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Interfacing Rydberg atoms with light and observing their interaction driven dynamics

G. Günter

Published Jan 1, 2014• 0 citations
Publisher

Abstract

This thesis investigates new phenomena that arise when light is strongly coupled to an interacting atomic gas. For this, a new apparatus has been built which allows to create ultracold and dense atomic samples and to detect individual atoms in high-lying atomic states, so-called Rydberg atoms. Strong light-matter coupling is achieved using the collective coupling of the atomic cloud to the light field under conditions of electromagnetically induced transparency (EIT). In experiments on EIT involving non-interacting Rydberg states, we characterize the light-matter coupling and demonstrate the first combined optical and matter based probing of EIT. By coupling to strongly-interacting Rydberg states, we investigate the effect of interactions which we observe as a strong nonlinear optical \nresponse of the atomic gas as well as in the emergence of strong correlations between the hybrid quasiparticles associated with the strong light-matter coupling. We employ the nonlinear response of the atomic cloud to image Rydberg atoms immersed in the atomic cloud. In a theoretical proposal, we show that this novel imaging technique allows to investigate many-body Rydberg states with single particle sensitivity. Using the proposed imaging method, we demonstrate imaging of small numbers of Rydberg atoms with high time-resolution in single shot experiments. In experiments exploiting the dipolar exchange interaction between Rydberg atoms, we employ the new imaging technique to follow dipole-mediated transport of Rydberg excitations through the cloud. The transport dynamics is determined by the continuous spatial projection of the electronic quantum state under observation and features an emergent spatial scale of micrometer size induced by Rydberg-Rydberg interactions.

