Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Acta Optica Sinica

The gain factor and energy conversion efficiency quasi- stationary stimulated electronic Raman scattering with focused broad-band pump lasers

Ang B

Published Jan 1, 1989• 0 citations
OpenAlex

Abstract

By using Raman-Maxwell-Bloch equations, we have calculated the gain factor and energy conversion efficiency of quasi-stationary stimulated electronic Raman scattering with focused broadband pump laser. The effects of laser pump depletion and saturation of Eaman medium as well as the absorption of the medium to the pump beam are considered in the calculation. The results are agreement with the experimental results of XeCl excimer laser radiation in Ba vapour.

Related papers

High-efficiency Raman Conversion of XeCl Laser Radiation in Lead Vapour

Qihong Lou, Hongping Guo, Yunsheng Huo

Raman energy-conversion efficiency in lead vapour as high as 52% was obtained with a pumping XeCl excimer laser used in an unstable-resonator configuration. The characteristics of stimulated Raman scattering in lead vapour pumped by the XeCl laser with unstable and stable resonators were compared in detail. Relaxation oscillations of the Raman-shifted pulse were observed, and these are related to the effect of ground-state depletion of atoms in the lead vapour.

Journal of Modern Optics•Feb 1, 1989•2 citations

Investigation of electronic stimulated Raman scattering of excimer laser radiation by metal atoms

V S Verkhovskiĭ, Vladimir M. Klimkin, В. Е. Прокопьев +3 more

An experimental investigation was made of stimulated Raman scattering (STRS) of excimer laser radiation in barium, thulium, and europium vapors. The energy of XeF* laser radiation ( λ = 351 nm) converted to the yellow range (585 nm) in barium vapor was 6 mJ and the conversion efficiency was ∼39%. The spectral composition of the converted radiation is governed by the STRS, by four-wave parametric processes, and also by lasing due to the natural barium transition. Selection of the pump frequencies is required to concentrate the converted radiation at a single frequency and to reduce its divergence. Stimulated Raman scattering of XeCl* laser radiation ( λ = 308 nm) was achieved in thulium vapor at λ = 422 nm. In europium vapor in quasiresonance with the 6 s 2 8 S 0 1/2 –5 d 2 10 P 0 11/2 forbidden transition, stimulated emission was obtained due to the natural 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 11/2 and 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 3/2 transitions.

Soviet Journal of Quantum Electronics•Nov 30, 1982•9 citations

Effects of ground-state depletion of atoms in stimulated Raman scattering of metal vapors

Yunsheng Huo, Qihong Lou, Zian Ding +1 more

The effects of ground-state depletion of atoms on the characteristics of stimulated Raman scattering in metal vapors are studied by simultaneously solving the rate equation of the atomic energy levels related in the Raman scattering, and the equations describing the energy conversion from the focused pump-laser pulses to the Raman down-converted pulses. The ground states of metal atoms are depleted most strongly in the regions near the focal spots of the pump beams because of the higher intensities of light and smaller available medium volume in those regions. This will result in the unsymmetrical shapes of the Raman-shifted pulses for the front and rear edges, and will reduce the energy-conversion efficiency.

Acta Physica Sinica•Jan 1, 1989•0 citations

Effects of ground-state depletion of atoms in stimulated Raman scattering of metal vapors

Yunsheng Huo, Qihong Lou, Zian Ding +1 more

The effects of ground state depletion of atoms on the characteristics of stimulated Raman scattering in metal vapors are studied by simultaniously solving the rate-equation of the atom energy levels related in the Raman scattering, and the equations describing the energy-conversion from the focused pump laser pulses to the Raman down-converted pulses. The ground state of metal atoms are depleted most strongly in the regions near the focal spots of the pump beams because of the higher intensities of light and smaller available medium volume in thosa regions. This will result in the unsymmetrical shapes of the Raman-shifted pulses for the front and rear edges, and will reduce the energy-conversion efficiency.

Acta Optica Sinica•Jan 1, 1987•0 citations

Stimulated Raman scattering subject to nonlinear effects

Yu. V. Petrushevich, Andrei N Starostin

A model is developed for the description of stimulated Raman scattering. This model allows for changes in the level populations due to radiative transitions and it can be used also for an arbitrary detuning of the pump radiation from the center of a line of an atom in the active medium. A study is made of the conversion of wide-band laser radiation into a Stokes signal. It is shown that this conversion is quite efficient and the Stokes signal gain corresponds to coherent scattering. This result is related to the matching of the phases of the pump and Stokes signals. Numerical investigations carried out using this model under the experimental conditions described elsewhere give results in agreement with the experimental data.

