We investigate the cooperative behavior of regular monolayers of driven two-level dipoles, using classical electrodynamics simulations. The dipolar response results from the interference of many cooperative eigenmodes, each frequency-shifted from the single resonant dipole case, and with a modified lifetime, due to the interactions between dipoles. Of particular interest is the kagome lattice, where the semiregular geometry permits simultaneous excitation of two dominant modes, one strongly subradiant, leading to an electromagnetically induced transparencylike interference in a two-level system. The interfering modes are associated with ferroelectric and antiferroelectric ordering in alternate lattice rows with long-range interactions.
The spectrum of resonance fluorescence and the second-order correlation function are calculated for a system of two identical two-level cooperative systems interacting via the dipole-dipole interaction. The results are valid for arbitrary incident-field strengths and for atomic separations much less than the resonant wavelength. The intensity of the sidebands at the Rabi frequency is diminished by the dipole interaction, whereas that of the sidebands at twice the Rabi frequency is enhanced. Both the cooperative behavior and the dipole-dipole interaction act to diminish the photon antibunching, as shown by the second-order correlation function.
We investigate the effect of the dipole-dipole interaction on the quantum jump statistics of three atoms. This is done for three-level systems in a
V configuration and in what may be called a
D configuration. The transition rates between the four different intensity periods are calculated in closed form. Cooperative effects are shown to increase by a factor of 2 compared to two of either three-level systems. This results in transition rates that are, for distances of about one wavelength of the strong transition, up to 100% higher than for independent systems. In addition the double and triple jump rates are calculated from the transition rates. In this case cooperative effects of up to 170% for distances of about one wavelength and still up to 15% around 10 wavelengths are found. Nevertheless, for the parameters of an experiment with
Hg+ ions the effects are negligible, in agreement with the experimental data. For three
Ba+ ions this seems to indicate that the large cooperative effects observed experimentally cannot be explained by the dipole-dipole interaction.