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Acta Physica Sinica

ENERGY-LEVEL DIFFERENCE AND LASER ABSOLUTE FREQUENCY MEASUREMENT BY POLARIZATION BEATS SPECTROSCOPY WITH PHASE-CONJUGATION GEOMETRY

ZHANG YAN-PENG, Gan Chen-Li, Zhu Jing-Ping, TANG TIAN-TONG, Panming Fu, (1)西安交通大学光电子系,西安 710049; (2)中国科学院物理研究所,北京 100080

Published Jan 1, 1999• 7 citations
Publisher

Abstract

We have studied the polarization beats spectroscopy with phase-conjugation geometry in a cascade three-level system.It was found that the accuracy for the energy-level difference measurement is determined by the homogeneous linewidths of the optical trans
DOI
10.7498/aps.48.1667

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Effects of fourth-order coherence on ultrafast modulation spectroscopy

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The effect of fourth-order coherence on ultrafast modulation spectroscopy with phase-conjugation geometry (PCUMS) in a cascade three-level system is investigated using chaotic and phase-diffusion models. It has been found that the temporal behavior of the beat signal depends on the stochastic properties of the lasers and the transverse relaxation rate of the transitions, and the modulation terms of the beat signal depend on the second-order coherence function, which is determined by the laser line shape. Since different stochastic models of the laser field affect only the fourth-order coherence function, they have little influence on the general temporal modulation behavior of the beat signal. The different roles of the phase fluctuation and amplitude fluctuation can be investigated in the time domain. The cases where the pump beams have either a narrow or broad band linewidth are considered and it has been found that for both cases a Doppler-free precision in the measurement of the energy-level difference between two states can be achieved. The difference between the PCUMS and the DeBeer, UMS [D. DeBeer et al., Phys. Rev. Lett. 56, 1128 (1986)] is discussed as well from a physical viewpoint.

Physical Review A•Jan 13, 2000•25 citations
We have studied theoretically a beat effect in a four-level system due to fifth-order optical polarization, and considered the cases that the pump beams have either narrowband or broadband linewidth. We have found that the accuracy for the energy-level splitting meaurement is determined by the homogeneous linewidths of the optical transitions. That is to say, this technique can achieve Doppler-free precision in the measurement of the eaergy level splitting between two excited states which are dipolar forbidden from the ground state.
Based on the second-order coherence function, we have studied a phase-conjugate ultrafast modulation spectroscopy due to the interference between the fifth- and fifth-order optical polarizations in cascade three-level Doppler-broadened system. It is found that the temporal behaviour of the beat signal depends on the stochastic properties of the lasers and the transverse relaxation rate of the transition. The beat signal depends on the second-order coherence function, which is determined by the laser line shape. Since different stochastic models of the laser field only affect higher than second-order coherence functions, they have little influence on the general temporal modulation behaviour of the beat signal. The cases that pump beams have either narrow band or broadband linewidth are considered and it has been found that for both cases the overall accuracy for the energy-level difference measurement is determined by the homogeneous linewidths of the optical transitions. Finally, the spatial modulation behaviour of the beat signal has also been discussed.
The effect of fourth-order coherence on ultrafast modulation spectroscopy with phase-conjugation geometry (PCUMS) in a cascade three-level system is investigated using chaotic and phase-diffusion models. It has been found that the temporal behavior of the beat signal depends on the stochastic properties of the lasers and the transverse relaxation rate of the transitions, and the modulation terms of the beat signal depend on the second-order coherence function, which is determined by the laser line shape. Since different stochastic models of the laser field affect only the fourth-order coherence function, they have little influence on the general temporal modulation behavior of the beat signal. The different roles of the phase fluctuation and amplitude fluctuation can be investigated in the time domain. The cases where the pump beams have either a narrow or broad band linewidth are considered and it has been found that for both cases a Doppler-free precision in the measurement of the energy-level difference between two states can be achieved. The difference between the PCUMS and the DeBeer, UMS [D. DeBeer et al., Phys. Rev. Lett. 56, 1128 (1986)] is discussed as well from a physical viewpoint.