A nondegenerate two-photon laser in a cascade three-level atomic system is studied. The difference between the laser and that derived from an effective Hamiltonian is discussed. Photon number distributions about field 1 are presented. The effects of field 2 on field 1 are studied in detail. Field 2 can play a role of gain enhancement or gain reduction for field 1. This is due to two actions of field 2: reducing the population of the intermediate level and changing the detuning really acting upon field 1, which is caused by the ac Stark shift.
The quantum theory of the three-energy-level two-mode laser in which all the levels are being pumped is investigated and the master equation of the laser operation is obtained. It contains two variables,
n1, the photon number of the first mode, and
n2, the photon number of the second mode. There appear four terms in the master equation which represent two-photon processes between the two modes, the absorption of a photon from one mode, and emission of a photon to the other. They are absent in the single-mode case and in the two-mode case with pumping only to the upper level. The master equation can be represented by a diagram of probability in two dimensions which can be extended to infinity, and each arrow of it represents a term on the right-hand side of the master equation. By summing each variable (
n1 or
n2) of the master equation, two equations can be obtained. Each equation contains only one variable, and can be expressed by a diagram of probability flow in one dimension. By considering the correspondence between macroscopic equilibrium and microscopic detailed balance the equations of motion in the steady state are obtained. By introducing a parameter
H, the equation of motion is simplified and a formal solution can be deduced which is dependent on
H. It appears that the parameter
H cannot be fully determined, but some properties of it can be deduced which prove that the introduction of
H is reasonable. The operation characteristics of the laser under different conditions are discussed on the basis of the formal solution: among them are the threshold condition, the condition for one-mode operation, and the change of the photon-statistical distribution. We especially discuss the laser output power curves under two-mode operation above threshold. The curve of one mode, which oscillates first, shows a bending-down phenomenon as the excitation increases when the other mode goes beyond its threshold as demonstrated experimentally by Otsuka. This phenomenon is explained qualitatively and is attributed to the two-photon processes between the two modes.
A quantum theory of a two-photon laser is developed by making use of the antinormal-ordering Q function. Starting from the microscopic atom-field interaction Hamiltonian for cascade three-level atoms and including saturable absorbers, we first present a master equation for the field-density operator, and then transform the master equation into a Fokker-Planck equation for the Q function. The Q-function approach enables us to study the two-photon laser analytically, obtaining simple expressions for nonlinear gain, mean photon number, frequency pulling, natural linewidth, and photon-number variance in a unified method. We find that the field in a two-photon laser will build up from a vacuum without triggering if its linear gain is larger than the cavity loss. Also hysteresis can occur in the two-photon laser even without triggering. With an overall two-photon resonance, the normalized photon-number variance approaches a common value 11/8 well above ``threshold,'' independent of the one-photon detuning. We compare these results with previous results obtained from an effective interaction Hamiltonian. We find that the domain of validity of the effective Hamiltonian for the photon-number variance is much smaller than that for the mean photon number. Well above ``threshold'' the effective Hamiltonian overestimates both the natural linewidth and the photon-number variance.
The photon statistic of two-photon processes is treated for the general case of two-level systems. After generalizing the generating-function method, we derived the generating function with parameter r (atomic population ratio), its partial differential equation, and equations of factoril moments as well as equations of correlation functions. Analytical solutions were obtained for various values of r. Curves of n and g(2) versus τ and r were deduced for three kinds of initial fields. Both the effect of r on photon antibunching and characteristics photon statistics for two-photon amplifiers are discussed. The photon superbunching is proposed as one of the criteria for two-photon amplification.