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Applied Optics

Far off-resonance laser frequency stabilization using multipass cells in Faraday rotation spectroscopy

Wei Quan, Yang Li, Rujie Li, Huining Shang, Zishan Fang, Jie Qin, Shuangai Wan

Published Mar 22, 2016• 15 citations
Publisher

Abstract

We propose a far off-resonance laser frequency stabilization method by using multipass cells in Rb Faraday rotation spectroscopy. Based on the detuning equation, if multipass cells with several meters optical path length are used in the conventional Faraday spectroscopy, the detuning of the lock point can be extended much further from the alkali metal resonance. A plate beam splitter was used to generate two different Faraday signals at the same time. The transmitted optical path length was L=50 mm and the reflected optical path length was 2L=100 mm. When the optical path length doubled, the detuning of the lock points moved further away from the atomic resonance. The temperature dependence of the detuning of the lock point was also analyzed. A temperature-insensitive lock point was found near resonance when the cell temperature was between 110°C and 130°C. We achieved an rms fluctuation of 0.9 MHz/23 h at a detuning of 0.5 GHz. A frequency drift of 16 MHz/h at a detuning of -5.6 GHz and 4 MHz/h at a detuning of -5.2 GHz were also obtained for the transmitted and reflected light Faraday signal.

DOI
10.1364/ao.55.002503

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We propose a far off-resonance laser frequency stabilization method by using multipass cells in Rb Faraday rotation spectroscopy. Based on the detuning equation, if multipass cells with several meters optical path length are used in the conventional Faraday spectroscopy, the detuning of the lock point can be extended much further from the alkali metal resonance. A plate beam splitter was used to generate two different Faraday signals at the same time. The transmitted optical path length was L=50 mm and the reflected optical path length was 2L=100 mm. When the optical path length doubled, the detuning of the lock points moved further away from the atomic resonance. The temperature dependence of the detuning of the lock point was also analyzed. A temperature-insensitive lock point was found near resonance when the cell temperature was between 110°C and 130°C. We achieved an rms fluctuation of 0.9 MHz/23 h at a detuning of 0.5 GHz. A frequency drift of 16 MHz/h at a detuning of -5.6 GHz and 4 MHz/h at a detuning of -5.2 GHz were also obtained for the transmitted and reflected light Faraday signal.
We propose a far off-resonance laser frequency stabilization method that can accurately adjust the frequency lock points based on the Faraday rotation spectroscopy. The atomic magnetometer based on the spin-exchange relaxation-free (SERF) theory needs to stabilize the frequency of the probe laser on the detuning of several gigahertz (GHz) away from the resonance of the alkali metal atom, to reduce the absorption of the probe light by the alkali metal vapor cell. We propose a laser frequency stabilization method that can accurately adjust the frequency lock points using an acousto-optic modulator based on Faraday rotation spectroscopy. We reveal the principles of the method and simulate the new Faraday rotation spectra. Besides, we study the effect of the amount of frequency shift of the acousto - optic modulator and the temperature of the alkali metal vapor cell on the frequency lock points of the spectra, and give the formula for calculating the frequency point. Our proposed laser frequency stabilization method can stabilize the laser frequency on the detuning of several gigahertz (GHz) away from the resonance of the alkali metal atom and can adjust the frequency lock points quickly and accurately. This method can be used in atomic magnetometer, degenerate Raman sideband cooling (DRSC) and two photon excitation of Rydberg states.
We present a simple technique for stabilization of a laser frequency off resonance using the Faraday effect in a heated vapor cell with an applied magnetic field. In particular, we demonstrate stabilization of a 780 nm laser detuned up to 14 GHz from the (85)Rb D(2) 5(2)S(1/2) F = 2 to 5(2)P(3/2) F' = 3 transition. Control of the temperature of the vapor cell and the magnitude of the applied magnetic field allows locking ~6-14 GHz red and blue detuned from the atomic line. We obtain an rms fluctuation of 7 MHz over 1 h without stabilization of the cell temperature or magnetic field.
Abstract Locking laser frequencies to Doppler-free spectra produced by the interaction of light with alkali atoms in a vapor cell is a promising approach for realizing compact atomic optical frequency reference. In this work, we employ counter-propagating monochromatic laser beams with a polarization angle of 45° to interact with 87 Rb atoms in a 3 mm cubic vapor cell, inducing coherent resonance. By detecting the laser polarization rotation, we obtain a Doppler free spectral line, which is used as a reference for laser frequency locking, thus realizing an optical reference. We build two nominally identical systems and measure their beatnote, yielding a fractional frequency stability of 5.3×10 -13 at 1 s. This study demonstrates that the proposed scheme is a competitive approach for realizing high performance compact atomic optical reference.
We present a method of diode laser frequency stabilization based on the Faraday rotation of linearly polarized light passing through an atomic sample in the presence of a very modest (1mT) magnetic field. Near the zero crossing of this spectroscopic feature, an optical system capable of very precise polarimetry detects and corrects for very small frequency fluctuations via a feedback system, which keeps the rotation signal at zero. In our application, we have demonstrated robust frequency stabilization over time scales from 10ms to 1h at the 1MHz level or below. We utilize this technique to lock our laser to a “forbidden” M1∕E2 transition in thallium at 1283nm, for which saturated absorption techniques are not straightforward. This technique has broad applicability to spectroscopy of various atomic systems as we also demonstrate using a Rb cell and a 780nm diode laser.
In atomic physics experiments, a frequency-stabilized or ‘locked’ laser source is commonly required. Many established techniques are available for locking close to an atomic resonance. However, in many instances, such as atomic magnetometer and magic wavelength optical lattices in ultra-cold atoms, it is desirable to lock the frequency of the laser far away from the resonance. This review presents several far off-resonance laser frequency stabilization methods, by which the frequency of the probe beam can be locked on the detuning as far as several tens of gigahertz (GHz) away from atomic resonance line, and discusses existing challenges and possible future directions in this field.
The frequency drifts of the probe laser could be coupled into the calibrated scale factor of the optically pumped magnetometer (OPM) and induce an error of the measurement accuracy. We propose a method to reduce the far off-resonance laser frequency drifts based on the second harmonic of the electro-optic modulator (EOM) detection system in the all-optical K-Rb hybrid pumping magnetometer. Adopting the closed-loop feedback by monitoring the second-harmonic component in real time, the frequency drift of the probe laser has been effectively reduced by about five times to ∼30 MHz/0.5 h at the detuning of 130 GHz and the cell temperature of 443 K. Besides, this technique has been demonstrated to be helpful for reducing the frequency drifts at different detuning points and temperatures. This method is not only suitable for the development of more compact, high-sensitivity OPMs due to the long-term stability improvement with no extra optical path, but also can be applied to other atomic devices and EOM detection systems for reducing the influence of the laser.