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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Second order optical nonlinear processes as tools to probe anomalies inside high confinement microcavities

Marc Collette, Normand Beaudoin, Serge Gauvin

Published May 8, 2013• 5 citations
Publisher

Abstract

The interest toward strong electromagnetic confinement structures through the use of microcavities is of great interest, from both the fundamental understanding and the technological application sides. Here, we focus our attention to second order nonlinear processes inside such structures. From a basic point of view, electromagnetic confinement leads, physically, to the manipulation of vacuum field fluctuations and, formally, to an anomalous commutation relation [Ueda, M. and Imoto, N., "Anomalous commutation relation and modified spontanenous emission inside a microcavity," Phys. Rev. A, 50(1), 89-92 (1994)]. However, an attempt to probe the resulting anomaly with a beam splitter located inside a cavity is theoretically proved inadequate for this task. For this reason, parametric fluorescence (PF, parametric down conversion) and second harmonic generation (SHG) are considered as potential tools to probe vacuum field fluctuations in confinement structures. Indeed, it was recently showed that PF can be strongly intensified, by two orders of magnitude or more, when it occurs inside a high confinement (open) cavity. Therefore, PF could efficiently be used to probe the expected anomaly. Additionally, in consideration of the simplest possible experimental scheme to probe the anomaly and because it is generally admitted that SHG is the time reversal of degenerate parametric fluorescence, here our attention is also directed toward SHG. Formally, we show that the equations describing SHG and PF are not symmetrical regarding quantum noise. It turns out that, conversely to the case of PF, the intensification of vacuum field fluctuations tends to inhibit SHG. We interpret this result as due to the reduction of waves coherence induced by stronger quantum noise. In conclusion, albeit both processes could be used as probes to prove or disprove the realm of quantum anomalies, PF appears as a more convenient tool.

DOI
10.1117/12.2017587

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The interest toward strong electromagnetic confinement structures through the use of microcavities is of great interest, from both the fundamental understanding and the technological application sides. Here, we focus our attention to second order nonlinear processes inside such structures. From a basic point of view, electromagnetic confinement leads, physically, to the manipulation of vacuum field fluctuations and, formally, to an anomalous commutation relation [Ueda, M. and Imoto, N., "Anomalous commutation relation and modified spontanenous emission inside a microcavity," Phys. Rev. A, 50(1), 89-92 (1994)]. However, an attempt to probe the resulting anomaly with a beam splitter located inside a cavity is theoretically proved inadequate for this task. For this reason, parametric fluorescence (PF, parametric down conversion) and second harmonic generation (SHG) are considered as potential tools to probe vacuum field fluctuations in confinement structures. Indeed, it was recently showed that PF can be strongly intensified, by two orders of magnitude or more, when it occurs inside a high confinement (open) cavity. Therefore, PF could efficiently be used to probe the expected anomaly. Additionally, in consideration of the simplest possible experimental scheme to probe the anomaly and because it is generally admitted that SHG is the time reversal of degenerate parametric fluorescence, here our attention is also directed toward SHG. Formally, we show that the equations describing SHG and PF are not symmetrical regarding quantum noise. It turns out that, conversely to the case of PF, the intensification of vacuum field fluctuations tends to inhibit SHG. We interpret this result as due to the reduction of waves coherence induced by stronger quantum noise. In conclusion, albeit both processes could be used as probes to prove or disprove the realm of quantum anomalies, PF appears as a more convenient tool.
It has been previously shown [Phys. Rev. A50, 89 (1994)PLRAAN1050-294710.1103/PhysRevA.50.89] that cavity-based electromagnetic confinement leads to an “anomalous” fields operators commutation relation that is undetectable by probing the cavity with a beam splitter. However, using this commutator in the case of parametric fluorescence (spontaneous parametric down conversion) when it occurs inside an open cavity implies a strong intensification of this process. This prediction can validate, or not, this commutation relation. The ab initio approach used is based entirely on vacuum field fluctuations and does not resort to the concept of density of states. Finally, through a generalization of creation and annihilation operators in the presence of noise, this approach raises fundamental questions about quantum modes. We expect this work to stimulate new theoretical developments and related experiments, which might lead to new applications in quantum nonlinear optics.
This work presents a quantum theory of the nonlinear optical process of second-harmonic generation (SHG) in one-dimensional microresonators. More specifically, we show how the manipulation of vacuum field fluctuations in high-confinement systems, leading to a spectrally (and spatially) modulated commutation relation for the photon's generalized formulations of their creation and annihilation operators, deeply affects SHG behavior and gives rise to a threshold level. The two main effects the modulated commutator has on this optical process are an inhibition of the SHG process at low pumping level and a significant (cubic) amplification of the second-harmonic signal production rate once the threshold is overcome (finally reaching the usual quadratic dependence at sufficiently high pumping level). Our predictions, which represent a concrete picture of a fractional quantum system, could be used to probe vacuum field fluctuations present in high-confinement microresonators and emphasize the fundamental importance of vacuum field fluctuations.
In this work we develop a quantum theory of second-order nonlinear optical processes such as parametric fluorescence and second-harmonic generation (SHG), generated by a strong electromagnetic field in an active medium placed in a microcavity. Fields are quantized and expanded in terms of a suitable set of cavity normal modes. In the first part of this work we consider a single many-level quantum system (an atom or molecule), which interacts with all the radiation field modes (spontaneous emission). We show how vacuum fluctuations affect both SHG and parametric processes. For SHG, we demonstrate that the presence of the microcavity allows the introduction of the concept of coherence length, even for a medium made of a single molecule. In the second part of this paper we discuss the case of a uniform distribution of emitting dipoles. For this configuration we calculate the differential extinction coefficient, and discuss the dependence of the emitting power on the microcavity's parameters. Finally we suggest the possibility of realizing a micro-optical parametric oscillator.
We analyze the quantum-fluctuation properties of second-harmonic radiation generated in the high-efficiency conversion process used in a recent experiment by Hakuta, Marmet, and Stoicheff [Phys. Rev. Lett. 66, 596 (1991)]. We extend their work by studying the second-harmonic generation inside an optical cavity. The active medium inside the cavity is modeled by three-level atoms with degenerated upper levels (1s, 2p, and 2s states of atomic hydrogen) interacting with a strong constant electric field. An enhancement of the conversion efficiency and a reduction of the added noise are found as a result of an electromagnetically induced transparency. We show that the scheme is capable of producing light in a squeezed or coherent state close to a minimum-uncertainty state with a large mean amplitude.
Long ago, it was predicted that stimulating two-photon processes such as two-photon absorption (TPA) and second harmonic generation (SHG) with entangled photons produced by parametric down-conversion (PDC) could result in higher efficiencies compared to classical illumination [1]. This was experimentally demonstrated for SHG [2] and TPA [3], where, however, the classical comparison was performed by adding losses to the PDC state rather than employing a true classical reference. In addition, these results considered spatially single-mode PDC radiation and were conducted at low photon fluxes, where the PDC modes are, on average, populated by less than one photon. This resulted in an extremely low SHG/TPA signal, considered of limited practical use for metrological applications (such as two-photon fluorescence microscopy or SHG imaging - see, e.g., [4]). A recent theoretical investigation [5] highlighted that a proper analysis of quantum-enhanced two-photon processes requires a fully spatiotemporal model of the nonlinear interactions. It further showed that highly multimode (in space and time) entangled PDC photons can provide a quantum advantage compared to an equivalent classical pulse, even in regimes well beyond the “one-photon-per-mode” limit, considered the boundary of quantum behavior.