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Physical Review A

Double Lorentzian atomic prism

David J. Starling, Steven M. Bloch, Praveen K. Vudyasetu, Joseph S. Choi, Bethany Little, John C. Howell

Published Aug 16, 2012• 18 citations
Publisher

Abstract

We present an atomic prism spectrometer that utilizes the steep linear dispersion between two strongly absorbing hyperfine resonances of rubidium. We resolve spectral lines 50 MHz apart and, utilizing a larger part of the available spectrum than only between the two resonances, we spatially separate collinear pump, signal, and idler beams resulting from a four-wave mixing process. Due to the high transparency possible between the resonances, these results have applications in the filtering of narrow-band entangled photons and interaction-free measurements.

DOI
10.1103/physreva.86.023826

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Journal of the Optical Society of America B•Jun 27, 2014•18 citations
We present an atomic prism spectrometer that utilizes the steep linear dispersion between two strongly absorbing hyperfine resonances of rubidium. We resolve spectral lines 50 MHz apart and, utilizing a larger part of the available spectrum than only between the two resonances, we spatially separate collinear pump, signal, and idler beams resulting from a four-wave mixing process. Due to the high transparency possible between the resonances, these results have applications in the filtering of narrow-band entangled photons and interaction-free measurements.
We report a new spectroscopy method achieved by combined refraction and propagation delay of light pulses passing through a prism cell filled with an atomic vapor. The atomic vapor medium has strong refractive index gradients near the atomic resonant absorption features, and these features enable the separation in time and space of different spectral features of a light pulse propagating through the vapor cell. The gradient of the refractive index leads to a slowing of the light pulse, while simultaneously, the magnitude of the refractive index and the prismatic windows or internal prism elements of the atomic vapor cell spatially separate the frequencies due to dispersion. The combination of these two effects leads to high-resolution spectral selectivity and strong suppression of out-of-band light. Applications are achieved for Rayleigh, Raman, and Thomson spectroscopy for which the wavelength of the scattering spectra tracks the wavelength of the excitation laser source. The laser is tuned such that the spectral line of interest falls near the resonance of the atomic vapor. Applications for rotational Raman spectroscopy are of particular interest since specific Raman lines can be selected while other Raman lines as well as background Rayleigh and other scattering are strongly rejected.
Four-wave-mixing (FWM) radiation is generated between the hyperfine structures of the 5D and 5P states in a thermally broadened rubidium atomic vapor using resonant atomic coherence. Background-free unidirectional signals having narrow spectral linewidths are isolated and experimentally studied in the frequency domain, and the effects of the driving beam parameters on the properties of the radiation are discussed. The radiation has several new properties compared to traditional FWM radiations generated between the 5P and 5S states. The high-resolution signals obtained in this method could make it favorable in spectroscopic procedures that rely on two-photon fluorescence.
Continuous wave extended cavity diode lasers are used to measure the absorptive and dispersive properties of the 5 2S1/2 → 5 (^2)Рз/2 resonance, at 780 nm, in Rubidium (Rb) vapour. The Doppler-broadened hyperfine transitions are studied both with and without a pump beam. The investigation concentrates on three-level Л-systems, realized in the presence of a pump beam, exhibiting Electromagnetically Induced Transparency (EIT). Electromagnetically Induced Absorption (EIA) IS also seen. The EIT and EIA resonances can be several orders of magnitude narrower than the natural line width of the atomic transitions in the absence of the pump beam. Further, the EIT resonances are sensitive to applied magnetic fields. The narrowest resonances measured in this work have a full-width at half- maximum of 〜 80 kHz. This is limited by the transit time of the atoms through the probe and pump beams. Predictions of theoretical calculations and models are compared to experimental results. The theory of beam splitters and interferometers is developed to enable the implementation of a Sagnac interferometer in a novel "biased" alignment. This allows the dispersion of atomic resonances to be measured directly. The direct measurement of the dispersion of the narrow EIT features in a "biased" Sagnac interferometer is presented. Such a signal is ideally suited to precision measurement applications such 88 inertial sensing and magnetometry.
An ongoing spectroscopic investigation of atomic rubidium utilizes a two-photon, single-laser excitation process. Transitions accessible with our tunable laser include 5P1/2 (F ′ ) ← 5S1/2 (F) and 5P3/2 (F ′ ) ← 5S1/2 (F). The laser is split into a pump and probe beam to allow for Doppler-free measurements of transitions between hyperfine levels. The pump and probe beams are overlapped in a counter-propagating geometry and the laser frequency scans over a transition. Absorption, fluorescence and polarization spectroscopy techniques are applied to this basic experimental setup. The temperature of the vapor cell and the power of the pump and probe beams have been varied to explore line broadening effects and signal-to-noise of each technique. This humble setup will hopefully grow into a more robust experimental arrangement in which double resonance, two-laser excitations are used to explore hyperfine state changing collisions between rubidium atoms and noble gas atoms. Rb-noble gas collisions can transfer population between hyperfine levels, such as 5P3/2 (F ′ = 3) Collision ←− 5P3/2 (F ′ = 2), and the probe beam couples 7S1/2 (F ′′ = 2) ← 5P3/2 (F ′ = 3). Polarization spectroscopy signal depends on the rate of population transfer due to the collision as well as maintaining the orientation created by the pump laser. Fluorescence spectroscopy relies only on transfer of population due to the collision. Comparison of these techniques yields information regarding the change of the magnetic sublevels, mF , during hyperfine state changing collisions.
We report on observations of four-wave mixing in rubidium vapor via two-photon resonant excitation with nd and (n+2)s states, for n=14–20. The intensity of the generated beam is studied in a collinear configuration, and the results are consistent with the predictions of a theoretical model based on the semiclassical Maxwell–Bloch equations, considering interference effects associated with multiple excitation pathways and with internally generated fields. We have also observed spectral broadening of the two-photon resonant lines, which is well described by a linear dependence on atomic density, in accordance with collision-induced broadening.