The subject of this work is the control of the quantum mechanical motional state of trapped neutral Cesium atoms. This is accomplished using a rarely considered method based on microwave radiation in combination with a spin dependent optical lattice potential. The setup used was designed to trap and to store on the order of ten atoms in a one dimensional optical lattice. Fluorescence imaging allows to determine both, the number and the position of the atoms. The spin degree of freedom is manipulated using microwave radiation and the trapping potential allows to shift the atoms to the 'left' or to the 'right' along the potential axis, depending on their spin orientation. A microwave spectrum with a slightly displaced lattice exhibits sideband peaks corresponding to a change of the vibrational quantum number. This is the mechanism which introduces coupling between the spin and the motional degree of freedom. The work draws parallels to the usually used sideband technique based on optical transitions instead of microwaves and exploiting the photon recoil instead of a state dependent potential. Similar to the optical method the microwave based approach allows for the realization of a resolved-sideband cooling technique which efficiently prepares the atomic ensemble in the motional ground state. Starting from this purified quantum mechanical state, other interesting states are prepared using successive sideband transitions. The result of the preparation is probed by implementing filtering schemes for the motional state. With this control technique the experimental setup in total is capable to control the spin, the position along the one dimensional periodic potential and the vibrational state of the atoms.
The subject of this work is the control of the quantum mechanical motional state of trapped neutral Cesium atoms. This is accomplished using a rarely considered method based on microwave radiation in combination with a spin dependent optical lattice potential. The setup used was designed to trap and to store on the order of ten atoms in a one dimensional optical lattice. Fluorescence imaging allows to determine both, the number and the position of the atoms. The spin degree of freedom is manipulated using microwave radiation and the trapping potential allows to shift the atoms to the 'left' or to the 'right' along the potential axis, depending on their spin orientation. A microwave spectrum with a slightly displaced lattice exhibits sideband peaks corresponding to a change of the vibrational quantum number. This is the mechanism which introduces coupling between the spin and the motional degree of freedom. The work draws parallels to the usually used sideband technique based on optical transitions instead of microwaves and exploiting the photon recoil instead of a state dependent potential. Similar to the optical method the microwave based approach allows for the realization of a resolved-sideband cooling technique which efficiently prepares the atomic ensemble in the motional ground state. Starting from this purified quantum mechanical state, other interesting states are prepared using successive sideband transitions. The result of the preparation is probed by implementing filtering schemes for the motional state. With this control technique the experimental setup in total is capable to control the spin, the position along the one dimensional periodic potential and the vibrational state of the atoms.
Spin-dependent optical potentials allow us to use microwave radiation to manipulate the motional state of trapped neutral atoms (Förster et al 2009 Phys. Rev. Lett. 103 233001). Here, we discuss this method in greater detail, comparing it to the widely employed Raman sideband coupling method. We provide a simplified model for sideband cooling in a spin-dependent potential, and we discuss it in terms of the generalized Lamb–Dicke parameter. Using a master equation formalism, we present a quantitative analysis of the cooling performance for our experiment, which can be generalized to other experimental settings. We additionally use microwave sideband transitions to engineer motional Fock states and coherent states, and we devise a technique for measuring the population distribution of the prepared states.
We control the quantum mechanical motion of neutral atoms in an optical lattice by driving microwave transitions between spin states whose trapping potentials are spatially offset. Control of this offset with nanometer precision allows for adjustment of the coupling strength between different motional states, analogous to an adjustable effective Lamb-Dicke factor. This is used both for efficient one-dimensional sideband cooling of individual atoms to a vibrational ground state population of 97% and to drive coherent Rabi oscillation between arbitrary pairs of vibrational states. We further show that microwaves can drive well resolved transitions between motional states in maximally offset, shallow lattices, and thus in principle allow for coherent control of long-range quantum transport.
Optical lattices induced by light detuned far from the frequency of any atomic resonance transition are ideal systems in which to develop techniques for the coherent control of atomic motional and internal states. Decoherence arising from spontaneous emission can be eliminated to an arbitrary degree by varying the detuning of the optical field. The atoms trapped in these lattices are to a large extent isolated from environmental disturbances and from each other. The first step towards the coherent control of atoms in a far-detuned lattice is their preparation in a single motional state. In this thesis the preparation of atoms in the ground vibrational state of a two-dimensional far-detuned optical lattice via resolved-sideband Raman cooling is presented. This sideband-cooling scheme involves stimulated Raman transitions between bound vibrational states of a pair of magnetic ground state sublevels, followed by an irreversible step due to optical pumping, resulting in a net loss of one quantum of vibrational energy per cooling cycle. This process provides efficient cooling in two-dimensions and leads to the accumulation of a large fraction of atoms in the 2-D ground vibrational state of a potential well associated with a single Zeeman substate. Experiments aimed at improving and monitoring the characteristics of the lar-detuned lattice and the sideband-Raman cooling efficiency are also described. Parametric excitation experiments and modelling are employed to investigate the degree of anharmonicity of the optical potential and the importance of heating induced by laser intensity noise, whilst Zeeman-state analysis of the sample is performed for monitoring the distribution of atoms over different magnetic sub- states. Finally, spin-polarization experiments are carried out in order to study the paramagnetic properties of the lattice and lead to an evaluation of a spin-temperature for the sample.
