Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review Letters

Field-Induced Quantum Criticality and Universal Temperature Dependence of the Magnetization of a Spin- 1/2 Heisenberg Chain

Yohei Kono, T. Sakakibara, Christopher Aoyama, Chisa Hotta, Mark M. Turnbull, C.P. Landee, Y. Takano

Published Jan 22, 2015• 70 citations
Publisher

Abstract

High-precision dc magnetization measurements have been made on Cu(C4H4N2) (NO3)2 in magnetic fields up to 14.7 T, slightly above the saturation field Hs=13.97 T, in the temperature range from 0.08 to 15 K. The magnetization curve and differential susceptibility at the lowest temperature show excellent agreement with exact theoretical results for the spin-1/2 Heisenberg antiferromagnet in one dimension. A broad peak is observed in magnetization measured as a function of temperature, signaling a crossover to a low-temperature Tomonaga-Luttinger-liquid regime. With an increasing field, the peak moves gradually to lower temperatures, compressing the regime, and, at Hs, the magnetization exhibits a strong upturn. This quantum critical behavior of the magnetization and that of the specific heat withstand quantitative tests against theory, demonstrating that the material is a practically perfect one-dimensional spin-1/2 Heisenberg antiferromagnet.

DOI
10.1103/physrevlett.114.037202

Related papers

Magnetization Study of the Quantum Critical Behavior of the One Dimensional Spin-1/2 Heisenberg Antiferromagnet CuPzN

Yohei Kono, Toshiro Sakakibara, Christopher Aoyama +3 more

High-precision DC magnetization (M) measurements have been performed on a single crystal of copper pyrazine dinitrate (CuPzN) in magnetic fields H up to 14.7 T at temperatures down to 0.08 K. This material is one of the best realizations of a one-dimensional (1D) S = 1/2 Heisenberg antiferromagnet. At the base temperature, full saturation of M is observed above Hs = 13.97 T with the M(H) curve closely following a prediction based on the Bethe ansatz. The peak in M(T ), which appears at about 7 K in zero field, moves to lower temperatures with increasing H and vanishes into a temperature region well below 0.08 K at H ∼ Hs; as a result, M(T ) exhibits a strong upturn as T → 0 at this field, in agreement with a theoretical prediction. These results constitute an observation of field-induced quantum critical behavior in bulk magnetization.

International Conference on Strongly Correlated Electron Systems (SCES)•Jun 16, 2014•1 citation

Magnetic quantum criticality in quasi‐one‐dimensional Heisenberg antiferromagnet

Vasily R. Shaginyan, V. A. Stephanovich, Konstantin G. Popov +2 more

We analyze exciting recent measurements [Phys. Rev. Lett. 114 (2015) 037202] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnet Cu(C4H4N2)(NO3)2 (CuPzN) subjected to strong magnetic fields. Using the mapping between magnons (bosons) in CuPzN and fermions, we demonstrate that magnetic field tunes the insulator towards quantum critical point related to so‐called fermion condensation quantum phase transition (FCQPT) at which the resulting fermion effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the (temperature—magnetic field) phase diagram, that contains Landau‐Fermi‐liquid, crossover and non‐Fermi liquid parts, thus resembling that of heavy‐fermion compounds.

Annalen der Physik•Mar 31, 2016•12 citations

Tomonaga–Luttinger liquid and quantum criticality in spin-12 antiferromagnetic Heisenberg chain C14H18CuN4O10 via Wilson ratio

Sharath Kumar Channarayappa, Sankalp Kumar, N. S. Vidhyadhiraja +9 more

Abstract The ground state of a one-dimensional spin-12 uniform antiferromagnetic Heisenberg chain (AfHc) is a Tomonaga–Luttinger liquid which is quantum-critical with respect to applied magnetic fields up to a saturation field μ0Hs beyond which it transforms to a fully polarized state. Wilson ratio has been predicted to be a good indicator for demarcating these phases [Phys. Rev. B 96, 220401 (2017)]. From detailed temperature and magnetic field-dependent magnetization, magnetic susceptibility and specific heat measurements in a metalorganic complex and comparisons with field theory and quantum transfer matrix method calculations, the complex was found to be a very good realization of a spin-12 AfHc. Wilson ratio obtained from experimentally obtained magnetic susceptibility and magnetic contribution of specific heat values was used to map the magnetic phase diagram of the uniform spin-12 AfHc over large regions of phase space demarcating Tomonaga–Luttinger liquid, saturation field quantum critical, and fully polarized states. Luttinger parameter and spinon velocity were found to match very well with the values predicted from conformal field theory.

