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Single atom emission in an optical resonator

James Childs, Kyungwon An, Ramachandra Rao Dasari

Published Dec 31, 1994• 8 citations
OpenAlex

Abstract

A single atom coupled to a single mode of a radiation field is a fundamental system for studying the interaction of radiation with matter. The study of such systems has come to be called cavity quantum electrodynamics (QED). Atoms coupled to a single mode of a resonator have been studied experimentally and theoretically in several interesting regimes since this basic system was first considered theoretically by Janes and Cummings. The objective of the present chapter is to provide a theoretical framework and present a unifying picture of the various phenomena which can occur in such a system. 35 refs., 11 figs.

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Cavity quantum electrodynamics (cavity QED) describes the interactions of single atoms and single photons in a resonator. In the laboratory, state-of-the-art experiments are able to observe the dynamics of these simple yet fundamental quantum systems. The recent development of quantum information science has also introduced a new role for cavity QED systems as quantum interfaces, in which information can be coherently mapped between photonic and atomic quantum bits. Groundbreaking optical cavity QED experiments in the past twenty years would not have been possible without the technological development of mirror coatings with extremely low scatter and absorption losses. Thermal noise has typically played a smaller role in cavity QED experiments but in certain instances is nevertheless important to consider. In this chapter, we begin with an overview of optical cavity QED experiments and some of the central questions that they address. It is hoped that this description, while by no means exhaustive, will provide a window for the nonspecialist into basic techniques and motivations in the field. We then turn to focus on the roles played by scattering and absorption loss and mechanical loss. We discuss how these losses have set limits on feasible experiments and the extent to which improvements may be possible. Experimental realizations of cavity QED systems An idealized cavity QED system consists of one atom placed between two highly reflective mirrors (Figure 17.1). In this model, a single atomic transition interacts with photons in a single cavity mode; the atom is often pictured at an antinode of the cavity standing wave, where it has a maximal dipole interaction with the cavity field.

Cambridge University Press eBooks•Jan 6, 2012•0 citations

Interaction between Atomic Ensembles and Optical Resonators: Classical Description

Haruka Tanji, Ian D. Leroux, Monika Schleier-Smith +4 more

Many effects in the interaction between atoms and a cavity that are usually de-scribed in quantum mechanical terms (cavity quantum electrodynamics, cavity QED) can be understood and quantitatively analyzed within a classical framework. We adopt such a classical picture of a radiating dipole oscillator to derive explicit ex- pressions for the coupling of single atoms and atomic ensembles to Gaussian modes in free space and in an optical resonator. The cooperativity parameter of cavity QED is shown to play a central role, and is given a geometrical interpretation. The classical analysis yields transparent, intuitive results that are useful for analyzing applications of cavity QED such as atom detection and counting, cavity cooling, cavity spin squeezing, cavity spin optomechanics, or phase transitions associated with the self-organization of the ensemble-light system.

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In this chapter, we discuss a purely quantum approach to the interaction between an atom and the electromagnetic field. In this treatment, the atom and electromagnetic field form a single quantum system, whose evolution is handled globally within a unified formalism. This will thus have the merit of being fully consistent from the theoretical standpoint. But the main advantage in an entirely quantum approach is that it can treat the full range of matter–radiation interaction phenomena. In particular, it provides a rigorous description of the spontaneous emission of light by an excited atom , something that falls outside the scope of the semi-classical framework applied in Chapters 2 and 3, where the lifetime of an excited atomic state had to be fed in phenomenologically. It can describe other phenomena of the same type, such as parametric fluorescence by a nonlinear crystal subjected to pumping radiation (see Chapter 7), which underlies many recent developments in quantum optics. The fully quantum approach also has the merit of allowing a simple interpretation in terms of photons for the various matter–radiation interaction processes, such as absorption, stimulated emission, scattering, and also the basic processes of nonlinear optics. Indeed, it provides a unified framework for both stimulated and spontaneous processes. Finally, it can be used to tackle completely new situations where matter and radiation interact, which lie outside the scope of any semi-classical description, such as cavity quantum electrodynamics or the production of single-photon or entangled-photons states .

