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Physical Review B

Effective spin diffusion in spin-polarized equilibrium and quasiequilibrium Fermi liquids

Hari P. Dahal, Kevin S. Bedell

Published May 3, 2013• 1 citation
Publisher

Abstract

We calculate the effective spin diffusion coefficient of weak ferromagnet and quasiequilibrium paramagnetic systems using Landau Fermi liquid theory. We find that the behavior of the diffusion coefficient of the quasiequilibrium system is determined primarily by the internal magnetic field, which, in turn, depends upon the nonequilibrium magnetization and the antisymmetric Landau parameters. We also show that this is qualitatively similar to the diffusion coefficient of the weak ferromagnetic system. We discuss its implication for the spin-polarized state created in cold atom systems.

DOI
10.1103/physrevb.87.174406

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We calculate the effective spin diffusion coefficient of weak ferromagnet and quasiequilibrium paramagnetic systems using Landau Fermi liquid theory. We find that the behavior of the diffusion coefficient of the quasiequilibrium system is determined primarily by the internal magnetic field, which, in turn, depends upon the nonequilibrium magnetization and the antisymmetric Landau parameters. We also show that this is qualitatively similar to the diffusion coefficient of the weak ferromagnetic system. We discuss its implication for the spin-polarized state created in cold atom systems.
Linear equations for the transverse spin dynamics in a weakly polarized degenerate Fermi liquid are derived from the Landau-Silin phenomenological kinetic equation with a general two-particle collision integral. Unlike a previous treatment where the Fermi velocity and density of states were taken to be constant independent of polarization we make no such assumption. The equations found describe the spin dynamics in a paramagnetic Fermi liquid with finite polarization as well in an itinerant ferromagnet. The results are confirmed by field theoretical calculations based on the integral equation for the vertex function. The transverse spin wave frequency in a polarized paramagnetic Fermi liquid is found to be proportional to k2{k}^{2}k2 with a complex diffusion coefficient such that the damping has a finite value proportional to the quasiparticles scattering rate at T=0T=0T=0. This behavior of a polarized Fermi liquid contrasts with the behavior of a Heisenberg ferromagnet in the hydrodynamic regime where the transverse spin-wave attenuation appears in terms proportional to k4{k}^{4}k4. The reactive part of the diffusion coefficient in a paramagnetic state at T=0T=0T=0 proves to be inversely proportional to the magnetization whereas in a ferromagnetic it is directly proportional to the magnetization. The dissipative part of the diffusion coefficient at T=0T=0T=0 in the paramagnetic state is polarization independent, whereas in the ferromagnetic state it is proportional to the square of the magnetization. Moreover, the spin wave spectrum in a ferromagnetic Fermi liquid proves to be unstable demonstrating the difficulty of applying a Fermi liquid description to itinerant ferromagnetism.
We derive the linearized spin dynamics for paramagnetic quantum liquids. In these systems, the existence of quantum-mechanical exchange in the presence of (an externally induced) broken symmetry in spin space gives rise to a coherent precession of the spins damped by diffusion. Such collective oscillations occur as a result of the precession of the spin current about a macroscopic local exchange field generated either by an external polarizing magnetic field (as in dilute nondegenerate spin-polarized gases) or by the long-lived nonequilibrium polarization (as in degenerate Fermi liquids). We use a unified approach based on the Kadanoff-Baym formulation of the kinetic equations to describe these phenomena. The connection between strongly and weakly interacting paramagnetic systems is made obvious by considering two special cases: (1) a weakly interacting spin-polarized quantum gas and (2) a parametrization of strongly correlated degenerate Fermi liquids in terms a weakly interacting gas of ``quasiparticles.'' Transport coefficients are calculated with a novel method which may be generalizable to systems with no translational invariance.
We present a finite temperature calculation of the transverse spin-diffusion coefficient ${D}_{\ensuremath{\perp}}$ in a dilute degenerate Fermi gas, in the presence of a small external magnetic field HHH. While the longitudinal diffusion coefficient displays the conventional Fermi-liquid dependence, ${D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}$, the behavior of ${D}_{\ensuremath{\perp}}$ shows three separate regimes: (a) ${D}_{\ensuremath{\perp}}\ensuremath{\sim}{H}^{\ensuremath{-}2}$ for $T\ensuremath{\ll}H$, (b) ${D}_{\ensuremath{\perp}}\ensuremath{\sim}{T}^{\ensuremath{-}2}$, $\frac{{D}_{\ensuremath{\perp}}}{{D}_{\ensuremath{\parallel}}}\ensuremath{\ne}1$ for $T\ensuremath{\gg}H$ and large spin-rotation parameter $\ensuremath{\xi}\ensuremath{\gg}1$, and (c) ${D}_{\ensuremath{\perp}}={D}_{\ensuremath{\parallel}}\ensuremath{\propto}{T}^{\ensuremath{-}2}$ for $T\ensuremath{\gg}H$ and $\ensuremath{\xi}\ensuremath{\ll}1$. Our results are qualitatively consistent with the experimental data in weakly spin-polarized 3He^{3}\mathrm{He}3He and 3He^{3}\mathrm{He}3He- 4He^{4}\mathrm{He}4He mixtures.
We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.
We have studied NMR spin echoes in 3He^{3}\mathrm{He}3He liquid in a magnetic field B0{\mathit{B}}_{0}B0​=8 T for temperatures T\ensuremath{\ge}4.5 mK. The data are analyzed in terms of the Leggett-Rice effect to obtain the transverse spin-diffusion coefficient ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$(T). For T20 mK we find that ${\mathit{D}}_{\mathrm{\ensuremath{\perp}}}$ is less than measured in earlier experiments at lower B0{\mathit{B}}_{0}B0​. This phenomenon has been predicted for degenerate Fermi systems, due to the phase space created for quasiparticle scattering by spin polarization. The effect we have measured is more pronounced than suggested by scaling a dilute-gas theory result by a Fermi-liquid factor.
With neutron star applications in mind, we developed a theory of diffusion in mixtures of superfluid, strongly interacting Fermi liquids. By employing the Landau theory of Fermi liquids, we determined matrices that relate the currents of different particle species, their momentum densities, and the partial entropy currents to each other. Using these results, and applying the quasiclassical kinetic equation for the Bogoliubov excitations, we derived general expressions for the diffusion coefficients, which properly incorporate all the Fermi-liquid effects and depend on the momentum transfer rates between different particle species. The developed framework can be used as a starting point for systematic calculations of the diffusion coefficients (as well as other kinetic coefficients) in superfluid Fermi mixtures, particularly, in superfluid neutron stars.