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Physical Review Letters

Photoionization of He(n$sup 1$ $sup 3$P) atoms excited by polarized light

V. L. Jacobs

Published Jun 24, 1974• 0 citations
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Photoionization of He(nsup1sup 1sup1 sup3sup 3sup3P) atoms excited by polarized light
We study time delay in atomic photoionization by circularly polarized light. By considering the Li atom in an excited 2p2p2p state, we demonstrate a strong time-delay asymmetry between the photoemission of the target electrons that are co- and counter-rotating with the electromagnetic field in the polarization plane. In addition, we observe the time-delay sensitivity to the polar angle of the photoelectron emission in the polarization plane. This modulation depends on the shape and duration of the electromagnetic pulse.
The photoionization cross sections of two even-parity excited states 5d6d3D15d6d\phantom{\rule{0.3em}{0ex}}^{3}D_{1}5d6d3D1​ and 6s7d3D26s7d\phantom{\rule{0.3em}{0ex}}^{3}D_{2}6s7d3D2​ of atomic Ba at the ionization-laser wavelength of 556.6nm556.6\phantom{\rule{0.3em}{0ex}}\mathrm{nm}556.6nm were measured. We found that the total cross section depends on the relative polarization of the atoms and the ionization-laser light. With density-matrix algebra, we show that, in general, there are at most three parameters in the photoionization cross section. Some of these parameters are determined in this work. We also present the measurement of the radiative lifetime of five even-parity excited states of barium.