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Quantum optics experiments in a microstructured ion trap

Ulrich Poschinger

Published Jan 1, 2010• 4 citations
Publisher

Abstract

This dissertation describes a prototype experiment aiming at the realization of scalable quantum information. The essential feature is the usage of a novel microstructured ion trap derived from the Paul trap. It allows for storing and manipulating a large number of ions, as compared to conventional linear Paul traps. This thesis describes how the way is paved towards the realization of quantum information experiments in this ion trap. An analysis of the electrostatic properties of the ion trap is presented, which is laying the foundation for understanding the limits of confinement stability and effects beyond standard Paul trap behavior. The focus of this work lies on the realization and characterization of single and dual qubit operations, which are achieved by means of (semiclassical) atom-light interaction. In our experiment, the qubit is implemented in the Zeeman sublevels of the ion’s ground state, i.e. in the spin of the bright electron of a 40Ca+ ion. The main body of this thesis then describes the realization of the necessary steps of preparation, manipulation and readout of this qubit. The preparation includes optical pumping and cooling close to the motional quantum ground state by means of sideband cooling. Several possible techniques for these steps are tested and analyzed. Coherent manipulations are carried out by means of stimulated Raman transitions. Here, a strong emphasis is put on the characterization of the various decoherence mechanisms, which are dominated by the motional excitation of the ion due to thermalization of the ion with the trap electrodes, and by imperfections in the ion-laser interactions. As by-product of the latter investigation, a new measurement scheme for the experimental determination of atomic dipole matrix elements is presented.

