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High resolution field imaging with atomic vapor cells

Andrew Horsley

Published Jan 1, 2015• 1 citation
Publisher

Abstract

In this thesis, I report on the development of imaging techniques in atomic vapor cells. This is a relatively unexplored area, despite the ubiquitous use of imaging in experiments with ultracold atoms. Our main focus is in high resolution imaging of microwave near fields, for which there is currently no satisfactory established technique. We detect microwave fields through Rabi oscillations driven by the microwave on atomic hyperfine transitions. The technique can be easily modified to also image dc magnetic fields. In addition, we have developed techniques to image vapor cell processes such as atomic T1 and T2 relaxation. These provide a new window into vapor cell physics, which we have used to obtain spatially resolved information on Rb interactions with the cell walls, and to estimate the Rb relaxation probability in a collision with the cell wall. \n \nAs a first application of our imaging techniques, we imaged the dc and microwave magnetic fields inside a state-of-the-art vapor cell atomic clock. This new clock characterisation technique should lead to real improvements in clock performance, and is in the process of being adopted by the atomic clock community. \n \nWe have developed a widefield, high resolution imaging setup using a microfabricated vapor cell, which we have used to image microwave and dc magnetic vector fields. With the addition of a 480 nm laser, the setup can be configured to image microwave electric fields. Our camera-based imaging system records 2D images with a 6x6 mm2 field of view at a rate of 10 Hz. It provides up to 50 um spatial resolution, and allows imaging of fields as close as 150 um above structures, through the use of extremely thin external cell walls. This is crucial in allowing us to take practical advantage of the high spatial resolution, as feature sizes in near-fields are on the order of the distance from their source, and represents an order of magnitude improvement in surface-feature resolution compared to previous vapor cell experiments. We demonstrate a microwave magnetic field sensitivity of 1.4 uT/sqrt-Hz per 50x50x140 um3 voxel, at present limited by the speed of our imaging system. Since we image 120x120 voxels in parallel, a single scanned sensor would require a sensitivity of at least 12 nT/sqrt-Hz to produce images with the same sensitivity. \n \nThe spatial resolution, distance of approach, and sensitivity of our high resolution setup are sufficient for characterising 6.8 GHz microwave fields above a range of real world devices. However, frequency tunability is essential for wider applications of our imaging technique. Industry is particularly interested in techniques for imaging high frequency microwaves, above 18 GHz, where simulations become increasingly unreliable. I have shown that our technique can be extended to image microwaves of any frequency, in principle from dc to 100s of GHz, by using a large dc magnetic field to Zeeman shift the hyperfine ground state transitions to the desired frequency. I present results from a proof-of-principle setup, where we have used a 0.8 T solenoid to detect and image microwaves from 2.3 GHz to 26.4 GHz. \n

