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Laser cooling of lithium atoms by a strong standing wave

J. J. Tollett, Jian Chen, C. C. Bradley, Nicholas W. M. Ritchie, J. G. Story, Randall G. Hulet

Published May 21, 1990• 0 citations
OpenAlex

Abstract

An atom moving in a strong standing wave radiation field may be translationally cooled by the induced or dipole force.1 The dipole force is proportional to I1/2, where I is the laser intensity, whereas the Doppler (usual) cooling force saturates with increasing I. Since laser sources can provide intensities which are much greater than the saturation intensities of many atomic transitions, cooling via the dipole force can be much more efficient than Doppler cooling. The dipole force has been used to cool the transverse2,3 and the longitudinal4 velocities of atoms in an atomic beam.

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We propose an efficient method of cooling atoms in a strong Gaussian standing wave. The steep gradients of the atomic potential energy give rise to large dipole forces, which can be much stronger than the maximum radiation pressure force and can therefore stop atoms in a much shorter distance. We have simulated the cooling process using a semi-classical Monte- Carlo method, which includes the radial motion, in addition to the motion along the beams. Both motions are calculated directly without separation the dynamics into force and diffusion terms. To cool a large range of atomic velocities the frame in which the standing wave is at rest was swept by changing the frequencies of the counter-propagating beams, in a similar way to the well-known chirp cooling technique using the radiation pressure force. If the curvature of Gaussian beams far from beam waist is employed the radial motion and velocities can be reduced even for the blue detuning comparing to the near waist case. The simulations show that it is possible to stop caesium atoms in a distance of several centimeters (the exact value depends on the laser power, beam waist radius and acceptable chirping force) starting from the most probable velocity at room temperature. Narrower radial and wider axial velocity distribution was obtained for red detuning comparing with the blue one.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jan 1, 1998•3 citations
An atom moving in a strong standing wave radiation field may be translationally cooled by the induced or dipole force.1 The dipole force is proportional to I1/2, where I is the laser intensity, whereas the Doppler (usual) cooling force saturates with increasing I. Since laser sources can provide intensities which are much greater than the saturation intensities of many atomic transitions, cooling via the dipole force can be much more efficient than Doppler cooling. The dipole force has been used to cool the transverse2,3 and the longitudinal4 velocities of atoms in an atomic beam.
The dressed atom approach is used to investigate the evolution of atoms moving in an intense standing wave laser field. When coherences between the dressed states can be neglected, a simple expression is obtained for the radiative force acting on the atoms. The Landau-Zener model, well-known in the theory of slow atomic collisions, is here used to include coherences in an analytic treatment. At high velocities, where the simplest approach breaks down, the results are in good agreement with exact numerical calculations. Applications outside the field of laser cooling are discussed.
The effect of the dipole force and its fluctuation on the motion of Li atoms in an intense, one-dimensional, near-resonant standing light wave has been investigated, both theoretically and experimentally. The duration of the interaction of the atoms with the standing wave was varied from several tens of spontaneous emission lifetimes to several hundred. For a standing wave frequency blue-detuned from resonance, diffusive heating can dominate the time-averaged dissipative dipole force so that there is no steady-state momentum distribution. However, for sufficiently large blue detunings the rate of diffusion is so slow that the resulting distribution approaches a quasi-steady state. For red detunings the diffusion is balanced with the force and a true steady-state is achieved. A Monte Carlo method based on the density matrix equations in the dressed-state representation is applied to simulate the atomic motion. The dynamics of atom channeling is studied. One of the important applications of this investigation is adiabatic laser cooling of atoms. Lithium atoms channeled in the nodes of an intense standing wave radiation field are cooled to near the recoil limit, a single photon's momentum hbark\\hbar{k}hbark, by adiabatically reducing the radiation intensity. The final momentum distribution has a narrow component with a root mean squared momentum of 2 hbark\\hbar{k}hbark in one-dimension. The data are compared with the results obtained by the Monte Carlo method. This process may be useful for cooling and increasing the phase-space density of atoms confined in a magnetic trap.
A new method is proposed for laser cooling atoms with Doppler shifts an order of magnitude larger than the homogeneous linewidth of the atomic transition. Two traveling waves cross at a small angle and form standing waves whose wavelength is much longer than that of either traveling wave. This allows one to extend the region in which the laser cooling force is proportional to velocity. The resulting broadband stimulated cooling forces are predicted to stop 0.1% of the flux of a 500-K atomic sodium beam in a distance of 300 μm and a time of a few microseconds. This is more than 100 times faster than current methods. Numerical integration and the method of Gordon and Ashkin have been used to calculate the cooling forces which result when two traveling waves cross at an angle 2a. The stimulated cooling forces are reduced in intensity by sin2a but are proportional to velocity over an interval which is larger by 1/sin a. This allows one to stop a substantial fraction of an atomic beam without chirping the laser or Zeeman tuning the atoms.
The optical forces exerted on a slowly moving two-level atom in a standing wave are profoundly modified when the normal decay rates of the atom are altered. The theory presented in this paper shows that the stimulated emission force becomes dominant at a very low laser intensity. Furthermore, it can change sign to provide an additional cooling force instead of a heating force at laser detunings below the atomic resonance. These phenomena can lead to equilibrium temperatures below the Doppler limit.
A theoretical discussion of laser cooling of multilevel atomic systems using intense, blue detuned laser beams is given. A method based on matrix continued fractions is presented, which enables the efficient calculation of the semi-classical force on a multilevel system. The method is applied to a three-level system driven by one standing wave and one travelling wave. The force curves obtained exhibit strong cooling features. Cooling of the three-level system is simulated using the fully quantum mechanical Monte Carlo wave function technique. The simulation predicts efficient cooling to sub-Doppler temperatures. The three-level model is related to a multilevel cooling experiment performed on sp7\\sp7sp7Li. The experimental results are found to be in reasonable agreement with the three-level model. However, a comparison of the simulation and experiment for a two-level atomic system reveals significant discrepancies, which raises questions about the model and experiment.
We propose an efficient method of cooling atoms in a strong Gaussian standing wave. The steep gradients of the atomic potential energy give rise to large dipole forces, which can be much stronger than the maximum radiation pressure force and can therefore stop atoms in a much shorter distance. We have simulated the cooling process using a semi-classical Monte- Carlo method, which includes the radial motion, in addition to the motion along the beams. Both motions are calculated directly without separation the dynamics into force and diffusion terms. To cool a large range of atomic velocities the frame in which the standing wave is at rest was swept by changing the frequencies of the counter-propagating beams, in a similar way to the well-known chirp cooling technique using the radiation pressure force. If the curvature of Gaussian beams far from beam waist is employed the radial motion and velocities can be reduced even for the blue detuning comparing to the near waist case. The simulations show that it is possible to stop caesium atoms in a distance of several centimeters (the exact value depends on the laser power, beam waist radius and acceptable chirping force) starting from the most probable velocity at room temperature. Narrower radial and wider axial velocity distribution was obtained for red detuning comparing with the blue one.