We examine the dynamics of Rydberg polaritons with dipolar interactions that propagate in multiple spatial modes. The dipolar excitation-exchange between different Rydberg states mediates an effective exchange between polaritons that enables photons to hop across different spatial channels. Remarkably, the efficiency of this photon exchange process can increase with the channel distance and becomes optimal at a finite rail separation. Based on this mechanism, we design a simple photonic network that realises a two photon quantum gate with a robust
π-phase, protected by the symmetries of the underlying photon interaction and the geometry of the network. These capabilities expand the scope of Rydberg-EIT towards multidimensional geometries for nonlinear optical networks and explorations of photonic many-body physics.
We theoretically investigate light propagation and electromagnetically induced transparency in a quasi-one-dimensional gas in which atoms interact strongly via exchange interactions. We focus on the case in which the gas is initially prepared in a many-body state that contains a single excitation and conduct a detailed study of the absorptive and dispersive properties of such a medium. This scenario is achieved in interacting gases of Rydberg atoms with two relevant S states that are coupled through exchange. Of particular interest is the case in which the medium is prepared in an entangled spin-wave state. This, in conjunction with the exchange interaction, gives rise to a nonlocal susceptibility that--in comparison to conventional Rydberg electromagnetically induced transparency--qualitatively alters the absorption and propagation of weak probe light, leading to nonlocal propagation and enhanced absorption.
This thesis investigates new phenomena that arise when light is strongly coupled to an interacting atomic gas. For this, a new apparatus has been built which allows to create ultracold and dense atomic samples and to detect individual atoms in high-lying atomic states, so-called Rydberg atoms. Strong light-matter coupling is achieved using the collective coupling of the atomic cloud to the light field under conditions of electromagnetically induced transparency (EIT). In experiments on EIT involving non-interacting Rydberg states, we characterize the light-matter coupling and demonstrate the first combined optical and matter based probing of EIT. By coupling to strongly-interacting Rydberg states, we investigate the effect of interactions which we observe as a strong nonlinear optical \nresponse of the atomic gas as well as in the emergence of strong correlations between the hybrid quasiparticles associated with the strong light-matter coupling. We employ the nonlinear response of the atomic cloud to image Rydberg atoms immersed in the atomic cloud. In a theoretical proposal, we show that this novel imaging technique allows to investigate many-body Rydberg states with single particle sensitivity. Using the proposed imaging method, we demonstrate imaging of small numbers of Rydberg atoms with high time-resolution in single shot experiments. In experiments exploiting the dipolar exchange interaction between Rydberg atoms, we employ the new imaging technique to follow dipole-mediated transport of Rydberg excitations through the cloud. The transport dynamics is determined by the continuous spatial projection of the electronic quantum state under observation and features an emergent spatial scale of micrometer size induced by Rydberg-Rydberg interactions.