DOI
10.5451/unibas-006504997

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In this thesis, I report on the development of imaging techniques in atomic vapor cells. This is a relatively unexplored area, despite the ubiquitous use of imaging in experiments with ultracold atoms. Our main focus is in high resolution imaging of microwave near fields, for which there is currently no satisfactory established technique. We detect microwave fields through Rabi oscillations driven by the microwave on atomic hyperfine transitions. The technique can be easily modified to also image dc magnetic fields. In addition, we have developed techniques to image vapor cell processes such as atomic T1 and T2 relaxation. These provide a new window into vapor cell physics, which we have used to obtain spatially resolved information on Rb interactions with the cell walls, and to estimate the Rb relaxation probability in a collision with the cell wall. \n \nAs a first application of our imaging techniques, we imaged the dc and microwave magnetic fields inside a state-of-the-art vapor cell atomic clock. This new clock characterisation technique should lead to real improvements in clock performance, and is in the process of being adopted by the atomic clock community. \n \nWe have developed a widefield, high resolution imaging setup using a microfabricated vapor cell, which we have used to image microwave and dc magnetic vector fields. With the addition of a 480 nm laser, the setup can be configured to image microwave electric fields. Our camera-based imaging system records 2D images with a 6x6 mm2 field of view at a rate of 10 Hz. It provides up to 50 um spatial resolution, and allows imaging of fields as close as 150 um above structures, through the use of extremely thin external cell walls. This is crucial in allowing us to take practical advantage of the high spatial resolution, as feature sizes in near-fields are on the order of the distance from their source, and represents an order of magnitude improvement in surface-feature resolution compared to previous vapor cell experiments. We demonstrate a microwave magnetic field sensitivity of 1.4 uT/sqrt-Hz per 50x50x140 um3 voxel, at present limited by the speed of our imaging system. Since we image 120x120 voxels in parallel, a single scanned sensor would require a sensitivity of at least 12 nT/sqrt-Hz to produce images with the same sensitivity. \n \nThe spatial resolution, distance of approach, and sensitivity of our high resolution setup are sufficient for characterising 6.8 GHz microwave fields above a range of real world devices. However, frequency tunability is essential for wider applications of our imaging technique. Industry is particularly interested in techniques for imaging high frequency microwaves, above 18 GHz, where simulations become increasingly unreliable. I have shown that our technique can be extended to image microwaves of any frequency, in principle from dc to 100s of GHz, by using a large dc magnetic field to Zeeman shift the hyperfine ground state transitions to the desired frequency. I present results from a proof-of-principle setup, where we have used a 0.8 T solenoid to detect and image microwaves from 2.3 GHz to 26.4 GHz. \n
We report on the experimental measurement of the dc and microwave magnetic field distributions inside a recently developed compact magnetron-type microwave cavity mounted inside the physics package of a high-performance vapor-cell atomic frequency standard. Images of the microwave field distribution with sub-100-μm lateral spatial resolution are obtained by pulsed optical-microwave Rabi measurements, using the Rb atoms inside the cell as field probes and detecting with a CCD camera. Asymmetries observed in the microwave field images can be attributed to the precise practical realization of the cavity and the Rb vapor cell. Similar spatially resolved images of the dc magnetic field distribution are obtained by Ramsey-type measurements. The T2relaxation time in the Rb vapor cell is found to be position dependent and correlates with the gradient of the dc magnetic field. The presented method is highly useful for experimental in situ characterization of dc magnetic fields and resonant microwave structures, for atomic clocks or other atom-based sensors and instrumentation.
We use an atomic vapor cell as a frequency tunable microwave field detector operating at frequencies from GHz to tens of GHz. We detect microwave magnetic fields from 2.3 GHz to 26.4 GHz, and measure the amplitude of the σ+ component of an 18 GHz microwave field. Our proof-of-principle demonstration represents a four orders of magnitude extension of the frequency tunable range of atomic magnetometers from their previous dc to several MHz range. When integrated with a high-resolution microwave imaging system [Horsley et al., New J. Phys. 17, 112002 (2015)], this will allow for the complete reconstruction of the vector components of a microwave magnetic field and the relative phase between them. Potential applications include near-field characterisation of microwave circuitry and devices, and medical microwave sensing and imaging.
We demonstrate a simple technique for microwave field imaging using alkali atoms in a vapor cell. The microwave field to be measured drives Rabi oscillations on atomic hyperfine transitions, which are detected in a spatially resolved way using a laser beam and a camera. Our vapor cell geometry enables single-shot recording of two-dimensional microwave field images with 350 μm spatial resolution. Using microfabricated vapor cell arrays, a resolution of a few micrometers seems feasible. All vector components of the microwave magnetic field can be imaged. Our apparatus is simple and compact and does not require cryogenics or ultra-high vacuum.
