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Physical Review A

Rephasing of optically driven atomic coherences by rapid adiabatic passage in Pr 3+ :Y 2 SiO 5

Simon Mieth, Daniel Schraft, Thomas Halfmann, Леонід Петрович Яценко

Published Dec 6, 2012• 15 citations
Publisher

Abstract

We present experimental investigations of rephasing optically driven atomic coherences, prepared by electromagnetically induced transparency in a Pr${}^{3+}$:Y${}_{2}$SiO${}_{5}\phantom{\rule{0.16em}{0ex}}$ crystal. In particular, we systematically study rephasing based on rapid adiabatic passage and compare the performance of the latter with standard rephasing based on Hahn spin echoes. The data clearly demonstrate the superior performance of rapid adiabatic passage for any application of rephasing, which suffers from large inhomogeneous broadenings in the medium or inevitable fluctuations in the experimental parameters.

DOI
10.1103/physreva.86.063404

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We experimentally study a broadband implementation of the atomic frequency comb (AFC) rephasing protocol with a cryogenically cooled P r 3 + : Y 2 S i O 5 crystal. To allow for storage of broadband pulses, we explore a novel, to the best of our knowledge, regime where the input photonic bandwidth closely matches the inhomogeneous broadening of the material ( ∼ 5 G H z ) , thereby significantly exceeding the hyperfine ground and excited state splitting ( ∼ 10 M H z ) . Through an investigation of different AFC preparation parameters, we measure a maximum efficiency of 10% after a rephasing time of 12.5 ns. With a suboptimal AFC, we witness up to 12 rephased temporal modes.
We examine electromagnetically induced transparency (EIT), the optical preparation of persistent nuclear spin coherences and the retrieval of light pulses both in a Λ-type and a V-type coupling scheme in a Pr 3+ :Y 2 SiO 5 crystal, cooled to cryogenic temperatures. The medium is prepared by optical pumping and spectral hole burning, creating a spectrally isolated Λ-type and a V-type system within the inhomogeneous bandwidth of the 3 H 4 ↔ 1 D 2 transition of the Pr 3+ ions. By EIT, in the Λ-type scheme we drive a nuclear spin coherence between the ground-state hyperfine levels, while in the V-type scheme we drive a coherence between the excited-state hyperfine levels. We observe the cancellation of absorption due to EIT and the retrieval of light pulses in both level schemes. This also permits the determination of dephasing times of the nuclear spin coherence, either in the ground state or the optically excited state.
We demonstrate efficient storage and retrieval of light pulses by electromagnetically induced transparency (EIT) in a Pr^{3+}:Y_{2}SiO_{5} crystal. Using a ring-type multipass configuration, we increase the optical depth (OD) of the medium up to a factor of 16 towards OD≈96. Combining the large optical depth with optimized conditions for EIT, we reach a light storage efficiency of (76.3±3.5)%. In addition, we perform extended systematic measurements of the storage efficiency versus optical depth, control Rabi frequency, and probe pulse duration. The data confirm the theoretically expected behavior of an EIT-driven solid-state memory.
Abstract We experimentally demonstrate spatial confinement of atomic excitation by adiabatic passage processes in a rare-earth ion-doped Pr3+:Y2SiO5 crystal. In particular, we apply stimulated Raman adiabatic passage (STIRAP) and compare its performance with electromagnetically induced transparency (EIT). Using a Stokes beam with Gaussian and a pump beam with donut shape we localize the atomic population in the zero-intensity center of the latter. Our data confirm that adiabatic passage confines excitation far below the diameter of the driving laser beams, and that this localization rapidly increases with laser intensity. We find, that STIRAP significantly outperforms EIT, as it was predicted by previous theory proposals, i.e., STIRAP reaches small excitation volumes with much lower laser intensity. The experimental data agree very well with numerical simulations. The findings serve as a step towards new applications for STIRAP, to prepare excitation regions or population patterns in space with large resolution.