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Cavity quantum electrodynamics (cavity QED) describes electromagnetic fields in a confined space and the radiative properties of atoms in such fields. The simplest example of such system is a single atom interacting with one mode of a high-finesse resonator. Besides observation and exploration of fundamental quantum mechanical effects, this system bears a high potential for applications quantum information science such as, e.g., quantum logic gates, quantum communication and quantum teleportation. In this thesis I present an experiment on the deterministic coupling of a single neutral atom to the mode of a high-finesse optical resonator. In Chapter 1 I describe our basic techniques for trapping and observing single cesium atoms. As a source of single atoms we use a high-gradient magneto-optical trap, which captures the atoms from background gas in a vacuum chamber and cools them down to millikelvin temperatures. The atoms are then transferred without loss into a standing-wave dipole trap, which provides a conservative potential required for experiments on atomic coherence such as quantum information processing and metrology on trapped atoms. Moreover, shifting the standing-wave pattern allows us to deterministically transport the atoms (Chapter 2). In combination with non-destructive fluorescence imaging of individual trapped atoms, this enables us to control their position with submicrometer precision over several millimeters along the dipole trap. The cavity QED system can distinctly display quantum behaviour in the so-called strong coupling regime, i.e., when the coherent atom-cavity coupling rate dominates dissipation in the system. This sets the main requirements on the resonator's properties: small mode volume and high finesse. Chapter 3 is devoted to the manufacturing, assembling, and testing of an ultra-high finesse optical Fabry-Perot resonator, stabilized to the atomic transition. In Chapter 4 I present the transportation of single atoms into the cavity and their coupling to the cavity mode. The strong coupling manifests itself in a strong reduction of the cavity transmission probed by a weak external laser. The atoms remain trapped and coupled to the cavity mode for several seconds until we move them out of the cavity for final analysis of their number and position.

•Jan 1, 2007•5 citations

Focus section on Cavity QED

Wolfgang Lange, Jean‐Michel Gérard

A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.

Journal of Optics B Quantum and Semiclassical Optics•Feb 1, 2004•0 citations

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Alexander Kubanek, Alexei Ourjoumtsev, I. Schuster +4 more

Atoms absorb and emit resonant light photon by photon. However, an atom strongly coupled to the light field of a high-finesse optical resonator forms a new system with new characteristics, enabling the emission and absorption of photon pairs. The energy eigenstates of the coupled system form an anharmonic ladder of doublets, the so-called Jaynes-Cummings ladder. The first doublet, consisting of the two so-called normal modes, has been observed in various cavity QED systems. It can be explained classically using Maxwell equations as arising from the coupling of a classical dipole to a classical electromagnetic field. In contrast, the higher-order doublet has so far no classical analogue. It requires both the quantization of the atomic internal state as well as the quantization of light.

