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Physical Review A

Two-photon-counting interferometry

Fabien Boitier, Antoine Godard, N. Dubreuil, Philippe Delaye, Claude Fabre, E. Rosencher

Published Jan 31, 2013• 33 citations
Publisher

Abstract

Two-photon-counting interferometry has been realized by measuring the electrical current due to two-photon absorption in the space-charge layer of a semiconductor detector located at the output port of an interferometer. We apply this technique to study the correlation properties of twin beams issued from parametric fluorescence. We describe in detail how the different second-order correlation functions (interbeam, intrabeam) can be extracted at the femtosecond time scale from raw data. The values of these correlation functions determined by our experiments are in excellent agreement with theory. More precisely, extrabunching in twin beams is unambiguously demonstrated and theoretically described using two models: a comprehensive multimode quantum optics model and a simpler classical stochastic approach. Given the high brightness of our twin-beam source, both theories yield similar results. Finally, convenient analytical expressions of the correlation functions were derived from both theories, expressions in which we have been able to relate specific terms to accidental and exact coincidences between photons. Two-photon interferometry thus determines to which extent twin photons are twin. This technique should become a useful tool for future quantum optics developments.

DOI
10.1103/physreva.87.013844

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Two-photon-counting interferometry has been realized by measuring the electrical current due to two-photon absorption in the space-charge layer of a semiconductor detector located at the output port of an interferometer. We apply this technique to study the correlation properties of twin beams issued from parametric fluorescence. We describe in detail how the different second-order correlation functions (interbeam, intrabeam) can be extracted at the femtosecond time scale from raw data. The values of these correlation functions determined by our experiments are in excellent agreement with theory. More precisely, extrabunching in twin beams is unambiguously demonstrated and theoretically described using two models: a comprehensive multimode quantum optics model and a simpler classical stochastic approach. Given the high brightness of our twin-beam source, both theories yield similar results. Finally, convenient analytical expressions of the correlation functions were derived from both theories, expressions in which we have been able to relate specific terms to accidental and exact coincidences between photons. Two-photon interferometry thus determines to which extent twin photons are twin. This technique should become a useful tool for future quantum optics developments.
For many years twin beams originating from parametric down-converted light beams have aroused great interest and attention in the photonics community. One particular aspect of the twin beams is their peculiar intensity correlation functions, which are related to the coincidence rate of photon pairs. Here we take advantage of the huge bandwidth offered by two-photon absorption in a semiconductor to quantitatively determine correlation functions of twin beams generated by spontaneous parametric down-conversion. Compared with classical incoherent sources, photon extrabunching is unambiguously and precisely measured, originating from exact coincidence between down-converted pairs of photons, travelling in unison. These results strongly establish that two-photon counting in semiconductors is a powerful tool for the absolute measurement of light beam photon correlations at ultrashort timescales. The second order correlation functiong(2) is used to test quantum correlation properties of light. Here, two-photon counting is used to measure g(2)and an extrabunching effect is demonstrated, providing evidence that two-photon counting is an appropriate method for measuring light beam photon correlations.
Two-photon correlation measurement provides a promising way to experimentally demonstrate the statistical nature of a light source, which is very significant for the deep understanding of the photon-generating process and the diagnosing of the coherence property. Quantitatively two- photon correlation is described by second-order coherence. Usually the behavior of the second-order coherence against any of the parameters defining the phase volume is different for different photon statistics. The Poisson photon statistics for coherent light gives its second-order coherence as a flat response; The Bose-Einstein photon statistics for chaotic light gives its second-order coherence as a bunching effect; While the Sub-Poisson photon statistics for non-classical light gives its second-order coherence as an anti-bunching effect. Therefore the measurement of two-photon correlation is proved to be a good finger print to check whether light is in coherent state or incoherent state such as thermal state or non-classical state. Historically the measurement of two-photon correlation was first performed by Hanbury-Brown and Twiss (HBT) in 1956. They used a linear mixer to realize the correlation of the two currents from the photoelectric detectors illuminated by a stationary thermal light souece, a mercury arc, and the photo-bunching effect was first successfully observed in the visible region of 435.8 nm. HBT method is no doubt a good way to extract the small excess