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Genuine multipartite entanglement in superconducting phases of doped quantum spin ladders

Sudipto Singha Roy, Himadri Shekhar Dhar, Debraj Rakshit, Aditi Sen De, Ujjwal Sen

Published Apr 22, 2016• 0 citations
OpenAlex

Abstract

We investigate the trends of genuine multipartite entanglement of high-temperature superconducting states, usually described by doping the Mott insulator. We begin by analyzing the ground states of a Hubbard model with large onsite interactions obtained by exact diagonalization in regimes where the superconducting phase is observed for relatively high doping. The ground states are observed to be genuine multipartite entangled, with the maximum value achieved close to the superconducting phase boundary. Subsequently, for finite hole doping, the short-range resonating valence bond (RVB) state is considered to be the ground state of the Hubbard model. We prove that doped RVB ladder states are always genuine multipartite entangled. We then formulate an analytical recursion method for the wave function, which allows us to efficiently estimate the entanglement as well as other physical quantities in large doped RVB ladders. The maximum genuine multipartite entanglement in these RVB states is observed at doping corresponding to the superconducting phase of the Hubbard model.

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We investigate the trends of genuine multipartite entanglement of high-temperature superconducting states, usually described by doping the Mott insulator. We begin by analyzing the ground states of a Hubbard model with large onsite interactions obtained by exact diagonalization in regimes where the superconducting phase is observed for relatively high doping. The ground states are observed to be genuine multipartite entangled, with the maximum value achieved close to the superconducting phase boundary. Subsequently, for finite hole doping, the short-range resonating valence bond (RVB) state is considered to be the ground state of the Hubbard model. We prove that doped RVB ladder states are always genuine multipartite entangled. We then formulate an analytical recursion method for the wave function, which allows us to efficiently estimate the entanglement as well as other physical quantities in large doped RVB ladders. The maximum genuine multipartite entanglement in these RVB states is observed at doping corresponding to the superconducting phase of the Hubbard model.
We formulate an analytical recursive method to generate the wave function of doped short-range resonating valence bond (RVB) states as a tool to efficiently estimate multisite entanglement as well as other physical quantities in doped quantum spin ladders. We prove that doped RVB ladder states are always genuine multipartite entangled. Importantly, our results show that within specific doping concentration and model parameter regimes, the doped RVB state essentially characterizes the trends of genuine multiparty entanglement in the exact ground states of the Hubbard model with large on-site interactions, in the limit that yields the $t\text{\ensuremath{-}}J$ Hamiltonian.
We propose a class of ground states for doped Mott insulators in the electron second quantization representation. They are obtained from a bosonic resonating valence bond (RVB) theory of the $t\text{\penalty1000-\hskip0pt}J$ model. At half filling, the ground state describes spin correlations of the S=1∕2S=1∕2S=1∕2 Heisenberg model very accurately. Its spin degrees of freedom are characterized by RVB pairing of spins, the size of which decreases continuously as holes are doped into the system. Charge degrees of freedom emerge upon doping and are described by twisted holes in the RVB background. We show that the twisted holes exhibit an off diagonal long range order (ODLRO) in the pseudogap ground state, which has a finite pairing amplitude, but is short of phase coherence. Unpaired spins in such a pseudogap ground state behave as free vortices, preventing superconducting phase coherence. The existence of nodal quasiparticles is also ensured by such a hidden ODLRO in the ground state, which is non-Fermi liquidlike in the absence of superconducting phase coherence. Two distinct types of spin excitations can also be constructed. The superconducting instability of the pseudogap ground state is discussed and a ddd-wave superconducting ground state is obtained. This class of pseudogap and superconducting ground states unifies antiferromagnetism, pseudogap, superconductivity, and Mott physics into a new state of matter.
We investigate the entanglement properties of resonating valence bond (RVB) states on a two-dimensional lattice in the presence of dopants that remove electrons from the lattice creating holes. The movement of the holes generated by the Hubbard Hamiltonian in the regime of strong Coulomb repulsion in this setting could be responsible for the phenomenon of high-temperature superconductivity as hypothesized by [Anderson Science 235, 1196 (1987)]. We argue that there is a particular density of dopants (holes) where the entanglement contained in the lattice attains its maximal value for the nearest-neighbor RVB liquid state. This result implies that many-body entanglement may be related to quantum phase transitions that are modeled by RVB theory.
We construct a family of simple fermionic projected entangled pair states (fPEPS) on the square lattice with bond dimension D=3D=3D=3 which are exactly hole-doped resonating valence bond (RVB) wave functions with short-range singlet bonds. Under doping the insulating RVB spin liquid evolves immediately into a superconductor with mixed d+isd+isd+is pairing symmetry whose pair amplitude grows as the square root of the doping. The relative weight between sss-wave and ddd-wave components can be controlled by a single variational parameter ccc. We optimize our ansatz with respect to ccc for the frustrated $t\text{\ensuremath{-}}{J}_{1}\text{\ensuremath{-}}{J}_{2}$ model (including both nearest and next-nearest neighbor antiferromagnetic interactions J1{J}_{1}J1​ and J2{J}_{2}J2​, respectively) for ${J}_{2}\ensuremath{\simeq}{J}_{1}/2$ and obtain an energy very close to the infinite-PEPS state (using full update optimization and same bond dimension). The orbital symmetry of the optimized RVB superconductor has predominant ddd-wave character, although we argue a residual (complex sss-wave) time reversal symmetry breaking component should always be present. Connections of the results to the physics of superconducting cuprates and pnictides are outlined.
We describe a new method to numerically evaluate the properties of correlated superconducting wave functions. We have applied it to the resonating-valence-bond (RVB) wave function for the Hubbard model on the square lattice. For the half-filled case we find that the ddd-wave RVB state and the antiferromagnetic ordered state have the same energy within numerical accuracy. At 10% doping we find ddd-wave superconductivity, consistent with previous studies. We show that the superconducting order parameter is proportional to the number of holes, for small hole concentrations.
Superconductivity is usually described in the framework of the Bardeen-Cooper-Schrieffer (BCS) wavefunction, which even includes the resonating-valence-bond (RVB) wavefunction proposed for the high-temperature superconductivity in the cuprate. A natural question is ififif any fundamental physics could be possibly missed by applying such a scheme to strongly correlated systems. Here we study the pairing wavefunction of two holes injected into a Mott insulator/antiferromagnet in a two-leg ladder using variational Monte Carlo approach. By comparing with density-matrix renormalization group (DMRG) calculation, we show that a conventional BCS or RVB pairing of the doped holes makes qualitatively wrong predictions and is incompatible with the fundamental pairing force in the $t\text{\ensuremath{-}}J$ model, which is kinetic-energy driven by nature. By contrast, a non-BCS-like wavefunction incorporating such novel effect will result in a substantially enhanced pairing strength and improved ground state energy as compared to the DMRG results. We argue that the non-BCS form of such a new ground state wavefunction is essential to describe a doped Mott antiferromagnet at finite doping.