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ACS symposium series

Optimal Quantum Control in Dissipative Environments: General Formalism and Perturbative Limits

Seogjoo Jang, Jianshu Cao

Published Jun 21, 2002• 0 citations
Publisher

Abstract

Optimal quantum control in dissipative environments is formulated combining the optimal control theory from the Wilson group with the projection operator technique. In the weak response limit, a set of formally exact equations defines the optimal weak field for arbitrary target states and arbitrary system-bath interactions. Perturbative approximations are then made to derive general equations for weakly dissipative non-Markovian systems, which are amenable to analytical and/or numerical solutions. Potential applications of these results are discussed.

DOI
10.1021/bk-2002-0821.ch009

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Optimal quantum control in dissipative environments is formulated combining the optimal control theory from the Wilson group with the projection operator technique. In the weak response limit, a set of formally exact equations defines the optimal weak field for arbitrary target states and arbitrary system-bath interactions. Perturbative approximations are then made to derive general equations for weakly dissipative non-Markovian systems, which are amenable to analytical and/or numerical solutions. Potential applications of these results are discussed.
We present a general state-independent optimal control strategy for weakly dissipative quantum systems which allows the identification of Hamilton operators which approximately perform a specified unitary operation and minimize the adverse effects of the dissipative environment. Compared to traditional approaches, it avoids the need for Lagrange multipliers and the repeated solving of the full kinetic equations of the quantum subsystem. This direct method is outlined for a single qubit raealization, such as the spin of an excess electron in a quantum dot or a Josephson qubit. We show that for this system formulated within the Lindblad equation, optimal solutions for arbitrary unitary single-qubit operations may be found analytically provided there is full control over the system Hamiltonian. Absolute bounds for controllability are derived analytically. Numerical implementations of this approach confirm these results and allow an efficient determination of optimal solutions for various dissipators, starting from various initial guesses, both for limited and full control over the Hamiltonian of the quantum system.
A general state-independent optimal control strategy for weakly dissipative quantum systems is presented. It allows the identification of Hamilton operators which approximately perform a preselected unitary operation and minimize the adverse effects from a dissipative environment. This direct method is demonstrated at the example of a single qubit, as realized, for example, by the spin of an excess electron in a quantum dot or a Josephson flux qubit, with Lindblad dissipator. We show that optimal solutions for arbitrary unitary single-qubit operations may be found both analytically and numerically.
This article provides a review of recent developments in the formulation and execution of optimal control strategies for the dynamics of quantum systems. A brief introduction to the concept of optimal control, the dynamics of of open quantum systems, and quantum information processing is followed by a presentation of recent developments regarding the two main tasks in this context: state-specific and state-independent optimal control. For the former, we present an extension of conventional theory (Pontryagin's principle) to quantum systems which undergo a non-Markovian time-evolution. Owing to its importance for the realization of quantum information processing, the main body of the review, however, is devoted to state-independent optimal control. Here, we address three different approaches: an approach which treats dissipative effects from the environment in lowest-order perturbation theory, a general method based on the time--evolution superoperator concept, as well as one based on the Kraus representation of the time-evolution superoperator. Applications which illustrate these new methods focus on single and double qubits (quantum gates) whereby the environment is modeled either within the Lindblad equation or a bath of bosons (spin-boson model). While these approaches are widely applicable, we shall focus our attention to solid-state based physical realizations, such as semiconductor- and superconductor-based systems. While an attempt is made to reference relevant and representative work throughout the community, the exposition will focus mainly on work which has emerged from our own group.
A Markovian master equation describing the evolution of open quantum systems in the presence of a time-dependent external field is derived within the Bloch-Redfield formalism. It leads to a system-bath interaction which depends on the control field. Optimal control theory is used to select control fields which allow accelerated or decelerated system relaxation, or suppression of relaxation (dissipation) altogether, depending on the dynamics we impose on the quantum system. The control-dissipation correlation and the nonperturbative treatment of the control field are essential for reaching this goal. The optimal control problem is formulated within Pontryagin's minimum principle and the resulting optimal differential system is solved numerically. As an application, we study the dynamics of a spin-boson model in the strong coupling regime under the influence of an external control field. We show how trapping the system in unstable quantum states and transfer of population can be achieved by optimized control of the dissipative quantum system. We also used optimal control theory to find the driving field that generates the quantum ZZZ gate. In several cases studied, we find that the selected optimal field which reduces the purity loss significantly is a multicomponent low-frequency field including higher harmonics, all of which lie below the phonon cutoff frequency. Finally, in the undriven case we present an analytic result for the Lamb shift at zero temperature.
Quantum dissipation involves both energy relaxation and decoherence, leading toward quantum thermal equilibrium. There are several theoretical prescriptions of quantum dissipation but none of them is simple enough to be treated exactly in real applications. As a result, formulations in different prescriptions are practically used with different approximation schemes. This review examines both theoretical and application aspects on various perturbative formulations, especially those that are exact up to second-order but nonequivalent in high-order system-bath coupling contributions. Discrimination is made in favor of an unconventional formulation that in a sense combines the merits of both the conventional time-local and memory-kernel prescriptions, where the latter is least favorite in terms of the applicability range of parameters for system-bath coupling, non-Markovian, and temperature. Also highlighted is the importance of correlated driving and dissipation effects, not only on the dynamics under strong external field driving, but also in the calculation of field-free correlation and response functions.
The problem of optimal control of non-Markovian open quantum system via weak measurement is presented. Based on the non-Markovian master equation, we evaluate exactly the non-Markovian effect on the dynamics of the system of interest interacting with a dissipative reservoir. We find that the non-Markovian reservoir has dual effects on the system: dissipation and backaction. The dissipation exhausts the coherence of the quantum system, whereas the backaction revives it. Moreover, we design the control Hamiltonian with the control laws attained by the stochastic optimal control and the corresponding optimal principle. At last, we considered the exact decoherence dynamics of a qubit in a dissipative reservoir composed of harmonic oscillators, and demonstrated the effectiveness of our optimal control strategy. Simulation results showed that the coherence will completely lost in the absence of control neither in non-Markovian nor Markovian system. However, the optimal feedback control steers it to a stationary stochastic process which fluctuates around the target. In this case the decoherence can be controlled effectively, which indicates that the engineered artificial reservoirs with optimal feedback control may be designed to protect the quantum coherence in quantum information and quantum computation.