arXiv:2408.11163•PNAS Nexus•Aug 23, 2024•6 citations

Universal behavior of one-dimensional quantum spin liquid in the $\rm {\bf Cu(C_4H_4N_2)(NO_3)_2}$ insulator

Vasily R. Shaginyan, V. A. Stephanovich, Konstantin G. Popov +1 more

We analyze exciting recent measurements [Phys. Rev. Lett. 114, 037202 (2015)] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnetic insulator Cu(C$_4$H$_4$N$_2$)(NO$_3$)$_2$ (CuPzN) subjected to strong magnetic fields. Our main finding is that the thermodynamic properties are defined by quantum spin liquid formed with spinons, while the magnetic field tunes the insulator towards quantum critical point related to so-called fermion condensation quantum phase transition (FCQPT) at which the spinon effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the $T-H$ (temperature---magnetic field) phase diagram, that contains Landau-Fermi-liquid, crossover and non-Fermi liquid parts, thus resembling that of heavy-fermion compounds.

•Oct 27, 2015•0 citations

Tomonaga–Luttinger Liquid in Quasi-One-Dimensional Antiferromagnet BaCo2V2O8in Magnetic Fields

Seiichiro Suga

Motivated by recent studies on the quasi-one-dimensional (1D) antiferromagnet BaCo2V2O8, we investigate the Tomonaga-Luttinger-liquid properties of the 1D S=1/2 XXZ Heisenberg-Ising model in magnetic fields. By using the Bethe ansatz solution, thermodynamic quantities and the divergence exponent of the NMR relaxation rate are calculated. We observe a magnetization minimum as a function of temperature (T) close to the critical field. As the magnetic field approaches the critical field, the minimum temperature asymptotically approaches the universal relation in agreement with the recent results by Maeda et al. in Phys. Rev. Lett. 99 (2007) 057205. We observe T-linear specific heat below the temperature of the magnetization minimum. The field dependence of its coefficient agrees with the results based on conformal field theory. The field dependence of the divergence exponent of the NMR relaxation rate with decreasing temperature is obtained, indicating a change in the critical properties. The results are discussed in connection with experiments on BaCo2V2O8.

arXiv:0805.2971•Journal of the Physical Society of Japan•Jul 10, 2008•14 citations

Phase diagram and quantum criticality of Heisenberg spin chains with Ising anisotropic interchain couplings

Yuchen Fan, Jiahao Yang, Weiqiang Yu +2 more

The authors find that the interchain Ising anisotropy of coupled spin-1/2 Heisenberg chains enhances longitudinal spin correlations and stabilizes an incommensurate antiferromagnetic order under a longitudinal magnetic field. The system shows a dimensional crossover in the quantum critical regime and exhibits Tomonaga-Luttinger liquid behavior over a broad field and temperature regime.

