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Chinese Journal of Quantum Electronics

Quantum interference effects in molecular and atom-molecular systems

Wang Zhu-geng

Published Jan 1, 2004• 0 citations
OpenAlex

Abstract

Recent investigations on quantum interference effects were introduced, including line-shape variation, spontaneous emission enhancement or cancellation, constructive interference and electromagnetically induced transparency in molecular and atomic-molecular mixed systems in our laboratory. It is instructive to the researches about quantum interference and control in molecular, condensed matter and material systems.

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Recent investigations on quantum interference effects were introduced, including line-shape variation, spontaneous emission enhancement or cancellation, constructive interference and electromagnetically induced transparency in molecular and atomic-molecular mixed systems in our laboratory. It is instructive to the researches about quantum interference and control in molecular, condensed matter and material systems.
In this review the author discusses the major effects resulting from the modification of spontaneous emission by quantum interference. He begins in Section II by presenting elementary concepts and definitions of the first- and second-order correlation functions, which are frequently used in the analysis of the interference phenomena. Section III describes the master equation approach used for analyzing quantum interference effects in atomic and molecular systems. In Sections IV and V the author reviews the fundamental quentum interference effects in spontaneous emission and in coherently driven systems. He discusses different schemes for suppression of spontaneous emission and population trapping and gives an alternative explanation of these effects in the dressed-atom picture. Section VI deals with the problem of amplification on dark transitions, which are important for information processing without spontaneous emission. The effect of quantum interference on photon correlations is discussed in Section VII. Multilevel systems composed of two transitions with parallel dipole moments and methods for generating two transitions with nonorthogonal dipole moments are briefly discussed in Section VIII. The final section (Section IX) deals with the experimental demonstration of constructive and desctructive interference effects in a driven molecular system.
Coherent interactions of laser fields with resonant atomic and molecular transitions significantly modify optical characteristics of the medium via quantum interference between transition amplitudes. This interference can result in reduction or enhancement of the laser absorption, decrease of the group velocity of the laser pulse etc. The origin of all these processes is electromagnetically induced transparency. This effect is intensively investigated in the connection with its multiple applications: lasing without inversion, group velocity control, quantum optical storage and quantum computing, effective nonlinear interactions of low field intensities, high-precision measurements, spectroscopy and metrology, plasma diagnostics, atomic clock etc.
The quantum interference between two spontaneous emission transitions, which are orthogonal, in a three-level system, can be greatly enhanced by using left-handed materials due to the focusing and phase compensation effects. The influence of the dispersion and dissipation of the materials on the quantum interference enhancement is investigated, and the enhancement of quantum interference is still significant. The quantum interference enhancement will result in a large quenching of the spontaneous emission, even if the distance between the materials and systems is larger than 10 wavelengths.
We describe the spontaneous emission properties of an M-type five-level atom embedded in a photonic crystal (PC), which is coherently driven by two external laser fields. It leads to two types of quantum interference: reservoir-induced interference and laser-induced interference. Considering different detunings of atomic transition frequencies from band edges, we reveal some interesting phenomena such as spectral-line enhancement, spectral-line suppression, spectral-line narrowing, reservoir-induced cancellation of spontaneous emission and the appearance of dark lines, which originate from the quantum interference effects and the control of external laser fields. These investigations suggest possible applications in quantum optics, optical communications and in the fabrication of novel optoelectronic devices.
Abstract Quantum interference plays a central role in the realm of quantum particles, revealing their wave‐like nature and probabilistic behavior. It relies on the concept of superposition, where the probability amplitudes of different processes that contribute to the given phenomenon interfere with each other. When combined, their phases can interfere either constructively or destructively. Quantum interference manifests in three distinct forms: optical interference, arising from the interaction of light waves and forming the basis for technologies such as lasers and optical filters; interference via atoms, which involves manipulating atomic states to control light–matter interactions and enables techniques like Stimulated Raman Adiabatic Passage and Electromagnetically Induced Transparency in quantum information processing; and interference of atoms with themselves, in which the matter waves of single atoms interfere with each other, as employed in precision measurements such as atom interferometry–a crucial tool for applications in quantum mechanics and precision navigation. These diverse forms of quantum interference have profound implications for numerous scientific disciplines, demonstrating that interference can involve particles beyond just photons.