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Springer eBooks

Adiabatic Population Inversion in Multilevel Systems

J. Oreg, F. T. Hioe, Joseph H. Eberly

Published Jan 1, 1984• 0 citations
Publisher
DOI
10.1007/978-1-4757-0605-5_145

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We applied our pictorial approach using the fundamental concept of the Hückel molecular orbital theory to the population inversion in the multilevel systems by the straddling-STIRAP (S-STIRAP). We showed that the mechanism of the population inversion in the multilevel system may be easily understood by our approach. It is also shown that our approach is useful to understand that the condition required for the laser frequency in the delayed pulse sequence is different for the even- and odd-level systems. © 2000 John Wiley & Sons, Inc. Int J Quant Chem 80: 1068–1075, 2000

International Journal of Quantum Chemistry•Jan 1, 2000•3 citations
A numerical analysis is presented of several potential pulsed-laser applications of adiabatic population inversion in atoms or molecules. A simple numerical method is demonstrated for evaluating adiabatic processes in multilevel systems for both swept-frequency and resonant, time-delayed pulses. Adiabatic inversion with time-delayed pulses is generalized to systems with any number of levels. The effect of Doppler broadening on time-delayed adiabatic pumping of a three-level system is investigated.
We applied our pictorial approach using the fundamental concept of the Hückel molecular orbital theory to the population inversion in the multilevel systems by the straddling-STIRAP (S-STIRAP). We showed that the mechanism of the population inversion in the multilevel system may be easily understood by our approach. It is also shown that our approach is useful to understand that the condition required for the laser frequency in the delayed pulse sequence is different for the even- and odd-level systems. © 2000 John Wiley & Sons, Inc. Int J Quant Chem 80: 1068–1075, 2000