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Chinese Physics Letters

Observation of Spin Polarized Clock Transition in 87 Sr Optical Lattice Clock

Qiang Wang, Yige Lin, Ye Li, Bai-Ke Lin, Fei Meng, Erjun Zang, Tianchu Li, Zhanjun Fang

Published Dec 1, 2014• 8 citations
Publisher

Abstract

We report our observation of the spin polarized 1 S 0 → 3 P 0 clock transition spectrum in an optical lattice clock based on fermionic 87 Sr. The atoms are trapped and pre-cooled to about 2 μK with two stages of laser cooling at 461 nm and 689 nm, respectively. Then the atoms are loaded into an optical lattice formed by the interference of counter-propagating laser beams at 813 nm. An external cavity diode laser at 698 nm, which is stabilized to a high finesse cavity with a linewidth of about 5 Hz and a drift rate of less than 0.2 Hz/s, is used to excite the atoms to the 3 P 0 state. The π-polarized clock transition spectrum of resolvable m F states is obtained by applying a small bias magnetic field along the polarization axis of the probe beam. A spin polarized clock transition spectrum as narrow as 10 Hz with an 80 ms probe pulse is obtained.

DOI
10.1088/0256-307x/31/12/123201

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We report our observation of the spin polarized 1 S 0 → 3 P 0 clock transition spectrum in an optical lattice clock based on fermionic 87 Sr. The atoms are trapped and pre-cooled to about 2 μK with two stages of laser cooling at 461 nm and 689 nm, respectively. Then the atoms are loaded into an optical lattice formed by the interference of counter-propagating laser beams at 813 nm. An external cavity diode laser at 698 nm, which is stabilized to a high finesse cavity with a linewidth of about 5 Hz and a drift rate of less than 0.2 Hz/s, is used to excite the atoms to the 3 P 0 state. The π-polarized clock transition spectrum of resolvable m F states is obtained by applying a small bias magnetic field along the polarization axis of the probe beam. A spin polarized clock transition spectrum as narrow as 10 Hz with an 80 ms probe pulse is obtained.
We demonstrate a spin-polarized clock transition spectrum of the 87Sr optical lattice clock. The clock transition 5s2 1S05s5p 3P0 of isotope 87Sr has a hyperfine structure due to non-zero nuclear spin, inducing ten -polarized transitions from each individual mF state under the condition of a bias magnetic field along the probing polarization axis. In this experiment, atoms are driven to a certain mF state by a circular-polarization pump light to maximize the atomic population, which is beneficial to the stability and uncertainty evaluation of the optical lattice clock. After two stages cooling and trapping, about 3.5106 atoms are trapped in the red magneto-optical trap with a temperature of 3.9 K. A grating-feedback external cavity diode laser with a tapered amplifier is used to build the optical lattice with a magic-wavelength of 813.426 nm. Both waists of the counter-propagating lattice beam along the horizontal direction are overlapped to form a one-dimensional (1D) optical lattice. The lifetime of the atoms trapped in the 1D optical lattice is 1600 ms. The clock laser at 698 nm is a grating-feedback diode laser, which is locked to an ultra-low expansion cavity by the Pound-Drever-Hall technique to stabilize the frequency and phase. As a result, the linewidth of clock laser is narrowed to Hz level. By the normalized shelving method, we obtain a resolved sideband spectrum of 87Sr 5s2 1S05s5p 3P0 transition. According to the spectrum, the lattice temperature along the longitudinal direction is approximately 4.2 K. After that a linewidth of 6.7 Hz of the degenerate clock transition is obtained at a probing time of 150 ms by utilizing a three-dimensional (3D) bias magnetic field, which is used to eliminate the stray magnetic fields. Then a small bias magnetic field of 300 mGs is applied along the polarization axis of the lattice light to achieve the spectrum of Zeeman magnetic sublevels of the clock transition. Furthermore, the mF=+9/2 and mF=-9/2 magnetic sublevels are picked to be respectively pumped by the +-polarized and --polarized light at 689 nm, a variable liquid crystal wave plate is employed to switch on both polarizations. Finally, the spin polarized clock transition spectrum is obtained at the interrogating pulse of 150 ms, and the linewidths of the mF=+9/2, mF=-9/2 magnetic sublevel transitions are 6.8 Hz and 6.2 Hz respectively.