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 1, 2009•13 citations
A single atom coupled to a single mode of a radiation field is a fundamental system for studying the interaction of radiation with matter. The study of such systems has come to be called cavity quantum electrodynamics (QED). Atoms coupled to a single mode of a resonator have been studied experimentally and theoretically in several interesting regimes since this basic system was first considered theoretically by Janes and Cummings. The objective of the present chapter is to provide a theoretical framework and present a unifying picture of the various phenomena which can occur in such a system. 35 refs., 11 figs.
Cavity quantum electrodynamics (cavity QED) describes the interactions of single atoms and single photons in a resonator. In the laboratory, state-of-the-art experiments are able to observe the dynamics of these simple yet fundamental quantum systems. The recent development of quantum information science has also introduced a new role for cavity QED systems as quantum interfaces, in which information can be coherently mapped between photonic and atomic quantum bits. Groundbreaking optical cavity QED experiments in the past twenty years would not have been possible without the technological development of mirror coatings with extremely low scatter and absorption losses. Thermal noise has typically played a smaller role in cavity QED experiments but in certain instances is nevertheless important to consider. In this chapter, we begin with an overview of optical cavity QED experiments and some of the central questions that they address. It is hoped that this description, while by no means exhaustive, will provide a window for the nonspecialist into basic techniques and motivations in the field. We then turn to focus on the roles played by scattering and absorption loss and mechanical loss. We discuss how these losses have set limits on feasible experiments and the extent to which improvements may be possible. Experimental realizations of cavity QED systems An idealized cavity QED system consists of one atom placed between two highly reflective mirrors (Figure 17.1). In this model, a single atomic transition interacts with photons in a single cavity mode; the atom is often pictured at an antinode of the cavity standing wave, where it has a maximal dipole interaction with the cavity field.
Many effects in the interaction between atoms and a cavity that are usually de-scribed in quantum mechanical terms (cavity quantum electrodynamics, cavity QED) can be understood and quantitatively analyzed within a classical framework. We adopt such a classical picture of a radiating dipole oscillator to derive explicit ex- pressions for the coupling of single atoms and atomic ensembles to Gaussian modes in free space and in an optical resonator. The cooperativity parameter of cavity QED is shown to play a central role, and is given a geometrical interpretation. The classical analysis yields transparent, intuitive results that are useful for analyzing applications of cavity QED such as atom detection and counting, cavity cooling, cavity spin squeezing, cavity spin optomechanics, or phase transitions associated with the self-organization of the ensemble-light system.
In this chapter, we discuss a purely quantum approach to the interaction between an atom and the electromagnetic field. In this treatment, the atom and electromagnetic field form a single quantum system, whose evolution is handled globally within a unified formalism. This will thus have the merit of being fully consistent from the theoretical standpoint. But the main advantage in an entirely quantum approach is that it can treat the full range of matter–radiation interaction phenomena. In particular, it provides a rigorous description of the spontaneous emission of light by an excited atom , something that falls outside the scope of the semi-classical framework applied in Chapters 2 and 3, where the lifetime of an excited atomic state had to be fed in phenomenologically. It can describe other phenomena of the same type, such as parametric fluorescence by a nonlinear crystal subjected to pumping radiation (see Chapter 7), which underlies many recent developments in quantum optics. The fully quantum approach also has the merit of allowing a simple interpretation in terms of photons for the various matter–radiation interaction processes, such as absorption, stimulated emission, scattering, and also the basic processes of nonlinear optics. Indeed, it provides a unified framework for both stimulated and spontaneous processes. Finally, it can be used to tackle completely new situations where matter and radiation interact, which lie outside the scope of any semi-classical description, such as cavity quantum electrodynamics or the production of single-photon or entangled-photons states .
Cavity quantum electrodynamics (cavity QED) describes electromagnetic fields in a confined space and the radiative properties of atoms in such fields. The simplest example of such system is a single atom interacting with one mode of a high-finesse resonator. Besides observation and exploration of fundamental quantum mechanical effects, this system bears a high potential for applications quantum information science such as, e.g., quantum logic gates, quantum communication and quantum teleportation. In this thesis I present an experiment on the deterministic coupling of a single neutral atom to the mode of a high-finesse optical resonator. In Chapter 1 I describe our basic techniques for trapping and observing single cesium atoms. As a source of single atoms we use a high-gradient magneto-optical trap, which captures the atoms from background gas in a vacuum chamber and cools them down to millikelvin temperatures. The atoms are then transferred without loss into a standing-wave dipole trap, which provides a conservative potential required for experiments on atomic coherence such as quantum information processing and metrology on trapped atoms. Moreover, shifting the standing-wave pattern allows us to deterministically transport the atoms (Chapter 2). In combination with non-destructive fluorescence imaging of individual trapped atoms, this enables us to control their position with submicrometer precision over several millimeters along the dipole trap. The cavity QED system can distinctly display quantum behaviour in the so-called strong coupling regime, i.e., when the coherent atom-cavity coupling rate dominates dissipation in the system. This sets the main requirements on the resonator's properties: small mode volume and high finesse. Chapter 3 is devoted to the manufacturing, assembling, and testing of an ultra-high finesse optical Fabry-Perot resonator, stabilized to the atomic transition. In Chapter 4 I present the transportation of single atoms into the cavity and their coupling to the cavity mode. The strong coupling manifests itself in a strong reduction of the cavity transmission probed by a weak external laser. The atoms remain trapped and coupled to the cavity mode for several seconds until we move them out of the cavity for final analysis of their number and position.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
Atoms absorb and emit resonant light photon by photon. However, an atom strongly coupled to the light field of a high-finesse optical resonator forms a new system with new characteristics, enabling the emission and absorption of photon pairs. The energy eigenstates of the coupled system form an anharmonic ladder of doublets, the so-called Jaynes-Cummings ladder. The first doublet, consisting of the two so-called normal modes, has been observed in various cavity QED systems. It can be explained classically using Maxwell equations as arising from the coupling of a classical dipole to a classical electromagnetic field. In contrast, the higher-order doublet has so far no classical analogue. It requires both the quantization of the atomic internal state as well as the quantization of light.