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Conference on Lasers and Electro-Optics

Laser frequency conversion using two-photon emission in barium vapor

Eric J. Korevaar, James J. Silva, C. S. Liu, Kenneth Y. Tang, David L. Huestis

Published Apr 25, 1988• 0 citations
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Lasing in barium vapor in a resonance light field

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Soviet Journal of Quantum Electronics•Feb 1, 1988•0 citations
An experimental investigation was made of stimulated Raman scattering (STRS) of excimer laser radiation in barium, thulium, and europium vapors. The energy of XeF* laser radiation ( λ = 351 nm) converted to the yellow range (585 nm) in barium vapor was 6 mJ and the conversion efficiency was ∼39%. The spectral composition of the converted radiation is governed by the STRS, by four-wave parametric processes, and also by lasing due to the natural barium transition. Selection of the pump frequencies is required to concentrate the converted radiation at a single frequency and to reduce its divergence. Stimulated Raman scattering of XeCl* laser radiation ( λ = 308 nm) was achieved in thulium vapor at λ = 422 nm. In europium vapor in quasiresonance with the 6 s 2 8 S 0 1/2 –5 d 2 10 P 0 11/2 forbidden transition, stimulated emission was obtained due to the natural 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 11/2 and 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 3/2 transitions.
Emission at wavelengths of 1.0615 and 1.074 μ from a self-mode-locked YAG:Nd3+ laser was observed at thresholds which were only 1.5 and 3.5 times higher than the threshold for the emission of radiation with λ = 1.064 μ. Efficient conversion (characterized by a quantum efficiency of ~ 15%) of the third harmonics of the radiations with λ = 1.064 and 1.0615 μ to the visible (590 nm) and ultraviolet (250 nm) ranges was achieved in atomic barium vapor. Electron stimulated Raman scattering due to a strongly forbidden transition in a system of Ba atoms was observed for the first time.