arXiv:1908.08467•Physical Review Research•Mar 19, 2020•19 citations
High-precision dc magnetization measurements have been made on Cu(C4H4N2) (NO3)2 in magnetic fields up to 14.7 T, slightly above the saturation field Hs=13.97 T, in the temperature range from 0.08 to 15 K. The magnetization curve and differential susceptibility at the lowest temperature show excellent agreement with exact theoretical results for the spin-1/2 Heisenberg antiferromagnet in one dimension. A broad peak is observed in magnetization measured as a function of temperature, signaling a crossover to a low-temperature Tomonaga-Luttinger-liquid regime. With an increasing field, the peak moves gradually to lower temperatures, compressing the regime, and, at Hs, the magnetization exhibits a strong upturn. This quantum critical behavior of the magnetization and that of the specific heat withstand quantitative tests against theory, demonstrating that the material is a practically perfect one-dimensional spin-1/2 Heisenberg antiferromagnet.
High-precision DC magnetization (M) measurements have been performed on a single crystal of copper pyrazine dinitrate (CuPzN) in magnetic fields H up to 14.7 T at temperatures down to 0.08 K. This material is one of the best realizations of a one-dimensional (1D) S = 1/2 Heisenberg antiferromagnet. At the base temperature, full saturation of M is observed above Hs = 13.97 T with the M(H) curve closely following a prediction based on the Bethe ansatz. The peak in M(T ), which appears at about 7 K in zero field, moves to lower temperatures with increasing H and vanishes into a temperature region well below 0.08 K at H ∼ Hs; as a result, M(T ) exhibits a strong upturn as T → 0 at this field, in agreement with a theoretical prediction. These results constitute an observation of field-induced quantum critical behavior in bulk magnetization.
We analyze exciting recent measurements [Phys. Rev. Lett. 114 (2015) 037202] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnet Cu(C4H4N2)(NO3)2 (CuPzN) subjected to strong magnetic fields. Using the mapping between magnons (bosons) in CuPzN and fermions, we demonstrate that magnetic field tunes the insulator towards quantum critical point related to so‐called fermion condensation quantum phase transition (FCQPT) at which the resulting fermion effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the (temperature—magnetic field) phase diagram, that contains Landau‐Fermi‐liquid, crossover and non‐Fermi liquid parts, thus resembling that of heavy‐fermion compounds.
Abstract The ground state of a one-dimensional spin-12 uniform antiferromagnetic Heisenberg chain (AfHc) is a Tomonaga–Luttinger liquid which is quantum-critical with respect to applied magnetic fields up to a saturation field μ0Hs beyond which it transforms to a fully polarized state. Wilson ratio has been predicted to be a good indicator for demarcating these phases [Phys. Rev. B 96, 220401 (2017)]. From detailed temperature and magnetic field-dependent magnetization, magnetic susceptibility and specific heat measurements in a metalorganic complex and comparisons with field theory and quantum transfer matrix method calculations, the complex was found to be a very good realization of a spin-12 AfHc. Wilson ratio obtained from experimentally obtained magnetic susceptibility and magnetic contribution of specific heat values was used to map the magnetic phase diagram of the uniform spin-12 AfHc over large regions of phase space demarcating Tomonaga–Luttinger liquid, saturation field quantum critical, and fully polarized states. Luttinger parameter and spinon velocity were found to match very well with the values predicted from conformal field theory.
Universal behavior of one-dimensional quantum spin liquid in the Cu(C4H4N2)(NO3)2\rm {\bf Cu(C_4H_4N_2)(NO_3)_2}Cu(C4​H4​N2​)(NO3​)2​ insulator
We analyze exciting recent measurements [Phys. Rev. Lett. 114, 037202 (2015)] of the magnetization, differential susceptibility and specific heat on one dimensional Heisenberg antiferromagnetic insulator Cu(C4_44​H4_44​N2_22​)(NO3_33​)2_22​ (CuPzN) subjected to strong magnetic fields. Our main finding is that the thermodynamic properties are defined by quantum spin liquid formed with spinons, while the magnetic field tunes the insulator towards quantum critical point related to so-called fermion condensation quantum phase transition (FCQPT) at which the spinon effective mass diverges kinematically. We show that the FCQPT concept permits to reveal the scaling behavior of thermodynamic characteristics, describe the experimental results quantitatively, and derive for the first time the T−HT-HT−H (temperature---magnetic field) phase diagram, that contains Landau-Fermi-liquid, crossover and non-Fermi liquid parts, thus resembling that of heavy-fermion compounds.
Motivated by recent studies on the quasi-one-dimensional (1D) antiferromagnet BaCo2V2O8, we investigate the Tomonaga-Luttinger-liquid properties of the 1D S=1/2 XXZ Heisenberg-Ising model in magnetic fields. By using the Bethe ansatz solution, thermodynamic quantities and the divergence exponent of the NMR relaxation rate are calculated. We observe a magnetization minimum as a function of temperature (T) close to the critical field. As the magnetic field approaches the critical field, the minimum temperature asymptotically approaches the universal relation in agreement with the recent results by Maeda et al. in Phys. Rev. Lett. 99 (2007) 057205. We observe T-linear specific heat below the temperature of the magnetization minimum. The field dependence of its coefficient agrees with the results based on conformal field theory. The field dependence of the divergence exponent of the NMR relaxation rate with decreasing temperature is obtained, indicating a change in the critical properties. The results are discussed in connection with experiments on BaCo2V2O8.