The present work investigates the state-selective transport of single neutral cesium atoms in a one-dimensional optical lattice. It demonstrates experimental applications of this transport, including a single atom interferometer, a quantum walk and controlled two-atom collisions. The atoms are stored one by one in an optical lattice formed by a standing wave dipole trap. Their positions are determined with sub-micrometer precision, while atom pair separations are reliably inferred down to neighboring lattice sites using real-time numerical processing. Using microwave pulses in the presence of a magnetic field gradient, the internal qubit states, encoded in the hyperfine levels of the atoms, can be separately initialized and manipulated. This allows us to perform arbitrary single-qubit operations and prepare arbitrary patterns of atoms in the lattice with single-site precision. Chapter 1 presents the experimental setup for trapping a small number of cesium atoms in a one-dimensional optical lattice. Chapter 2 is devoted to fluorescence imaging of atoms, discussing the imaging setup, numeric methods and their performance in detail. Chapter 3 focuses on engineering of internal states of trapped atoms in the lattice using optical methods and microwave radiation. It provides a detailed investigation of coherence properties of our experimental system. Finally manipulation of individual atoms with almost single-site resolution and preparation of regular strings of atoms with predefined distances are presented. In Chapter 4, basic concepts, the experimental realization and the performance of the state-selective transport of neutral atoms over several lattice sites are presented and discussed in detail. Coherence properties of this transport are investigated in Chapter 5, using various two-arms single atom interferometer sequences in which atomic matter waves are split, delocalized, merged and recombined on the initial lattice site, while the interference contrast and the accumulated phase difference are measured. By delocalizing a single atom over several lattice sites, possible spatial inhomogeneities of fields along the lattice axis in the trapping region are probed. In Chapter 6, experimental realization of a discrete time quantum walk on a line with single optically trapped atoms is presented as an advanced application of multiple path quantum interference in the context of quantum information processing. Using this simple example of a quantum walk, fundamental properties of and differences between the quantum and classical regimes are investigated and discussed in detail. Finally, by combining preparation of atom strings, position-dependent manipulation of qubit states and state-selective transport, in Chapter 7, two atoms are deterministically brought together into contact, forming a starting point for investigating two-atom interactions on the most fundamental level. Future prospects and suggestions are finally presented in Chapter 8.
Advances in the preparation and detection, but most importantly in the coherent manipulation of single neutral atoms have allowed the observation of intriguing phenomena of quantum physics in recent years. We discuss developments to prepare and detect single neutral atoms in a one-dimensional optical lattice potential with single site resolution. Moreover, using two different experimental techniques, a state-dependent optical lattice potential on the one hand and a high-finesse optical cavity on the other hand, we have obtained coherent control over single neutral atoms. The former has enabled us to observe the quantum walk of atoms in position space, and to coherently control the motion of trapped atoms via microwave radiation. The latter offers a means to non-destructively detect the atomic spin state, thereby revealing quantum jumps of single atoms, or the altered optical properties of single atoms when subject to electromagnetically-induced transparency.
This dissertation reports on quantum state preparation of cesium atoms in a two-dimensional optical lattice, by resolved-sideband Raman cooling. An optical lattice is a periodic potential produced by the light shift interaction between an atom and light field. Laser cooled atoms can become strongly localized about the bottom of potential wells in an optical lattice, where they occupy a discrete spectrum of bound vibrational energy levels. The distribution over vibrational levels of atoms in the lattice is characterized by the mean vibrational excitation, n . In an optical lattice, absorption and emission of photons from lattice beams causes n to increase in time. This source of heating is always present, but its rate can be greatly reduced in a lattice detuned far from the atomic resonance. Sideband cooling is an efficient means of transferring atoms from higher into lower-lying vibrational levels and, thus, it reduces n for the ensemble. If the sideband cooling rate is much greater than the heating rate, then n approaches zero and virtually all atoms are in the lowest vibrational level in their potential wells. Our sideband cooling scheme involves stimulated Raman transitions between bound states in the potential wells of a pair of magnetic sublevels, followed by optical pumping, for a net loss of one quantum of vibration per cooling cycle. The process accumulates 98% of atoms in the ground vibrational level of a potential well associated with a single Zeeman substate. Each atom in the lattice is then very close to a pure state. For two-dimensional lattice with sideband cooling we find nx≈ny≈0.008 &parl0;16&parr0; . Various issues related to state preparation and sideband cooling are also discussed in the context of a one dimensional lin ⊥ lin optical lattice. These include improvement of laser cooling in a near resonance lattice by application of weak magnetic fields, transfer of atoms from near into far off-resonance lattices, and heating rates in far off-resonance lattices.