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Frontiers in Optics

Second Harmonic Generation Inside Microcavities: On the Existence of a Threshold

Serge Gauvin, Marc Collette, Normand Beaudoin

Published Jan 1, 2014• 2 citations
Publisher

Abstract

The anomalous commutation relation [Ueda, M. and Imoto, N., "Anomalous commutation relation and modified spontaneous emission inside a microcavity," Phys. Rev. A, 50(1), 89-92 (1994)] is used to demonstrate the existence of a threshold for second harmonic generation when it occurs from inside microcavities. This is an unexpected result.

DOI
10.1364/fio.2014.jtu3a.29

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The anomalous commutation relation [Ueda, M. and Imoto, N., "Anomalous commutation relation and modified spontaneous emission inside a microcavity," Phys. Rev. A, 50(1), 89-92 (1994)] is used to demonstrate the existence of a threshold for second harmonic generation when it occurs from inside microcavities. This is an unexpected result.
The interest toward strong electromagnetic confinement structures through the use of microcavities is of great interest, from both the fundamental understanding and the technological application sides. Here, we focus our attention to second order nonlinear processes inside such structures. From a basic point of view, electromagnetic confinement leads, physically, to the manipulation of vacuum field fluctuations and, formally, to an anomalous commutation relation [Ueda, M. and Imoto, N., "Anomalous commutation relation and modified spontanenous emission inside a microcavity," Phys. Rev. A, 50(1), 89-92 (1994)]. However, an attempt to probe the resulting anomaly with a beam splitter located inside a cavity is theoretically proved inadequate for this task. For this reason, parametric fluorescence (PF, parametric down conversion) and second harmonic generation (SHG) are considered as potential tools to probe vacuum field fluctuations in confinement structures. Indeed, it was recently showed that PF can be strongly intensified, by two orders of magnitude or more, when it occurs inside a high confinement (open) cavity. Therefore, PF could efficiently be used to probe the expected anomaly. Additionally, in consideration of the simplest possible experimental scheme to probe the anomaly and because it is generally admitted that SHG is the time reversal of degenerate parametric fluorescence, here our attention is also directed toward SHG. Formally, we show that the equations describing SHG and PF are not symmetrical regarding quantum noise. It turns out that, conversely to the case of PF, the intensification of vacuum field fluctuations tends to inhibit SHG. We interpret this result as due to the reduction of waves coherence induced by stronger quantum noise. In conclusion, albeit both processes could be used as probes to prove or disprove the realm of quantum anomalies, PF appears as a more convenient tool.
We present a quantum theory to derive the analytical expression of microcavity enhancement for second harmonic generation. The expression explicitly gives the dependence of the enhancement on detunings and the Purcell factor of the relevant microcavity mode, and it is suitable for microcavities with any dimensions and arbitrary geometric shapes. The result for a one-dimensional microcavity agrees well with a recent microcavity-enhanced second harmonic generation experiment by Cao et al (2000 Appl. Phys. Lett. 76 538).
A formula describing the intensity of spontaneous emission outside a planar microcavity is derived quantum mechanically. It reflects the quantum mechanical interference of the atom and the emitted photon via multiple reflections in the cavity. The expression derived for the power spectrum reproduces the results of the classical theory by Huang et al.. [Appl. Phys. Lett. 61 (1992) 2961]. The quantum mechanical expression for the electric field amplitude for a single emission event is given together with its evolution equation.