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Whispering-Gallery Mode Resonators For Nonlinear And Quantum Optical Applications

Matthew T. Simons

Published Jan 1, 2014• 1 citation
Publisher

Abstract

Quantum information is the next frontier in communications. to realize quantum communications, the quantum mechanical properties of today's best communication medium, light, must be harnessed in a scalable and efficient manner. Whispering-gallery mode resonators (WGMRs), a type of optical cavity, have advantages over traditional designs that can enhance processes used in the generation of nonclassical (quantum) states of light. In particular they reduce the power threshold for intensity-dependent nonlinear phenomena. One such process, second harmonic generation, can reduce the shot noise of light below the standard quantum limit. This dissertation explores the theoretical analysis and experimental tests of noise reduction through second harmonic generation in a crystalline whispering-gallery mode resonator. We also observe the generation of another nonlinear optical process, hyper-Raman scattering, at modest optical powers inside a crystalline WGMR. The change in optical properties of vanadium dioxide due to an optically-induced phase transition is also studied as a potential Q-switching material in a WGMR-type cavity.

DOI
10.21220/s2-kw9e-9360

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Quantum information is the next frontier in communications. to realize quantum communications, the quantum mechanical properties of today's best communication medium, light, must be harnessed in a scalable and efficient manner. Whispering-gallery mode resonators (WGMRs), a type of optical cavity, have advantages over traditional designs that can enhance processes used in the generation of nonclassical (quantum) states of light. In particular they reduce the power threshold for intensity-dependent nonlinear phenomena. One such process, second harmonic generation, can reduce the shot noise of light below the standard quantum limit. This dissertation explores the theoretical analysis and experimental tests of noise reduction through second harmonic generation in a crystalline whispering-gallery mode resonator. We also observe the generation of another nonlinear optical process, hyper-Raman scattering, at modest optical powers inside a crystalline WGMR. The change in optical properties of vanadium dioxide due to an optically-induced phase transition is also studied as a potential Q-switching material in a WGMR-type cavity.
High- and ultrahigh-Q whispering-gallery mode resonators have the capability to trap photons by total internal reflection for a duration ranging from nanoseconds to milliseconds. These exceptionally long photon lifetimes enhance the light–matter interactions at all scales, namely at the electronic, molecular, and lattice levels. As a consequence, nonlinear photon scattering can be triggered with very low threshold powers, down to a few microwatts. The possibility to efficiently harness photon–photon interactions with a system optimizing size, weight, power, and cost constraints has created a new, quickly thriving research area in photonics science and technology. This topic is inherently cross-disciplinary, as it stands at the intersection of nonlinear and quantum optics, crystallography, optoelectronics, and microwave photonics. From a fundamental perspective, high-Q whispering-gallery mode resonators have emerged as an ideal platform to investigate light–matter interactions in nonlinear bulk materials. From an applied viewpoint, technological applications include time-metrology, aerospace engineering, coherent optical fiber communications, or nonclassical light generation, among others. The aim of this paper is to provide an overview of the most recent advances in this area, which is increasingly gaining importance in contemporary photonics.
Efficient generation of harmonics in nonlinear optical resonators, particularly in whispering-gallery-mode (WGM) resonators, has led to successes such as parametric oscillators, narrow-band single-photon sources, and versatile frequency converters. A subtle problem, though, has strongly limited efficiency and hindered precise out-coupling of the generated light. Implementing their own prior theory and a polarization-selective birefringent coupling prism, the authors demonstrate an improvement of more than an order of magnitude in the amount of out-coupled light. The results are particularly interesting for applications in quantum optics relying on WGMs.