DOI
10.11588/heidok.00016312

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•Jan 1, 2014•1 citation
This thesis investigates new phenomena that arise when light is strongly coupled to an interacting atomic gas. For this, a new apparatus has been built which allows to create ultracold and dense atomic samples and to detect individual atoms in high-lying atomic states, so-called Rydberg atoms. Strong light-matter coupling is achieved using the collective coupling of the atomic cloud to the light field under conditions of electromagnetically induced transparency (EIT). In experiments on EIT involving non-interacting Rydberg states, we characterize the light-matter coupling and demonstrate the first combined optical and matter based probing of EIT. By coupling to strongly-interacting Rydberg states, we investigate the effect of interactions which we observe as a strong nonlinear optical \nresponse of the atomic gas as well as in the emergence of strong correlations between the hybrid quasiparticles associated with the strong light-matter coupling. We employ the nonlinear response of the atomic cloud to image Rydberg atoms immersed in the atomic cloud. In a theoretical proposal, we show that this novel imaging technique allows to investigate many-body Rydberg states with single particle sensitivity. Using the proposed imaging method, we demonstrate imaging of small numbers of Rydberg atoms with high time-resolution in single shot experiments. In experiments exploiting the dipolar exchange interaction between Rydberg atoms, we employ the new imaging technique to follow dipole-mediated transport of Rydberg excitations through the cloud. The transport dynamics is determined by the continuous spatial projection of the electronic quantum state under observation and features an emergent spatial scale of micrometer size induced by Rydberg-Rydberg interactions.
We propose a new all-optical method to image individual Rydberg atoms embedded within dense gases of ground state atoms. The scheme exploits interaction-induced shifts on highly polarizable excited states of probe atoms, which can be spatially resolved via an electromagnetically induced transparency resonance. Using a realistic model, we show that it is possible to image individual Rydberg atoms with enhanced sensitivity and high resolution despite photon-shot noise and atomic density fluctuations. This new imaging scheme could be extended to other impurities such as ions, and is ideally suited to equilibrium and dynamical studies of complex many-body phenomena involving strongly interacting particles. As an example we study blockade effects and correlations in the distribution of Rydberg atoms optically excited from a dense gas.
This thesis investigates how a single highly excited atom, called Rydberg atom, can be optically imaged. Direct detection methods based on the scattering of light are hardly applicable due to the small scattering rate of the ground to Rydberg state transition. Instead, a cloud of ground state atoms, normally absorptive, is rendered transparent using electromagnetically induced transparency (EIT), involving an auxiliary probe Rydberg state. The cloud acts as a contrast medium, whose optical response is locally perturbed by the strong Rydberg-Rydberg interaction between the probe and the Rydberg impurity which we want to detect. This perturbation restores absorption within a small volume around the impurity, readily detected and \nspatially resolved on a camera. We call this technique Interaction Enhanced Imaging (IEI). To implement IEI we characterize the optical response of the EIT contrast \nmedium in absence of interactions. By combining measurements of the spatially resolved optical spectrum and of the total Rydberg atom number, we can reconstruct \nthe full one-body density matrix of the three-level system. Next, we excite |nS> or |nP> states and, using IEI, we demonstrate spatially resolved imaging, enabling us \nto study dipolar energy transport. To reach single impurity sensitivity we investigate our current detection fidelity and characterize the signal and noise contributions in \nIEI. We model our interacting system, finding good agreement with experimental data. Based on this model, we predict combinations of Rydberg states for which single-shot single impurity sensitivity should be possible in future experiments.
This thesis experimentally explores the application of strongly interacting states of Rydberg atoms as means to introduce and control correlations in many-body systems. A new apparatus has been built, which combines high atomic densities possible using optical dipole traps with the ability to detect and probe Rydberg atoms via both field ionization detection and electromagnetically induced transparency. In the first study, the interaction induced excitation of Rydberg atom pairs ('antiblockade') is demonstrated using detuned laser excitation. This provides \nthe possibility to engineer spatial correlations and to control interactions between Rydberg atoms. We then investigate the effects of Rydberg-Rydberg interactions \nand correlations on the spontaneous evolution of the system to an ultracold plasma. The initial correlations between Rydberg atoms should be preserved, suggesting a new route to overcome disorder-induced heating and to enter new strongly coupled regimes. Finally the back-action of Rydberg-Rydberg interactions on propagating light fields is explored. Dissipative interactions between dark-state polaritons give rise to a strongly nonlinear optical response and sub-Poissonian statistics of polaritons \nwhich reflect the emergence of correlations in both the atomic and light fields. Combined, these experiments help elucidate the effects of Rydberg induced correlations on diverse physical systems involving atoms, ions and photons.
This thesis investigates different aspects of strongly interacting ultracold Rydberg gases coupled by light, including the excitation of correlated structures called Rydberg aggregates and dipolar energy transport. For this purpose an experimental apparatus has been constructed. We study coherent population trapping (CPT) and electromagnetically induced transparency (EIT) involving Rydberg states. To study the formation of Rydberg aggregates we use full counting statistics (FCS) which makes it possible to infer the size of Rydberg aggregates. Dephasing during the excitation is found to have a dramatic effect on the formation process, leading to sequential growth around an initial grain. Rydberg state EIT is used to realize a new direct optical imaging scheme for Rydberg atoms which combines highly sensitive detection with high spatial and temporal resolution. Applying this technique we observe dipole-mediated energy transport processes between Rydberg atoms. We study classical transport in the presence of strong measurement induced decoherence. The strong interactions are seen to mediate long-range hopping significantly beyond nearest neighbors. We present first indications for coherent transport in this system. These experiments shed light on the role of correlations in the excitation and evolution of strongly interacting quantum systems and e.g. could possibly be used to model energy transport in biological systems. \n
High optical nonlinearities can be achieved at the single photon level by coupling the photon states to strongly interacting Rydberg excitations under the conditions of electromagnetically induced transparency. The nonlinear response in Rydberg quantum optics comes as a direct result of the long range dipole-dipole interactions via Rydberg blockade and interaction induced dephasing. In this thesis, Rydberg quantum optics experiments are performed with two spatially separated mediums with a nonlinear response at the single photon level. Two ultracold rubidium atomic clouds are tightly confined by a pair of in-vacuo aspheric lenses such that only a few Rydberg excitations can exist in each one of the clouds simultaneously. The long range character of the dipole-dipole interactions leads to the generation of quantum states of light. The effective photon-photon interactions are directly observed as an anti-correlation in the simultaneous photon retrieval as a result of the non resonant van der Waals interactions. The collective Rydberg excitations, stored in the non-overlapping mediums, experience an additional spatial non-uniform phase. In addition, we experimentally characterize the cooperative optical response of a cold atomic medium at a single photon level. This aims to exploit the enhancement of the spontaneous emissions decay rate (superradiance) as a dependence of the number of atoms involved in the ensemble. The observed atomic response in two different regimes gives a further understanding of the system dynamics and unlocks a promising potential route towards the implementation in scalable, multichannel quantum optical devices.
Subject of this thesis is the theoretical investigation of ensembles of atoms that are coherently laser-excited to a Rydberg state. Rydberg excited atoms interact with each other over large distances, which leads to strongly correlated many-body dynamics, demanding powerful numerical tools for their modeling. The first part of the thesis deals with effective two-level atoms consisting of a ground and a Rydberg state only. For resonant laser excitation a modified scaling behavior of the excitation number is observed, which is caused by effects of finite system size and coarse graining of the medium due to the finite atomic density. For off-resonant excitation, ordered structures arise out of an initially homogeneous gas, which are reflected in strongly peaked spatial correlations and modified excitation statistics. In the second part a fast decaying intermediate level is additionally taken into account. In this situation the phenomenon of electromagnetically induced transparency (EIT) is encountered. This effect is suppressed in the presence of strong interactions between the Rydberg atoms leading to an optical nonlinearity. A model predicting the properties of a cloud of Rydberg atoms in EIT configuration is developed. In both parts the models are validated by comparing their predictions to recent experimental observations.