DOI
10.18725/oparu-1898

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arXiv:quant-ph/0003096•Journal of Modern Optics•Nov 1, 2000•25 citations
This dissertation describes a prototype experiment aiming at the realization of scalable quantum information. The essential feature is the usage of a novel microstructured ion trap derived from the Paul trap. It allows for storing and manipulating a large number of ions, as compared to conventional linear Paul traps. This thesis describes how the way is paved towards the realization of quantum information experiments in this ion trap. An analysis of the electrostatic properties of the ion trap is presented, which is laying the foundation for understanding the limits of confinement stability and effects beyond standard Paul trap behavior. The focus of this work lies on the realization and characterization of single and dual qubit operations, which are achieved by means of (semiclassical) atom-light interaction. In our experiment, the qubit is implemented in the Zeeman sublevels of the ion’s ground state, i.e. in the spin of the bright electron of a 40Ca+ ion. The main body of this thesis then describes the realization of the necessary steps of preparation, manipulation and readout of this qubit. The preparation includes optical pumping and cooling close to the motional quantum ground state by means of sideband cooling. Several possible techniques for these steps are tested and analyzed. Coherent manipulations are carried out by means of stimulated Raman transitions. Here, a strong emphasis is put on the characterization of the various decoherence mechanisms, which are dominated by the motional excitation of the ion due to thermalization of the ion with the trap electrodes, and by imperfections in the ion-laser interactions. As by-product of the latter investigation, a new measurement scheme for the experimental determination of atomic dipole matrix elements is presented.
Scalability and the implementation of fault tolerant quantum gates are the two main challenges which must be overcome in order to unlock the vast potential of quantum computing. This thesis describes work with calcium ions trapped in both microscopic and macroscopic linear Paul traps addressing both of these issues. We describe the assembly of a microstructured multi-zone ion trap which forms part of our group's contribution to the European "Microtrap" collaboration. We report the successful trapping of ions and characterization of the trap as well as a measurement of the heating rate. In miniaturized trap structures such as this one, background scattered light from the cooling beam causes difficulties. We introduce and demonstrate experimentally two techniques to overcome this problem. The first achieves background-free detection of ions using different repumping methods to enable the filtering out of the excitation wavelength. The second makes possible background-free readout of trapped ion qubits by separating in time the excitation and detection steps The second half of the thesis describes our experimental efforts towards implementing a two-qubit entangling gate with a mixed-species crystal. We describe the setup and characterization of a new macroscopic trap including the trapping and coherent manipulation of the internal states of both 40Ca+ and 43Ca+ ions. We accomplish the simultaneous independent readout of two qubits implemented in a 40Ca+ - 43Ca+ ion pair. We also present the setup and characterization of two injection-locked frequency-doubled Raman lasers and demonstrate coherent manipulation as well as a measurement of the off-resonant photon scattering error they introduce. Finally, we use them to achieve sideband cooling to the motional ground state of a mixed species ion crystal.
Single ions in Paul traps are investigated for quantum information processing. Superpositions of the S1/2 and the D5/2 states are used to implement a qubit. The ions are optically cooled and fluorescence light at 397 nm on the S1/2-P1/2 transition is monitored for a state measurement by the “electron shelving” technique. The S1/2-D5/2 quadrupole transition at 729 nm is excited for sideband cooling and for quantum state preparation and manipulation. Individual ions in a linear string are addressed by a tightly focused 729 nm laser beam. A single Ca+ ion has been cooled in the spherical Paul trap to the ground state of vibration with up to 99.9% probability. Cooling is achieved in all three dimensions simultaneously as well as ground state cooling of two ions. Starting from a Fock state |n=0> coherent quantum state manipulation on the S1/2-D5/2 transition is achieved. The data show that decoherence is negligible on the time scale of a few oscillations, i.e. during the time required for a quantum gate operation. The measured several decoherence time of a few ms is attributed to residual laser and magnetic field fluctuations. Heating of the motional degrees of freedom has been measured directly and appears at a rate of 1 phonon per 190 ms (70 ms) at the secular frequencies ωaxial (ωradial). A novel type of ground state laser cooling of a single trapped ion is achieved using a technique which tailors the absorption profile for the cooling laser by exploiting electromagnetically induced transparency in the Zeeman structure of the S1/2–P1/2 dipole transition. This new method is robust, easy to implement and proves particularly useful for cooling several motional degrees of freedom simultaneously, which is of great practical importance for the implementation of quantum logic schemes with trapped ions.
Summary form only given. Single ions in Paul traps are investigated for quantum information processing. Superpositions of the S/sub 1/2/ and the D/sub 5/2/ states are used to implement a qubit. Single /sup 40/Ca/sup +/ ions are either held in a spherical Paul trap or alternatively, in a linear Paul trap. The ions are optically cooled and fluorescence light at 397 nm on the S/sub 1/2/-P/sub 1/2/ transition is monitored for a state measurement by the electron shelving technique. The S/sub 1/2/-D/sub 5/2/ quadrupole transition at 729 nm is excited for sideband cooling and for quantum state preparation. Individual ions in a linear string are addressed by a tightly focused 729 nm laser beam. In the spherical Paul trap (4.5 MHz trap frequency) a single Ca/sup +/ ion has been cooled to the ground state of vibration with a probability of up to 99.9%. Starting from this Fock state |n=0> coherent quantum state manipulation on the S/sub 1/2/-D/sub 5/2/ transition is achieved.
Trapped ions are currently one of the most promising architectures for realising the quantum information processor. The long lived internal states are ideal for representing qubit states and, through controlled interactions with electromagnetic radiation, ions can be manipulated to execute coherent logic operations. In this thesis an experiment capable of trapping Yb+ ions, including 171Yb+, is presented. Since ion energy can limit the coherence of qubit manipulations, characterisation of an ion trap heating rate is vital. Using a trapped 174Yb+ ion a heating rate consistent with previous measurements of other ion species in similar ion traps is obtained. This result shows abnormal heating of Yb+ does not occur, further solidifying the suitability of this species for quantum information processing. Efficient creation, and cooling of trapped ions requires exact wavelengths for the ionising, cooling and repump transitions. A simple technique to measure the 1S0 ? 1P1 transition wavelengths, required for isotope selective photoionisation of neutral Yb, is developed. Using the technique new wavelengths, accurate to 60 MHz, are obtained and differ from previously published results by 660 MHz. Through a simple modification the technique can also predict Doppler shifted transition frequencies, which may be required in non-perpendicular atom-laser interactions. Using trapped ions, the 2S1=2 ? 2P1/2 Doppler cooling and 2D3/2 ? 2D[3/2]1/2 repump transitions are also measured to a greater accuracy than previously reported. Many experiments require wavelengths which can only be obtained using complex expensive laser systems. To remedy this a simple cost effective laser is developed to enable laser diodes to be operated at sub zero temperatures, extending the range of obtainable wavelengths. Additional diode modulation capabilities allow for the manipulation of atoms and ions with hyperfine structures. The laser is shown to be suitable for manipulating Yb+ ions by cooling a diode from 372 nm to 369 nm and simultaneously generating 2.1 GHz frequency sidebands. Coherent manipulation such as arbitrary qubit rotations, motional coupling and ground state cooling, are required for trapped ion quantum computing. Two photon stimulated Raman transitions are identified as a suitable technique to implement all of these requirements and an investigation into implementing this technique with 171Yb+ is conducted. The possibility of exciting a Raman transition via either a dipole or quadrupole transitions in 171Yb+ is analysed, with dipole transitions preferred because quadrupole transitions are found to be too demanding experimentally. An inexpensive setup, utilising a dipole transition, is designed and tested. Although currently limited the setup shows potential to be an inexpensive, high fidelity method of exciting a Raman transition.
Laser-cooled trapped ions are one of the main systems used in experiments in the fields of quantum optics and quantum information. There are two commonly-used types of ion trap, the radiofrequency trap and the Penning trap. In general, the RF trap has been more widely used in quantum information experiments, meaning that the set of experimental tools for conducting these types of experiments in a Penning trap is currently less complete. The aim of the work presented in this thesis is to increase this array of tools. Our experiment uses 40Ca+ ions in a Penning trap alongside lasers. Spectroscopy has been performed on single Doppler cooled ions, and on ions that have been prepared close to their ground state of motion using a multiple-stage sideband cooling technique resulting in an average phonon occupation number of $\nzbar = 0.029\pm 0.011$ from an initial $\nzbar \approx 24$. This corresponds to a quantum ground state population of 97%97\%97%, which is close to the sideband cooling limit in our system. An axial heating rate measurement of $\dot{\bar{n}}_z=\SI{0.56\pm0.52}{\per\second}$ has also been obtained, which is the lowest recorded to date, due in part to the large dimensions of our trap. Additionally improved control of the Penning trap radial motion has been demonstrated and the average phonon occupation number of the modified cyclotron motion has been reduced from $\ncbar\approx150$ after Doppler cooling to $\ncbar=0.6$ after sideband cooling. Some preliminary single-ion coherent operations have also been performed. In the future we hope that this system of ground state cooled ions in a Penning trap can be used to generate highly-entangled states in two or more ions, with a view to performing simple quantum error-correcting codes and eventually an analogue quantum simulation of spin systems.
We investigate single ions of 40Ca+ in Paul traps for quantum information processing. Superpositions of the S½ electronic ground state and the metastable D5/2; state are used to implement a qubit. Laser light on the S½ ↔ D5/2 transition is used for the manipulation of the ion's quantum state. We apply sideband cooling to the ion and reach the ground state of vibration with up to 99.9% probability. Starting from this Fock state (n = 0), we demonstrate coherent quantum state manipulation. A large number of Rabi oscillations and a ms-coherence time is observed. Motional heating is measured to be as low as one vibrational quantum in 190ms. We also report on ground state cooling of two ions.