Soviet Journal of Quantum Electronics•Feb 28, 1991•0 citations

Theory of stimulated Raman scattering with broad-band lasers

Michael G. Raymer, Jan Mostowski, John L. Carlsten

The authors have extended the theory of stimulated Raman scattering to include the effects of laser bandwidths, in both the transient and steady-state regimes. The case of two interacting laser beams, a pump laser and a probe (Stokes) laser, is treated. Using the phase-diffusion model for laser bandwidth, the authors demonstrate that in the absence of dispersion, the forward Raman gain is essentially independent of the laser bandwidths in the high-gain limit, while in the low-gain limit the gain coefficient is inversely proportional to the sum of the bandwidths. It is further shown that when the pump-laser bandwidth is much larger than the linewidth of the Raman medium, the stimulated Stokes output assumes the same spectrum as the pump laser in the high-gain limit. A possible interpretation of these results is discussed assuming a "phase-locking" of the Stokes phase to the fluctuations in the pump-laser phase, due to the nonlinear interaction of the two beams through the Raman medium.

Physical Review A•Jun 1, 1979•136 citations
By using Raman-Maxwell-Bloch equations, we have calculated the gain factor and energy conversion efficiency of quasi-stationary stimulated electronic Raman scattering with focused broadband pump laser. The effects of laser pump depletion and saturation of Eaman medium as well as the absorption of the medium to the pump beam are considered in the calculation. The results are agreement with the experimental results of XeCl excimer laser radiation in Ba vapour.
An experimental investigation was made of stimulated Raman scattering (STRS) of excimer laser radiation in barium, thulium, and europium vapors. The energy of XeF* laser radiation ( λ = 351 nm) converted to the yellow range (585 nm) in barium vapor was 6 mJ and the conversion efficiency was ∼39%. The spectral composition of the converted radiation is governed by the STRS, by four-wave parametric processes, and also by lasing due to the natural barium transition. Selection of the pump frequencies is required to concentrate the converted radiation at a single frequency and to reduce its divergence. Stimulated Raman scattering of XeCl* laser radiation ( λ = 308 nm) was achieved in thulium vapor at λ = 422 nm. In europium vapor in quasiresonance with the 6 s 2 8 S 0 1/2 –5 d 2 10 P 0 11/2 forbidden transition, stimulated emission was obtained due to the natural 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 11/2 and 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 3/2 transitions.
The effects of ground-state depletion of atoms on the characteristics of stimulated Raman scattering in metal vapors are studied by simultaneously solving the rate equation of the atomic energy levels related in the Raman scattering, and the equations describing the energy conversion from the focused pump-laser pulses to the Raman down-converted pulses. The ground states of metal atoms are depleted most strongly in the regions near the focal spots of the pump beams because of the higher intensities of light and smaller available medium volume in those regions. This will result in the unsymmetrical shapes of the Raman-shifted pulses for the front and rear edges, and will reduce the energy-conversion efficiency.
The effects of ground state depletion of atoms on the characteristics of stimulated Raman scattering in metal vapors are studied by simultaniously solving the rate-equation of the atom energy levels related in the Raman scattering, and the equations describing the energy-conversion from the focused pump laser pulses to the Raman down-converted pulses. The ground state of metal atoms are depleted most strongly in the regions near the focal spots of the pump beams because of the higher intensities of light and smaller available medium volume in thosa regions. This will result in the unsymmetrical shapes of the Raman-shifted pulses for the front and rear edges, and will reduce the energy-conversion efficiency.
A model is developed for the description of stimulated Raman scattering. This model allows for changes in the level populations due to radiative transitions and it can be used also for an arbitrary detuning of the pump radiation from the center of a line of an atom in the active medium. A study is made of the conversion of wide-band laser radiation into a Stokes signal. It is shown that this conversion is quite efficient and the Stokes signal gain corresponds to coherent scattering. This result is related to the matching of the phases of the pump and Stokes signals. Numerical investigations carried out using this model under the experimental conditions described elsewhere give results in agreement with the experimental data.
The authors have extended the theory of stimulated Raman scattering to include the effects of laser bandwidths, in both the transient and steady-state regimes. The case of two interacting laser beams, a pump laser and a probe (Stokes) laser, is treated. Using the phase-diffusion model for laser bandwidth, the authors demonstrate that in the absence of dispersion, the forward Raman gain is essentially independent of the laser bandwidths in the high-gain limit, while in the low-gain limit the gain coefficient is inversely proportional to the sum of the bandwidths. It is further shown that when the pump-laser bandwidth is much larger than the linewidth of the Raman medium, the stimulated Stokes output assumes the same spectrum as the pump laser in the high-gain limit. A possible interpretation of these results is discussed assuming a "phase-locking" of the Stokes phase to the fluctuations in the pump-laser phase, due to the nonlinear interaction of the two beams through the Raman medium.