A master equation for strongly interacting dipoles

Kristofor B. Nyquist

Adam Stokes, Ahsan Nazir

We consider a pair of dipoles such as Rydberg atoms for which direct electrostatic dipole–dipole interactions may be significantly larger than the coupling to transverse radiation. We derive a master equation using the Coulomb gauge, which naturally enables us to include the inter-dipole Coulomb energy within the system Hamiltonian rather than the interaction. In contrast, the standard master equation for a two-dipole system, which depends entirely on well-known gauge-invariant S -matrix elements, is usually derived using the multipolar gauge, wherein there is no explicit inter-dipole Coulomb interaction. We show using a generalised arbitrary-gauge light-matter Hamiltonian that this master equation is obtained in other gauges only if the inter-dipole Coulomb interaction is kept within the interaction Hamiltonian rather than the unperturbed part as in our derivation. Thus, our master equation depends on different S -matrix elements, which give separation-dependent corrections to the standard matrix elements describing resonant energy transfer and collective decay. The two master equations coincide in the large separation limit where static couplings are negligible. We provide an application of our master equation by finding separation-dependent corrections to the natural emission spectrum of the two-dipole system.

Bassano Vacchini

Peter G. Brooke, Karl-Peter Marzlin, James D. Cresser +1 more

We analyze the stability of super- and subradiant states in a system of identical two-level atoms in the near-Dicke limit, i.e., when the atoms are very close to each other compared to the wavelength of resonant light. The dynamics of the system are studied using a renormalized master equation, both with multipolar and minimal-coupling interaction schemes. We show that both models lead to the same result and, in contrast to nonrenormalized models, predict that the relative orientation of the (coaligned) dipoles is unimportant in the Dicke limit. Our master equation is of relevance to any system of dipole-coupled two-level atoms, and gives bounds on the strength of the dipole-dipole interaction for closely spaced atoms. Exact calculations for small atom systems in the near-Dicke limit show the increased emission times resulting from the evolution generated by the strong dipole-dipole interaction. However, for large numbers of atoms in the near-Dicke limit, it is shown that as the number of atoms increases, the effect of the dipole-dipole interaction on collective emission is reduced.

Wen-Xuan Zhang, Lei Tan

Based on the master-equation approach, we investigate the dynamics of two dipole-coupled atoms by examining the atomic population and entanglement evolution. We show that the population decays rapidly and the entanglement is inhibited when the pump field is weak, while for the strongly pumped case, the evolution of population and entanglement is similar to one driven in the classical field. Furthermore, the evolution of the population can be controlled by the dipole–dipole interaction and detunings.

W. Cassing