The optical forces exerted on a slowly moving two-level atom in a standing wave are profoundly modified when the normal decay rates of the atom are altered. The theory presented in this paper shows that the stimulated emission force becomes dominant at a very low laser intensity. Furthermore, it can change sign to provide an additional cooling force instead of a heating force at laser detunings below the atomic resonance. These phenomena can lead to equilibrium temperatures below the Doppler limit.
The optical forces exerted on a slowly moving two-level atom in a standing wave are profoundly modified when the normal decay rates of the atom are altered. The theory presented in this paper shows that the stimulated emission force becomes dominant at a very low laser intensity. Furthermore, it can change sign to provide an additional cooling force instead of a heating force at laser detunings below the atomic resonance. These phenomena can lead to equilibrium temperatures below the Doppler limit.
We have observed a new type of laser cooling1mainly based on stimulated emission, which can be much more efficient than the usual laser cooling, i.e., the so-called radiation pressure optical molasses. This cooling occurs in a strong laser standing wave, detuned blue with respect to the atomic resonance. The force exerted on the atom results from a coherent redistribution of photons between the two running waves forming the standing wave. The cooling process can also be seen in the dressed atom picture as a microscopic realization of the Sisyphus myth: the atoms in this diagram see more uphill parts than downhill parts.
The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.
The process of laser cooling in a quasi resonant standing laser wave is one of the principal techniques of laser cooling of free atoms. It will be shown that the nonlinear interaction between the counter propagating waves in a standing wave have a profound affect on the mechanical manifestations of the light on the atoms. This can be understood simply by noting that in the Two Wave Mixing (TWM) process, a momentum kick of 2ℏk is transferred to the atom, as a photon is absorbed from one wave and emitted into the counter propagating wave. This process is in fact responsible for the so called "Dipole force" Or "Stimulated Molasses" and has been verified experimentally!. However, since the TWM process requires high laser intensity under normal conditions it does not usually lead to lower equilibrium temperatures. Nevertheless, It has been shown that the TWM process can be modified when the normal decay rates of the atom are altered. This modification can give rise to the appearance of the TWM at lower intensity and can even change its lineshape. This in turn have an important implications on the laser cooling process in a standing wave. Among the important effects: (i) The appearance of the stimulated force at lower intensity when the dipole decay rate is increased by dephasing events.(ii) The appearance of a narrow resonance characterized by the ground state decay in an open system. (iii) The modification of the stimulated force when the quantum fluctuations of the vacuum field are modified by quadrature squeezing3. Processes (ii) and (iii) can change the sign of the stimulated force from a heating force to a cooling force at the red side of the atomic resonance and give additional cooling force much larger than the radiation pressure force.
An atom moving in a strong standing wave radiation field may be translationally cooled by the induced or dipole force.1 The dipole force is proportional to I1/2, where I is the laser intensity, whereas the Doppler (usual) cooling force saturates with increasing I. Since laser sources can provide intensities which are much greater than the saturation intensities of many atomic transitions, cooling via the dipole force can be much more efficient than Doppler cooling. The dipole force has been used to cool the transverse2,3 and the longitudinal4 velocities of atoms in an atomic beam.
The process of laser cooling in a quasi resonant standing laser wave is one of the principal technics of laser cooling of atoms. Recent advances in this field include breaking both the "Doppler and the recoil limits". On another front modification of the quantum statistical properties of the "vacuum" fluctuations by squeezing has been achieved in the laboratory. It is, therefore, interesting to find what is the nature of the modification of the laser cooling process when the atoms are also embedded in squeezed vacuum. Such a state can be produced in principle by a degenerate parametric amplifier whose input are vacuum fluctuations. It is shown that due to the modified decay rates of an atom which is embedded in such a state, profound modification of the cooling processes in a standing wave is achieved . Among the important results obtained is the change of sign of the stimulated force from a heating force in normal vacuum to a cooling force in squeezed vacuum. This phenomenon can result in cooling forces more than two orders of magnitude larger than the maximum force in normal vacuum. In this talk the method for calculating the force in squeezed vacuum will be given. The modified force will be compared to the force in normal vacuum and finally the practical implications of these results for laser cooling will be discussed.
Rectified dipole forces1 offer the possibility of providing deep potential wells for neutral atoms. In the intense standing wave, a two-level atom can experience a large dipole force due to the large intensity gradient. However, this force changes sign on the optical wavelength scale, preventing the formation of deep potential wells. If a second, nearly commensurate, standing wave is added, its ac Stark shift causes the effective detuning of the first field to vary on the optical wavelength scale. The resulting change in sign of the detuning can counteract the change in sign of the intensity gradient, causing the force to maintain its sign over many wavelengths (i.e., the force becomes rectified), thereby forming a deep potential well. This rectified force is periodic with the beat wavelength between the two laser fields. In a three-level atom the same basic mechanism applies, but with the advantage that the two frequencies of the bichromatic standing wave can now be tuned dose to resonance with the two transitions of the atom.