We present our experiment on magnetic field induced spectroscopy of the 1 S 0 − 3 P 0 transition of 88 Sr atoms with a 10 Hz linewidth laser. The 88 Sr atoms are cooled by two stage laser cooling. After the second stage narrow line laser cooling, the temperature of the atoms is reduced to ∼3 μK. The atoms are then loaded into an 813 nm one-dimensional optical lattice. A homemade 698 nm laser with 10 Hz linewidth and maximum intensity of more than 100 W/cm 2 is used to probe the 88 Sr atoms in the lattice. By means of a magnetic field of ∼1 mT and a probe laser with 50 ms pulse and ∼6 W/cm 2 intensity, the Doppler free 88 Sr 1 S 0 − 3 P 0 transition spectrum with a linewidth of 208 Hz is obtained.
We performed spectroscopic observations of the 698-nm clock transition in 87 Sr confined in an optical lattice using a laser linewidth transfer technique. A narrow-linewidth laser interrogating the clock transition was prepared by transferring the linewidth of a master laser (1064 nm) to that of a slave laser (698 nm) with a high-speed controllable fiber-based frequency comb. The Fourier-limited spectrum was then observed for an 80-ms interrogating pulse. We determined that the absolute frequency of the 5s 2 1 S 0 –5s5p 3 P 0 clock transition in 87 Sr is 429 228 004 229 872.0 (1.6) Hz referenced to the SI second.
The optical lattice clock with neutral atoms occupies an outstanding position in the research field of atomic clocks, demonstrating the great potential of its performance (like the uncertainty and the stability). At present, the optical lattice clock has realized a 10-18 level of its uncertainty. In this paper, we present the realization of loading bosonic atoms 88Sr (strontium, alkaline-earth metals) into a one-dimensional (1D) optical lattice in our laboratory. The optical lattice where the atoms are trapped can make the energy level shift, called Stark shift. But there is the special optical lattice operating at the “magic” wavelength for clock transitions (5s2) 1S0-(5s5p) 3P0, which can make the same Stark light-shift for both of them, indicating a zero light-shift relative to the clock. In our experiment, Sr atoms are cooled in a two-stage cooling and its temperature can be as low as 2 μK. Then these cold atoms are confined in the Lamb-Dicke region by the lattice laser output from an amplified diode laser operating at the “magic” wavelength, 813 nm. Experimentally, it is straightforward to provide 850 mW of lattice power focused to a 38 μm beam radius. After the cold atoms have trapped in the optical lattice, the lifetime of atoms in 1D optical lattice is measured to be 270 ms. The temperature and the number are about 3.5 μK and 1.2×105 respectively. Besides, effects of the power of the lattice laser on both the number and temperature are analyzed. The number changes linearly with the laser power, while there is no obvious influence on the temperature by the power. This original and special approach for atoms trapped in the optical lattice can provide a long interrogation time for probing the clock transition. Furthermore, it may be the foundation for developing our optical lattice clock of strontium atoms.
A clock laser based on a 30-cm-long ultrahigh finesse optical cavity was developed to improve the frequency stability of the Sr optical lattice clock at the National Institute of Metrology. Using this clock laser to probe the spin-polarized Sr87 atoms, a Rabi transition linewidth of 1.8 Hz was obtained with 500 ms interrogation time. Two independent digital servos are used to alternatively lock the clock laser to the S01 (mF=+9/2)→P03 (mF=+9/2) transition. The Allan deviation shows that the short-term frequency stability is better than 3.2×10−16 and averages down followed by 1.8×10−15/τ.
We present experimental results for an optical lattice clock operating on the1S0harr3P0transition in88Sr, which is excited with the technique of magnetic field-induced spectroscopy To reduce the complexity of the setup we have developed a set of new experimental techniques that greatly simplifies the clock spectroscopy in Sr atoms. First, we developed a method for finding the clock transition that removes the need for extensive frequency metrology hardware and optical frequency combs. This technique exploits a near coincidence in the atomic wavelengths of the1S0harr3P0clock and1S0harr3P1second stage cooling transitions in Sr, which are only 5 THz far apart. This coincidence enables the use of an optical (transfer) cavity to reference the frequency of the clock transition relative to that of the much stronger coolign transition Second, all laser sources in the experimental setup are based on semiconductor technology, which greatly reduces the complexity of the apparatus. With this setup, about 10488Sr atoms are trapped in a 1D lattice formed by 200 mW of radiation tuned near the magic wavelength at 813 nm. Preliminar uncertainty budget for our optical lattice clock is also presented, with particular attention to density dependent collisions, which led to an unexpectedly high signal contrast for long interaction times.