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Acta Physica Sinica

TUNABLE IR STIMULATED RADIATION GENERATED BY TWO-STEP HYB1RD EXCITING IN Na2-Na SYSTEM

TANG XIAO-LING, Zugeng Wang, QIN LI-JUAN, Zheng Yishan, (1)华东师范大学物理系; (2)陕西师范大学物理系

Published Jan 1, 1988• 0 citations
Publisher

Abstract

We report the generation of turnable IR stimulated emission covering 3.39-3.46 μm, by using a new exciting mechanism called "two-step hybird exciting" in sodium molecular-atomic system. We analyse and discuss carefully this IR emission. The computed relative intensity of the IR emission varies with the pumping deturning. The computational results matched well with experimental data.

DOI
10.7498/aps.37.1227

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Acta Optica Sinica•Jan 1, 1986•0 citations
We report the generation of turnable IR stimulated emission covering 3.39-3.46 μm, by using a new exciting mechanism called "two-step hybird exciting" in sodium molecular-atomic system. We analyse and discuss carefully this IR emission. The computed relative intensity of the IR emission varies with the pumping deturning. The computational results matched well with experimental data.
STIMULATED EMISSION BASED ON TWO-STEP HYBRID RESONANCE A1Σu+A^{1}\Sigma_{u}^{+}A1Σu+​ OR B1ΠuB^{1}\Pi_{u}B1Πu​ STATE OF Na.∗Na.^{*}Na.∗
The first step of the hybrid excitation in the experiment was achieved by using a pulse broadband ($\\sim$200 {\\AA}) dye laser beam through a heat pipe oven. But the total covered pumping wavelength region from 4600 {\\AA} to 6800 {\\AA} the populated upper electronic state in Na2Na_{2}Na2​ should be either AprimeSigmauA^{\\prime}\\Sigma_{u}AprimeSigmau​ or BprimePiuB^{\\prime}\\Pi_{u}BprimePiu​ state. The excited sodium dimers Na2astNa_{2}^{\\ast}Na2ast​ transfered their energy to sodium atoms Na by near resonace collisions and the Na then would populate up the 3P level from ground state 3s. The Na were consequentely pumped up to 4D, 5D, 5S or 6S level from 3P by using a narrowband dye laser pumped by the same N2N_{2}N2​ laser. The infrared stimulated radiation corresponding to the transitions of 4D-4P(2.34 mu\\mumum). 5D-4P(5.02mu\\mumum), 5S-4P(3.42 mu\\mumum) and 6S-5P(7.52 mu\\mumum) with cascade stimulated emission from 4P to 4S (2.20 mu\\mumum) and from 5P to 5S (5.43 mu\\mumum) were then obtained, Furthermore the dependence of the output energy on the pumping wavelengthes was measured and discussed.
For the first time by means of two-photon hybrid excitation in the Na2-Na system, which is distinguished from the usual two-photon excitation in atomic vapor, tunable UV coherent radiation (between 337.6 and 339.1 nm and between 358.0 and 359.6 nm) and tunable infrared stimulated radiation (3.38-3.46 µm) were generated. By optically pumping with a pulsed dye laser scanning from 614.5 to 617.4 nm for sodium vapor in a heat-pipe oven, Na2 was excited by the first photon absorption from the X ′ Σ g + to the A ′ Σ u + state. The energy was transferred to Na by Na2*-Na collision to populate the levels 3p1/2,3/2 in Na, which was followed by another photon excitation from the same beam up to near the 5S level, resulting in SERS (3P1/2-4P and 3P3/2-4P) and OPSE(5S → 4P and 4P → 4S) radiation. Assuming the detunings of pumping frequency ω1, from ω(5S,3P3/2) and ω(5s,3p1/2) to be Δ1 and Δ2, respectively, the three UV coherent radiation components were supposed to be generated by the following mixing processes: ωUV = 2ω1 − ω(5S − 4P); ω U V ′ = 2 ω 1 − [ ω ( 5 S → 4 P ) + Δ 1 ] ; ω U V ′ ′ = 2 ω 1 − [ ω ( 5 S → 4 P ) + Δ 2 ] , and also ω U V ′ ′ ′ = 2 ω 1 − ω ( 4 P → 4 S ) . The SERS and the UV signals were tuned as the pumping wavelength was tuned. The measured wavelengths agreed well with the calculated values.