We analyze exciting recent measurements [Phys. Rev. Lett. 114 (2015) 037202] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnet Cu(C4H4N2)(NO3)2 (CuPzN) subjected to strong magnetic fields. Using the mapping between magnons (bosons) in CuPzN and fermions, we demonstrate that magnetic field tunes the insulator towards quantum critical point related to so‐called fermion condensation quantum phase transition (FCQPT) at which the resulting fermion effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the (temperature—magnetic field) phase diagram, that contains Landau‐Fermi‐liquid, crossover and non‐Fermi liquid parts, thus resembling that of heavy‐fermion compounds.
We analyze exciting recent measurements [Phys. Rev. Lett. 114 (2015) 037202] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnet Cu(C4H4N2)(NO3)2 (CuPzN) subjected to strong magnetic fields. Using the mapping between magnons (bosons) in CuPzN and fermions, we demonstrate that magnetic field tunes the insulator towards quantum critical point related to so‐called fermion condensation quantum phase transition (FCQPT) at which the resulting fermion effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the (temperature—magnetic field) phase diagram, that contains Landau‐Fermi‐liquid, crossover and non‐Fermi liquid parts, thus resembling that of heavy‐fermion compounds.
Universal behavior of one-dimensional quantum spin liquid in the Cu(C4H4N2)(NO3)2 insulator
We analyze exciting recent measurements [Phys. Rev. Lett. 114, 037202 (2015)] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnetic insulator Cu(C4H4N2)(NO3)2 (CuPzN) subjected to strong magnetic fields. Our main finding is that the thermodynamic properties are defined by quantum spin liquid formed with spinons, while the magnetic field tunes the insulator towards quantum critical point related to so-called fermion condensation quantum phase transition (FCQPT) at which the spinon effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the T−H (temperature---magnetic field) phase diagram, that contains Landau-Fermi-liquid, crossover and non-Fermi liquid parts, thus resembling that of heavy-fermion compounds.
High-precision dc magnetization measurements have been made on Cu(C4H4N2) (NO3)2 in magnetic fields up to 14.7 T, slightly above the saturation field Hs=13.97 T, in the temperature range from 0.08 to 15 K. The magnetization curve and differential susceptibility at the lowest temperature show excellent agreement with exact theoretical results for the spin-1/2 Heisenberg antiferromagnet in one dimension. A broad peak is observed in magnetization measured as a function of temperature, signaling a crossover to a low-temperature Tomonaga-Luttinger-liquid regime. With an increasing field, the peak moves gradually to lower temperatures, compressing the regime, and, at Hs, the magnetization exhibits a strong upturn. This quantum critical behavior of the magnetization and that of the specific heat withstand quantitative tests against theory, demonstrating that the material is a practically perfect one-dimensional spin-1/2 Heisenberg antiferromagnet.
The behavior of Fermi systems that approach the fermion condensation quantum phase transition (FCQPT) from the disordered phase is considered. We show that the quasiparticle effective mass M * diverges as M * ∝ 1/¦ x − x FC ¦, where x is the system density and x FC is the critical point at which FCQPT occurs. Such behavior is of general form and takes place in both three-dimensional (3D) and two-dimensional (2D) systems. Since the effective mass M * is finite, the system exhibits the Landau Fermi liquid behavior. At ¦ x − x FC ¦/ x FC ≪1, the behavior can be viewed as highly correlated, because the effective mass is large and strongly depends on the density. In the case of electronic systems, the Wiedemann-Franz law is valid and the Kadowaki-Woods ratio is preserved. Beyond the region ¦ x – x FC ¦/ x FC ≪1, the effective mass is approximately constant and the system becomes a conventional Landau Fermi liquid.
The behavior of Fermi systems which approach the fermion condensation quantum phase transition (FCQPT) from the disordered phase is considered. We show that the quasiparticle effective mass M ∗ diverges as M ∗ ∝ 1/|x − xFC | where x is the system density and xFC is the critical point at which FCQPT occurs. Such a behavior is of general form and takes place in both three dimensional (3D) systems and two dimensional (2D) ones. Since the effective mass M ∗ is finite, the system exhibits the Landau Fermi liquid behavior. At |x −xFC|/xFC ≪ 1, the behavior can be viewed as a highly correlated one, because the effective mass is large and strongly depends on the density. In case of electronic systems the Wiedemann-Franz law is held and Kadowaki-Woods ratio is preserved. Beyond the region |x−xFC|/xFC ≪ 1, the effective mass is approximately constant and the system becomes conventional Landau Fermi liquid.
Strongly correlated Fermi systems are among the most intriguing, best experimentally studied and fundamental systems in physics. There is, however, lack of theoretical understanding in this field of physics. The ideas based on the concepts like Kondo lattice and involving quantum and thermal fluctuations at a quantum critical point have been used to explain the unusual physics. Alas, being suggested to describe one property, these approaches fail to explain the others. This means a real crisis in theory suggesting that there is a hidden fundamental law of nature. It turns out that the hidden fundamental law is well forgotten old one directly related to the Landau-Migdal quasiparticles, while the basic properties and the scaling behavior of the strongly correlated systems can be described within the framework of the fermion condensation quantum phase transition (FCQPT). The phase transition comprises the extended quasiparticle paradigm that allows us to explain the non-Fermi liquid (NFL) behavior observed in these systems. In contrast to the Landau paradigm stating that the quasiparticle effective mass is a constant, the effective mass of new quasiparticles strongly depends on temperature, magnetic field, pressure, and other parameters. Our observations are in good agreement with experimental facts and show that FCQPT is responsible for the observed NFL behavior and quasiparticles survive both high temperatures and high magnetic fields.
The quantum phase transition, scaling behaviors, and thermodynamics in the spin-1/2 quantum Heisenberg model with antiferromagnetic coupling J>0 in the armchair direction and ferromagnetic interaction J^{'}<0 in the zigzag direction on a honeycomb lattice are systematically studied using the continuous-time quantum Monte Carlo method. By calculating the Binder ratio Q_{2} and spin stiffness ρ in two directions for various coupling ratios α=J^{'}/J under different lattice sizes, we found that a quantum phase transition from the dimerized phase to the stripe phase occurs at the quantum critical point α_{c}=-0.93. Through the finite-size scaling analysis on Q_{2}, ρ_{x}, and ρ_{y}, we determined the critical exponent related to the correlation length ν to be 0.7212(8), implying that this transition falls into a classical Heisenberg O(3) universality. A zero magnetization plateau is observed in the dimerized phase, whose width decreases with increasing α. A phase diagram in the coupling ratio α-magnetic field h plane is obtained, where four phases, including dimerized, stripe, canted stripe, and polarized, are identified. It is also unveiled that the temperature dependence of the specific heat C(T) for different α's intersects precisely at one point, similar to that of liquid ^{3}He under different pressures and several magnetic compounds under various magnetic fields. The scaling behaviors of Q_{2}, ρ, and C(T) are carefully analyzed. The susceptibility is compared with the experimental data to give the magnetic parameters of both compounds.