Research of hot atomic vapor systems has a long history. Recently, much-improved technologies, such as lasers, microwaves and digital/analog control systems, have led to exciting progress in this reviving field. Due to its cryogenic-free and vacuum-free deployment potential, room-temperature and quantum-enabled sensing devices using gaseous atoms have become a popular research topic, and engineering such devices has received considerable attention. Proof-of-principle experiments have been performed demonstrating new ideas such as quantum-enhanced motion sensors, next-generation magnetometers, Rydberg enabled microwave sensors, etc. This thesis focuses on my work related to electromagnetic-field sensing using Rydberg atoms in vapor cells, where Rydberg atoms are excited and detected by electromagnetically induced transparency (EIT) spectroscopy. I first investigate the detection of strong magnetic fields (simsimsim 1~T) in the Paschen-Back regime. The diamagnetic (quadratic) response of the Rydberg levels makes the atoms sensitive to small fluctuations in field strength on a large background. By implementing an isotope-mixed cell, we demonstrate that accurate measurement, within a relative uncertainty of pm0.12pm 0.12pm0.12%. Many Rydberg-enabled radio frequency and microwave sensing applications require a capability of zeroing or intentional tuning of small DC electric fields inside the vapor cell. For this purpose, I explore an in-situ DC electric-field sensing and tuning method without using any bulk or thin film electrodes. I find that the photoelectric effect on the vapor cell walls (with invisible, atomic Rb aggregate layers covering the surfaces) can generate tuning fields up to 0.8~V/cm, with an inhomogeneity of about 2%. The spatial distribution of these fields can be directly monitored by quadratic Stark shifts of the Rydberg atoms. This work may inspire new approaches for DC-field control in miniaturized, metal-free atomic vapor-cell devices. Like many other quantum measurements on hot gaseous samples, short interaction time and other technical decoherence processes are the major factors which limit the precision and, in certain cases, the accuracy of the metrological results. In order to study these effects in the context of EIT, I performed an EIT experiment using a LambdaLambdaLambda-type quantum system consisting of the hyperfine ground states and the first excited electronic state of the Rb atoms contained in a buffer-gas-free thermal vapor cell without anti-relaxation coating. Technical line-broadening effects due to inhomogeneity of stray magnetic fields, laser frequency jitter, transverse beam intensity distribution, interaction time distribution, and atom-wall/impurity gas collisions are studied. Experimental results and numerical simulations are compared. These results provide crucial information and quantitative insights for vapor cell sensor design. The development of compact and multi-functional spectroscopy vapor cells is widely considered to be a critical engineering step towards manufacturing field-deployable sensors for real life applications. My R&D efforts towards fabrication of glass spectroscopy cells with integrated, highly-conductive silicon components are presented in the last part of my thesis. I explored various technical challenges and successfully developed a proof-of-principle prototype from scratch. The device allows the application of electric fields inside the cell for particle trapping and for tuning Rydberg transitions. Further, the highly-conductive silicon components enable microwave polarization filtering for microwave sensing applications, plasma-physics studies, etc. Preliminary experimental/technical data and simulations are presented. In summary, in my thesis I report on a comprehensive study of several spectroscopic and field sensing applications of Rydberg and ground-state atoms in vapor cells, as well as forays into novel methods to engineer vapor cells with embedded electrodes.
In this work, we demonstrate a microwave magnetic field imaging technique based on Rabi resonance with a cesium atom vapor cell. Rabi resonance signals are generated when atoms interact with a phase-modulated microwave (MW) field and are detected by a photodiode and camera. A low noise, high quantum efficiency camera is used to capture a series of frames for different phase modulation frequencies. Rabi frequencies of each spatial point in the field can be measured by scanning the frames. Thus, the strength of the MW magnetic field distribution is obtained by combing the Rabi frequencies, measured with camera pixels in the range of the probe laser beam. The simple architecture of this imaging setup holds great potential for the construction of compact/miniature MW field sensors for material testing, field imaging of MW components, and biomedical imaging.
We present a characterization technique for atomic vapor cells, combining time-domain measurements with absorption imaging to obtain spatially resolved information on decay times, atomic diffusion, and coherent dynamics. The technique is used to characterize a 5-mm-diameter, 2-mm-thick microfabricated Rb vapor cell, with N2{}_{2}2​ buffer gas, placed inside a microwave cavity. Time-domain Franzen and Ramsey measurements are used to produce high-resolution images of the population (T1{T}_{1}T1​) and coherence (T2{T}_{2}T2​) lifetimes in the cell, while Rabi measurements yield images of the ${\ensuremath{\sigma}}_{\ensuremath{-}}$, $\ensuremath{\pi}$, and ${\ensuremath{\sigma}}_{+}$ components of the applied microwave magnetic field. For a cell temperature of $90{\phantom{\rule{0.16em}{0ex}}}^{\ensuremath{\circ}}$C, the T1{T}_{1}T1​ times across the cell center are found to be a roughly uniform $265\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}$s, while the T2{T}_{2}T2​ times peak at around $350\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}$s. We observe a ``skin'' of reduced T1{T}_{1}T1​ and T2{T}_{2}T2​ times around the edge of the cell due to the depolarization of Rb after collisions with the silicon cell walls. Our observations suggest that these collisions are far from being 100% depolarizing, consistent with earlier observations made with Na and glass walls. Images of the microwave magnetic field reveal regions of optimal field homogeneity, and thus coherence. Our technique is useful for vapor cell characterization in atomic clocks, atomic sensors, and quantum information experiments.