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Cambridge University Press eBooks

Interaction between light and a two-level atom

L. Mandeļ, E. Wolf

Published Sep 29, 1995• 0 citations
Publisher

Abstract

Light is both radiated and absorbed by atoms, and the interaction between the quantized electromagnetic field and an atom represents one of the most fundamental problems in quantum optics. However, real atoms are complicated systems, and even the simplest real atom, the hydrogen atom, has a non-trivial energy level structure. It is therefore often necessary or desirable to approximate the behavior of a real atom by that of a much simpler quantum system. For many purposes only two atomic energy levels play a significant role in the interaction with the electromagnetic field, so that it has become customary in many theoretical treatments to represent the atom by a quantum system with only two energy eigenstates. This is the most basic of all quantum systems, and it generally simplifies the treatment substantially. In a real atom the selection rules limit the allowed transitions between states, so that, in some cases, a certain state may couple to only one other. Moreover, optical pumping techniques have been developed that allow such preferred states to be prepared in the laboratory, and they have been successfully used in experiments (Abate, 1974). The two-level atom approximation is therefore close to the truth and not merely a mathematical convenience in some experimental situations. In the following we begin by developing the algebra for such a two-level atom. Dynamical variables for a two-level atom We consider an atomic quantum system with the two energy levels shown in Fig. 15.1.

