property of the source but a complex interplay between source, measurement and eventually post processing. This new avenue paves the way for adaptive and scalable quantum information processing. However, to reach this ambitious goal, multimode degaussification has to be implemented. Single-photon subtraction and addition have proved to be such key operations, but are usually performed with linear optics elements on single-mode resources. We present a device able to perform mode dependant non Gaussian operation on a spectrally multimode squeezed vacuum states. Sum frequency generation between the state and a bright control beam whose spectrum has been engineered through ultrafast pulse-shaping is performed. The detection of a single converted photon heralds the success of the operation. The resulting multimode quantum state is analysed with standard homodyne detection whose local oscillator spectrum is independently engineered. The device can be characterized through quantum process tomography using weak multimode coherent states as inputs. Its single-mode character can be quantified and its inherent subtraction modes can be measured. The ability to simultaneously control the state engineering and its detection ensures both flexibility and scalability in the production of highly entangled non-Gaussian quantum states.