two-photon correlation for a stationary light because the background, that is the DC components, has been cut off automatically by the broad band amplifiers, which is in fact the key of the success of HBT experiment. However there exists a general problem, to which no attention has ever been paid, in measuring the two-photon correlation of non-stationary light such as synchrotron radiation (SR) by the HBT method. Here the "non-stationary" means a sense of classical mechanics that the observed intensity has some deterministic time structure. The systematic time structure of SR decided by the bunch distribution of the electric current in a storage ring will give rise to a large amount of unexpected accidental correlation, which in fact has nothing to do with the inherent photon statistics of light source and usually l000~l0000 times larger than the true two-photon correlation due to the short bunch separation length (2ns) and the short coherence time (~0.1ps) which is not comparable to the time resolution (1ns) of the measuring system. The existence of the accidental correlation would severely prevent us from observing the bunching effect of the true two-photon correlation. Therefore to suppress the much larger accidental correlation and to extract the small true two-photon correlation, a novel intensity interferometer has been developed for soft X-ray synchrotron radiation. This intensity interferometer consists of an optical vacuum chamber and an electric correlator. All the essential optical elements which includes a wire scanner, a precise diffraction slit, a grating monochromator with a coherence time modulator, a beam divider and two fast-response photon detectors (microchannel plates) are mounted in this high vacuum chamber. The electric correlator completes the multiplication of the two broad band electric currents coming from the photoelectric detectors. The basic idea to suppress the much larger accidental correlation is to modulate the coherence time by modulating the entrance slit width of the monochromator by a piezoclectric translator. The two sets of light intensity are simultaneously modulated too. When the frequency of modulation is f, the third harmonics 3f is detected with a loch-in amplifier because the 3f components include only the true two-photon correlation. Practically it is difficult to modulate with frequency f without any higher order harmonics distortion which might add some false 3f components. To overcome this difficulty we have used a sharp bandpass filter of l00~350 MHz in each branch of the correlator, which is lower than the RF frequency 500 MHz and much higher than 1.6 MHz, the revolution frequency of the stored beam of the 2.5 GeV storage ring. This new apparatus has been operated successfully in the measurement of the horizontal two-photon correlation for the first harmonic of undulator radiation with photon energy of 70 eV at the Photon Factory, KEK. By narrowing the precise slit width which correspondingly changes the spatial coherence of the incident SR, a bunching effect of the normalized excess two-photon correlation has been clearly observed. This explicit bunching effect implies that synchrotron radiation is chaotic radiation. Further investigation shows that although second-order coherence is completely determined by the first-order coherence for the case of chaotic light, the measured information from the light source is essentially different. The two-photon correlation of synchrotron radiation does not depend on the response time of the detectors but gives the information of instantaneous emittance of the stored beam with the time scale of coherence time τC. By fitting the experimental data, the horizontal instantaneous emittance of the stored beam is estimated to be 40nmrad. This intensity interferometer can be utilized to characterize the coherence properties of incomplete FELs, such as SASE, because if they are fully coherent light sources the normalized excess two-photon correlation would have a flat response, but not showing a photon-bunching effect.
Two-photon absorption in GaAs occurs once two photon impinge on the semiconductor surface within the virtual state lifetime, i.e. few fs. Two photon conductivity (TPC) in GaAs is thus particulary well fitted to measure photon coincidence rates in the femtosecond range. Using this new TPC technique we have evidenced various original quantum properties of light, such as photon bunching in thermal light and extrabunching of twin beams. This technique opens new avenues in quantum optics, for quantum cryptography, ghost imaging or non linear optics.
Abstract Quantum metrology deals with improving the resolution of instruments that are otherwise limited by shot noise and it is therefore a promising avenue for enabling scientific breakthroughs. The advantage can be even more striking when quantum enhancement is combined with correlation techniques among several devices. Here, we present and realize a correlation interferometry scheme exploiting bipartite quantum correlated states injected in two independent interferometers. The scheme outperforms classical analogues in detecting a faint signal that may be correlated/uncorrelated between the two devices. We also compare its sensitivity with that obtained for a pair of two independent squeezed modes, each addressed to one interferometer, for detecting a correlated stochastic signal in the MHz frequency band. Being the simpler solution, it may eventually find application to fundamental physics tests, e.g., searching for the effects predicted by some Planck scale theories.