DOI
10.1017/cbo9781139644105.016

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Cambridge University Press eBooks•Feb 3, 2011•1 citation
Light is both radiated and absorbed by atoms, and the interaction between the quantized electromagnetic field and an atom represents one of the most fundamental problems in quantum optics. However, real atoms are complicated systems, and even the simplest real atom, the hydrogen atom, has a non-trivial energy level structure. It is therefore often necessary or desirable to approximate the behavior of a real atom by that of a much simpler quantum system. For many purposes only two atomic energy levels play a significant role in the interaction with the electromagnetic field, so that it has become customary in many theoretical treatments to represent the atom by a quantum system with only two energy eigenstates. This is the most basic of all quantum systems, and it generally simplifies the treatment substantially. In a real atom the selection rules limit the allowed transitions between states, so that, in some cases, a certain state may couple to only one other. Moreover, optical pumping techniques have been developed that allow such preferred states to be prepared in the laboratory, and they have been successfully used in experiments (Abate, 1974). The two-level atom approximation is therefore close to the truth and not merely a mathematical convenience in some experimental situations. In the following we begin by developing the algebra for such a two-level atom. Dynamical variables for a two-level atom We consider an atomic quantum system with the two energy levels shown in Fig. 15.1.
Atomic, molecular and optical physics is a field which, during the last few decades, has known spectacular developments in various directions, like nonlinear optics, laser cooling and trapping, quantum degenerate gases, quantum information. Atom–photon interactions play an essential role in these developments. This book presents an introduction to quantum optics which, I am sure, will provide an invaluable help to the students, researchers and engineers who are beginning to work in these fields and who want to become familiar with the basic concepts underlying electromagnetic interactions. Most books dealing with these subjects follow either a semi-classical approach, where the field is treated as a classical field interacting with quantum particles, or a full quantum approach where both systems are quantized. The first approach is often oversimplified and fails to describe correctly new situations that can now be investigated with the development of sophisticated experimental techniques. The second approach is often too difficult for beginners and lacks simple physical pictures, very useful for an initial understanding of a physical phenomenon. The advantage of this book is that it gives both approaches, starting with the first, illustrated by several simple examples, and introducing progressively the second, clearly showing why it is essential for the understanding of certain phenomena. The authors also clearly demonstrate, in the case of non-linear optics and laser cooling, how advantageous it may be to combine both approaches in the analysis of an experimental situation and how one can get from each point of view useful, complementary physical insights.
One of the simplest nontrivial problems involving the atom–field interaction is the coupling of a two-level atom with a single mode of the electromagnetic field. A two-level atom description is valid if the two atomic levels involved are resonant or nearly resonant with the driving field, while all other levels are highly detuned. Under certain realistic approximations, it is possible to reduce this problem to a form which can be solved exactly; allowing essential features of the atom-field interaction to be extracted. In this chapter we present a semiclassical theory of the interaction of a single two-level atom with a single mode of the field in which the atom is treated as a quantum two-level system and the field is treated classically. A fully quantum mechanical theory will be presented in Chapter 6. A two-level atom is formally analogous to a spin-1/2 system with two possible states. In the dipole approximation, when the field wavelength is larger than the atomic size, the atom–field interaction problem is mathematically equivalent to a spin-1/2 particle interacting with a time-dependent magnetic field. Just as the spin-1/2 system undergoes the so-called Rabi oscillations between the spin-up and spin-down states under the action of an oscillating magnetic field, the two-level atom also undergoes optical Rabi oscillations under the action of the driving electromagnetic field. These oscillations are damped if the atomic levels decay. An understanding of this simple model of the atom–field interaction enables us to consider more complicated problems involving an ensemble of atoms interacting with the field.
In the preceding chapters concerning the interaction of a radiation field with matter, we assumed the field to be classical. In many situations this assumption is valid. There are, however, many instances where a classical field fails to explain experimentally observed results and a quantized description of the field is required. This is, for example, true of spontaneous emission in an atomic system which was described phenomenologically in Chapter 5. For a rigorous treatment of the atomic level decay in free space, we need to consider the interaction of the atom with the vacuum modes of the universe. Even in the simplest system involving the interaction of a single-mode radiation field with a single two-level atom, the predictions for the dynamics of the atom are quite different in the semiclassical theory and the fully quantum theory. In the absence of the decay process, the semiclassical theory predicts Rabi oscillations for the atomic inversion whereas the quantum theory predicts certain collapse and revival phenomena due to the quantum aspects of the field. These interesting quantum field theoretical predictions have been experimentally verified. In this chapter we discuss the interaction of the quantized radiation field with the two-level atomic system described by a Hamiltonian in the dipole and the rotating-wave approximations. For a single-mode field it reduces to a particularly simple form. This is a very interesting Hamiltonian in quantum optics for several reasons. First, it can be solved exactly for arbitrary coupling constants and exhibits some true quantum dynamical effects such as collapse followed by periodic revivals of the atomic inversion.
Interactions of a quantized electromagnetic field In the preceding chapters we have studied the quantum properties of the electromagnetic field, but we have treated it as a free or non-interacting quantum system until now. However, both the emission and the absorption of light imply interactions with other quantum systems, and we now turn to the treatment of such interaction problems. It is true that, to a limited extent, we have already succeeded in treating some interactions of light in previous chapters, without invoking the full apparatus of the quantum theory of interacting systems. For example, in Chapter 9 the electromagnetic field was treated as a classical potential acting on an atomic quantum system, and in Sections 12.2 and 12.9 we invoked simple heuristic arguments to describe the operation of certain optical detectors. But these are limited applications, and, in any case, the validity of results obtained in this way needs to be confirmed. To describe the state of a quantized electromagnetic field (F) in interaction with some other quantum system (A), we evidently require an enlarged, or product Hilbert space, which encompasses both F and A, of which the Hilbert spaces of F and A are subspaces. We shall find it convenient to refer to the other system A as an ‘atomic system’, simply to give a name, without restricting the nature of A. The dynamical variables of the field Ô F( t ) and of the atomic system Ô A( t ) commute at the same time t , and at the beginning, when the interaction between them is assumed to be turned on, each operator acts only on the state vectors within its respective Hilbert space.
The two-level atom can, for good reason, be considered the basic material structure for the study of quantum optics [1]. The two-level atom has played a fundamental role in studies of physical processes, including self-induced transparency (SIT), photon echoes, optical nutation, saturation spectroscopy, and, most recently, slow- and fast-light research. This latter field has recently been the subject of great activity, as researchers have learned how to utilize various physical processes to exert control over the velocity of propagation of light pulses through material systems [2]. This interest stems both from the intellectual intrigue in situations in which the velocity of light can be speeded up or slowed down by many orders of magnitude and the promise that such techniques might be useful for applications in fields such as telecommunications and optical computing [3‐6]. Most of the recent work in this field has made use of the process of electromagnetically induced transparency (EIT) to induce a narrow transparency region in an otherwise highly absorbing optical material [7, 8]. The rapid variation of the refractive index n associated with this transparency window then leads to a strong modification of the group velocity n g in accordance with the standard relation
The analysis in Chapter 3 used a phenomenological form of the permittivity to describe active materials. A proper understanding of optical amplification requires a quantum-mechanical approach for describing the interaction of light with atoms of an active medium [1]. However, even a relatively simple atom such as hydrogen or helium allows so many energy transitions that its full description is intractable even with modern computing machinery [2, 3]. The only solution is to look for idealized models that contain the most essential features of a realistic system. The semiclassical two-level-atom model has proven to be quite successful in this respect [4]. Even though a real atom has infinitely many energy levels, two energy levels whose energy difference nearly matches the photon energy suffice to understand the interaction dynamics when the atom interacts with nearly monochromatic radiation. Moreover, if the optical field contains a sufficiently large number of photons (> 100), it can be treated classically using a set of optical Bloch equations. In this chapter, we learn the underlying physical concepts behind the optical Bloch equations. We apply these equations in subsequent chapters to actual optical amplifiers and show that they can be solved analytically under certain conditions to provide a realistic description of optical amplifiers. It is essential to have a thorough understanding of the concept of a quantum state [5]. To effectively use the modern machinery of quantum mechanics, physical states need to be represented as vectors in so-called Hilbert space [6].