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Instabilities, mode coexistence, and bistable behavior in a dye ring laser and an argon-ion laser at low excitation near threshold

Yongqing Li, Changsheng Wang, Yuzhu Wang

Published May 21, 1990• 0 citations
OpenAlex

Abstract

The factors affecting the dynamic instabilities of a cw dye laser operating near threshold are pumping fluctuation, spontaneous emission, nonlinear mode coupling, and spatial hole burning. Several experiments have found the surprising influence of these factors on the photon statistics,1 mode coexistence,2 bistable behavior,3 and sensitivity of intracavity laser spectroscopy4 in standing wave dye lasers.

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Quantum Electronics•Nov 30, 1994•1 citation
The factors affecting the dynamic instabilities of a cw dye laser operating near threshold are pumping fluctuation, spontaneous emission, nonlinear mode coupling, and spatial hole burning. Several experiments have found the surprising influence of these factors on the photon statistics,1 mode coexistence,2 bistable behavior,3 and sensitivity of intracavity laser spectroscopy4 in standing wave dye lasers.
The fluctuation properties of a cw dye laser, pumped by an argon-ion laser, have been investigated by photon-counting and two-time correlation measurements. The results show significant departures from the usual single-mode laser theory in the region of threshold and below. However, there are indications that the departures may be due to extraneous rather than intrinsic effects, and when these effects are subtracted out, the results are in substantial agreement with the predictions of the usual theory.
The spectral and temporal dynamics of a multimode dye laser has been studied theoretically and experimentally. The analytical model includes quantum fluctuations as well as four-wave mixingdue to population pulsations, stimulated Brillouin scattering, and Rayleigh scattering both in a standing-wave linear laser, and in a unidirectional ring laser. The nonlinearity found most important in the multimode dye laser is four-wave mixing due to pulsations of the populationof the upper laser level. Numerical simulations show features that characterize this particular type of mode coupling: broadening of the emission spectrum, oscillations of the light flux in individual laser modes, suppression of certain beat notes. Observations of these features confirm population pulsations dominating the laser dynamics. Four-wave mixing due to population pulsations tends to arrange the phases of the laser modes such as to minimize the pulsations and to limit its own strength.
Stimulated Brillouin scattering in the dye jet inside a linear laser cavity has been investigated and found to be of significant importance for the dynamical behavior of multimode cw dye lasers. At high spectral power densities, it is responsible for a strong coupling of thousands of individual modes into a few mode packets, thus drastically reducing the number of actually existing degrees of freedom of the system. For a decreasing spectral power density, the mode-coupling strength due to stimulated Brillouin scattering lowers, accompanied by an increase of the number of mode packets. At low spectral power densities, additional mode-coupling mechanisms are supposed to account for a stepwise reduction of the number of independently oscillating mode packets. As an interesting application, the spectroscopic technique of intracavity optical-optical double resonance is discussed and demonstrated.
A short-cavity dye laser has been constructed to study fluctuations arising from quantum noise and mode coupling in multimode systems. Typical dye lasers (i.e., long-cavity) have been found to have cw dynamics that are dominated by coherent wave mixing effects.1 The quantum noise in these lasers also manifests itself as a variance in the buildup times of the laser light intensity. Buildup times of singlemode long-cavity lasers have been studied.2 The relative importance of quantum noise is enhanced in short cavities making the turn-on transient the dominant feature in the laser light fluctuations. We have measured the turn-on transient of individual modes from a multimode short-cavity dye laser following sudden turn-on of the pump power. The shortness of the cavity has the effect of making the decay times of the intracavity field and the molecular population similar. The observed buildup and rise times are compared with those predicted by a semiclassical multimode laser theory with stochastic noise added for several pump rates. Moreover, semiregular oscillations of the total intensity have been observed to occur in short bursts separating intervals of nearly constant cw laser output.
A model using rate equations which allow for quantum noise is used to make a theoretical analysis of the steady-state lasing regime of a cw dye laser. Equations describing the laser performance are derived in the adiabatic approximation neglecting spatial inhomogeneities in the burnup of the active medium. An investigation is made of the stability of steady-state multimode laser action and it is found that this is weak in certain modes. Calculations are made of correlation functions describing fluctuations in the numbers of photons in the modes and fluctuations in the total intensity. Although the fluctuations in individual modes are large, the integrated intensity fluctuates negligibly. An analysis is made of the influence of quantum intensity fluctuations on the attainment of maximum sensitivity in intracavity laser spectroscopy.
The stimulated emission threshold of a dye laser was found to depend on the method of formation of a longitudinal pulsed laser beam used as the pump. Excitation with a focused pump beam reduced the lasing threshold. The effect was strongest when the Q factor of the resonator cavity was low. This reduction in the lasing threshold by focusing the pump laser beam was attributed to an increase in the rate of spontaneous emission resulting from lasing of desqueezed states (enhancement of 'zero-field' fluctuations responsible for the appearance of spontaneous emission). An increase in the spontaneous emission rate reduced the buildup time of stimulated emission during the early stages and thus reduced the lasing threshold.