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Frontiers in Optics

Cavity Nonlinear Optics at Low Photon Numbers from Collective Atomic Motion

Subhadeep Gupta, Kevin L. Moore, Kater W. Murch, Dan Stamper-Kurn

Published Jan 1, 2007• 48 citations
Publisher

Abstract

We report on nonlinear optical phenomena from collective motion of ultracold atoms within a strong-coupling cavity. The nonlinearity arises from probe-induced atom displacement. Longevity of motional coherence allows nonlinearity at extremely low cavity photon numbers.
DOI
10.1364/fio.2007.pdp_c1

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We report on Kerr nonlinearity and dispersive optical bistability of a Fabry-Perot optical resonator due to the displacement of ultracold atoms trapped within. In the driven resonator, such collective motion is induced by optical forces acting upon up to 10(5) 87Rb atoms prepared in the lowest band of a one-dimensional intracavity optical lattice. The longevity of atomic motional coherence allows for strongly nonlinear optics at extremely low cavity photon numbers, as demonstrated by the observation of both branches of optical bistability at photon numbers below unity.
A common goal of recent research is the elucidation and control over quantum mechanical behavior in ever-larger physical systems. In this thesis I present an alternative target for investigating the quantum motion of macroscopic bodies: the collective motion of an ultracold atomic gas trapped within a high-finesse Fabry-Perot optical cavity in the single-atom strong-coupling regime of cavity quantum electrodynamics (CQED). When ultracold atoms are trapped in the Lamb-Dicke regime, the cavity-mode structure selects a single collective degree of freedom that is at once actuated by the optical forces from cavity probe light and measured by the cavity’s optical properties. Dispersive optical bistability arising from collective motion of the atomic medium was observed. Measurement of the collective motion was subject to quantum measurement backaction by the quantum force fluctuations of the cavity optical field. The strength and spectrum of these backaction force fluctuations was measured by quantifying the cavity-light-induced heating rate of the intracavity atomic ensemble, finding quantitative agreement with the expected heating rate from quantum optical fluctuations. Dynamical phenomena in the optomechanical system were explored experimentally and theoretically. Quantum limited measurements are discussed and were
We report on collective nonlinear dynamics in an optical lattice formed inside a high finesse ring cavity in a so far unexplored regime, where the light shift per photon times the number of trapped atoms exceeds the cavity resonance linewidth. We observe bistability and self-induced squeezing oscillations resulting from the retroaction of the atoms upon the optical potential wells. We can well understand most of our observations within a simplified model assuming adiabaticity of the atomic motion. Nonadiabatic aspects of the atomic motion are reproduced by solving the complete system of coupled nonlinear equations of motion.
The generation of correlated photons typically requires a highly nonlinear medium that is strongly coupled to an optical mode. Recently, significant advances have been made in this direction by strongly coupling photons to quantum emitters and exploiting the inherently nonlinear response of the latter. A number of methods have been pursued for this purpose, employing, e.g., high finesse optical cavities or strongly interacting Rydberg atoms. However, the implementation of strong and low-loss photon-photon interactions remains a challenging goal.
Abstract Single atoms coupled to a cavity offer unique opportunities as quantum optomechanical devices because of their small mass and strong interaction with light. A particular regime of interest in optomechanics is that of ‘single-photon strong coupling’, where motional displacements on the order of the zero-point uncertainty are sufficient to shift the cavity resonance frequency by more than its linewidth. In many cavity QED platforms, however, this is unfeasible due to the large cavity linewidth. Here, we propose an alternative route in such systems, which instead relies on the coupling of atomic motion to the much narrower cavity-dressed atomic resonance frequency. We discuss and optimize the conditions in which the scattering properties of single photons from the atom-cavity system become highly entangled with the atomic motional wave function. We also analyze the prominent observable features of this optomechanical strong coupling, which include a per-photon motional heating that is significantly larger than the single-photon recoil energy, as well as mechanically-induced oscillations in time of the second-order correlation function of the emitted light. This physics should be realizable in current experimental setups, such as trapped atoms coupled to photonic crystal cavities, and more broadly opens the door to realizing qualitatively different phenomena beyond what has been observed in optomechanical systems thus far.