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arXiv:1401.1008 · Applied Physics Express

Spectroscopy and frequency measurement of the87Sr clock transition by laser linewidth transfer using an optical frequency comb

Daisuke Akamatsu, Hajime Inaba, Kazumoto Hosaka, Masami Yasuda, Atsushi Onae, Tomonari Suzuyama, Masaki Amemiya, Feng-Lei Hong

Published Dec 18, 2013• 50 citations
arXivHTMLPDF

Abstract

We performed spectroscopic observations of the 698-nm clock transition in 87 Sr confined in an optical lattice using a laser linewidth transfer technique. A narrow-linewidth laser interrogating the clock transition was prepared by transferring the linewidth of a master laser (1064 nm) to that of a slave laser (698 nm) with a high-speed controllable fiber-based frequency comb. The Fourier-limited spectrum was then observed for an 80-ms interrogating pulse. We determined that the absolute frequency of the 5s 2 1 S 0 –5s5p 3 P 0 clock transition in 87 Sr is 429 228 004 229 872.0 (1.6) Hz referenced to the SI second.

DOI
10.7567/apex.7.012401

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We performed spectroscopic observations of the 698-nm clock transition in 87 Sr confined in an optical lattice using a laser linewidth transfer technique. A narrow-linewidth laser interrogating the clock transition was prepared by transferring the linewidth of a master laser (1064 nm) to that of a slave laser (698 nm) with a high-speed controllable fiber-based frequency comb. The Fourier-limited spectrum was then observed for an 80-ms interrogating pulse. We determined that the absolute frequency of the 5s 2 1 S 0 –5s5p 3 P 0 clock transition in 87 Sr is 429 228 004 229 872.0 (1.6) Hz referenced to the SI second.
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The present decade has seen great advances in optical frequency standards following the development of femtosecond laser frequency combs. With this technology, combined with a stable and narrow probe laser source (50-100 Hz linewidth), we made a systematic study of the 5s 2S1/2-4d 2D5/2 (S-D) transition frequency of the 88Sr+ ion as a function of the quantization axis in the trap. This study revealed the presence of systematic shifts caused by residual micromotion in our rf Paul trap and led to an evaluation of those shifts. Also, a method was developed based on the measurement of the Zeeman spectrum of the clock transition to cancel the electric quadrupole shift caused by patch potentials on the trap electrodes. From these results, we also determined the absolute frequency of the S-D clock transition frequency at 674 nm with a fractional frequency uncertainty of 3.4 × 10-14. We have since made improvements to our probe laser system and have observed 5 Hz Fourier transform limited linewidths on a Zeeman component of the S-D transition of the 88Sr+ ion. To observe such a narrow transition it is essential to have a known and well behaved drift of the laser frequency during the few minutes it takes to measure the ion resonance using the quantum jump signal. Our approach to minimize the drift rate and its sensitivity to temperature fluctuations has been to stabilize the cavity at the temperature where its coefficient of thermal expansion is zero. We will present an overview of our recent progress made on the frequency standard based on the laser-cooled and trapped single ion of 88Sr+.
We report our observation of the spin polarized 1 S 0 → 3 P 0 clock transition spectrum in an optical lattice clock based on fermionic 87 Sr. The atoms are trapped and pre-cooled to about 2 μK with two stages of laser cooling at 461 nm and 689 nm, respectively. Then the atoms are loaded into an optical lattice formed by the interference of counter-propagating laser beams at 813 nm. An external cavity diode laser at 698 nm, which is stabilized to a high finesse cavity with a linewidth of about 5 Hz and a drift rate of less than 0.2 Hz/s, is used to excite the atoms to the 3 P 0 state. The π-polarized clock transition spectrum of resolvable m F states is obtained by applying a small bias magnetic field along the polarization axis of the probe beam. A spin polarized clock transition spectrum as narrow as 10 Hz with an 80 ms probe pulse is obtained.
Recent results from the JILA 87Sr optical lattice clock are presented. Using the tight confinement of an optical lattice in combination wit a sub-Hz linewidth diode laser we have achieved a pulse-length limited linewidth of 1.8 Hz for the 1S0- 3P0 clock transition. This corresponds to a quality factor of Q ≈ 2.4 x 1014, and is a record for coherent spectroscopy. With the addition of a small magnetic bias field, the high line Q of the clock transition has also allowed us to resolve the nuclear-spin sublevels, and make a precision measurement of the differential Landé g-factor between the 1S0 and 3P0. We present the current accuracy and stability of the lattice clock, and in addition, we report on our development of precision tools for the lattice clock, including a stabilized clock laser, fs-comb based technology allowing accurate clock comparison in both the microwave and optical domains, and clock transfer over an optical fiber in an urban environment.
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Laser frequency stabilization and atom manipulation are important techniques for optical frequency metrology. We report on the development of an ytterbium (171Yb) and a strontium (87Sr) optical lattice clock at the National Metrology Institute of Japan (NMIJ). The result of absolute frequency measurement of the171Yb lattice clock is shown. We also report on narrow-linewidth fiber-based frequency combs that are used not only to measure the absolute frequency of the optical lattice clocks but also to servo control the frequency of the lasers for cooling and trapping Yb and Sr atoms.