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Bulletin of the American Physical Society

Controlled Rapid Adiabatic Passage in a V-Type System

Yunheung Song, Han-gyeol Lee, Hanlae Jo, Jaewook Ahn

Published May 26, 2016• 0 citations
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We present the experimental demonstration of a novel, efficient, and selective technique to prepare population inversion. The technique is an extension of Stark-chirped rapid adiabatic passage (SCRAP), i.e., SCRAP among three states. In this process a Lambda-type quantum system is driven by two laser pulses, the pump and Stokes pulses, which are appropriately detuned from transition frequencies. A third laser pulse induces a dynamic Stark shift in the upper energy level, and the timing of all three pulses is controlled in order to prepare population inversion between the two lower states in the Lambda-type level scheme. Our data on population transfer in nitric oxide (NO) molecules clearly show that SCRAP among three states provides an advantageous alternative to such techniques as stimulated Raman adiabatic passage.
Inhomogeneous broadening of energy levels is one of the principal limiting factors for achieving ``slow'' or ``stationary'' light in solid-state media by means of electromagnetically induced transparency, a quantum version of stimulated Raman adiabatic passage (STIRAP). Stark-shift-chirped rapid adiabatic-passage (SCRAP) has been shown to be far less sensitive to inhomogeneous broadening than STIRAP, a population transfer technique to which it is closely related. We further optimize the pulses used in SCRAP to be even less sensitive to inhomogeneous broadening in a $\ensuremath{\Lambda}$-type three-level system. The optimized pulses perform at a higher fidelity than the standard Gaussian pulses for a wide range of detunings (i.e., large inhomogeneous broadening).