In this thesis, we study three cases of insulating states of matter in terms of the renormalization procedure where the conventional renormalization group scheme is not simply applicable. The first subject is the spectral weight structure of hole-doped Mott insulators. As the mixing between two separate Hubbard bands is dynamically generated, additional charge degrees of freedom is required to give a proper description to the relevant low-energy physics. On this account, we first discuss how the low-energy Hubbard band should be partitioned to account for the extra degrees of freedom. Following the exact integration procedure of the upper Hubbard band, we explicitly demonstrate that the conserved charge cannot be exhausted by counting quasiparticles. In addition, we argue that it is the existence of dynamically generated charge degrees of freedom that gives rise to the coexistence of poles and zeroes in the single-particle Green function. In comparison to the Fermi arc structure, which is intrinsic to cuperate phenomenology, we suggest that the suppression of the spectral weight at the back side of the arc is a consequence of composite excitations, arising from dynamical mixing. The second topic we study is the nature of the transition between two insulating states of matter in a weakly disordered bosonic system. In particular, we investigate the instabilities of the Mott-insulating phase within a renormalization group analysis of the replica field theory obtained by a strong-coupling expansion around the atomic limit. To this end, we identify a new order parameter and associated correlation length scale that are capable of capturing the transition from a state with zero compressibility, the Mott insulator, to another insulating state with finite compressibility, the Bose glass. The order parameter is the relative variance of the disorder-induced mass distribution. From its distinctive behavior on each phase, we find that the divergence of the relative variance in the Bose glass signals the breakdown of self-averaging. Lastly, we also emphasize that the transition at commensurate filling is governed by a different fixed point in the renormalization group flow. The last topic discussed is the thermoelectric properties of the correlated Kondo lattice system at low temperature. Specifically, we explore the periodic Anderson impurity model with spin-orbit interactions, using the slave-particle method. As the thermopower is related to the entropy per carrier, particle-hole asymmetry and a large density of states at the chemical potential make Kondo insulator an ideal platform for thermoelectrics. In this respect, we further explore the possibility to improve the thermoelectric performance by tuning the crystal electric field splitting, the spin-orbit interaction strength, and orbital degeneracy.
In this thesis, we study three cases of insulating states of matter in terms of the renormalization procedure where the conventional renormalization group scheme is not simply applicable. The first subject is the spectral weight structure of hole-doped Mott insulators. As the mixing between two separate Hubbard bands is dynamically generated, additional charge degrees of freedom is required to give a proper description to the relevant low-energy physics. On this account, we first discuss how the low-energy Hubbard band should be partitioned to account for the extra degrees of freedom. Following the exact integration procedure of the upper Hubbard band, we explicitly demonstrate that the conserved charge cannot be exhausted by counting quasiparticles. In addition, we argue that it is the existence of dynamically generated charge degrees of freedom that gives rise to the coexistence of poles and zeroes in the single-particle Green function. In comparison to the Fermi arc structure, which is intrinsic to cuperate phenomenology, we suggest that the suppression of the spectral weight at the back side of the arc is a consequence of composite excitations, arising from dynamical mixing. The second topic we study is the nature of the transition between two insulating states of matter in a weakly disordered bosonic system. In particular, we investigate the instabilities of the Mott-insulating phase within a renormalization group analysis of the replica field theory obtained by a strong-coupling expansion around the atomic limit. To this end, we identify a new order parameter and associated correlation length scale that are capable of capturing the transition from a state with zero compressibility, the Mott insulator, to another insulating state with finite compressibility, the Bose glass. The order parameter is the relative variance of the disorder-induced mass distribution. From its distinctive behavior on each phase, we find that the divergence of the relative variance in the Bose glass signals the breakdown of self-averaging. Lastly, we also emphasize that the transition at commensurate filling is governed by a different fixed point in the renormalization group flow. The last topic discussed is the thermoelectric properties of the correlated Kondo lattice system at low temperature. Specifically, we explore the periodic Anderson impurity model with spin-orbit interactions, using the slave-particle method. As the thermopower is related to the entropy per carrier, particle-hole asymmetry and a large density of states at the chemical potential make Kondo insulator an ideal platform for thermoelectrics. In this respect, we further explore the possibility to improve the thermoelectric performance by tuning the crystal electric field splitting, the spin-orbit interaction strength, and orbital degeneracy.
We investigate the instabilities of the Mott-insulating phase of the weakly disordered Bose-Hubbard model within a renormalization group analysis of the replica field theory obtained by a strong-coupling expansion around the atomic limit. We identify an order parameter and associated correlation length scale that are capable of capturing the transition from a state with zero compressibility, the Mott insulator, to one in which the compressibility is finite, the Bose glass. The order parameter is the relative variance of the disorder-induced mass distribution. In the Mott insulator, the relative variance renormalizes to zero, whereas it diverges in the Bose glass. The divergence of the relative variance signals the breakdown of self-averaging. The length scale governing the breakdown of self-averaging is the distance between rare regions. This length scale is finite in the Bose glass but diverges at the transition to the Mott insulator with an exponent of $\ensuremath{\nu}=1/D$ for incommensurate fillings. Likewise, the compressibility vanishes with an exponent of $\ensuremath{\gamma}=4/D\ensuremath{-}1$ at the transition. At commensurate fillings, the transition is controlled by a different fixed point at which both the disorder and interaction vertices are relevant.
The phase diagrams and phase transitions of bosons with short-ranged repulsive interactions moving in periodic and/or random external potentials at zero temperature are investigated with emphasis on the superfluid-insulator transition induced by varying a parameter such as the density. Bosons in periodic potentials (e.g., on a lattice) at T=0 exhibit two types of phases: a superfluid phase and Mott insulating phases characterized by integer (or commensurate) boson densities, by the existence of a gap for particle-hole excitations, and by zero compressibility. Generically, the superfluid onset transition in d dimensions from a Mott insulator to superfluidity is ``ideal,'' or mean field in character, but at special multicritical points with particle-hole symmetry it is in the universality class of the (d+1)-dimensional XY model. In the presence of disorder, a third, ``Bose glass'' phase exists. This phase is insulating because of the localization effects of the randomness and analogous to the Fermi glass phase of interacting fermions in a strongly disordered potential.The Bose glass phase is characterized by a finite compressibility, no gap, but an infinite superfluid susceptibility. In the presence of disorder the transition to superfluidity is argued to occur only from the Bose glass phase, and never directly from the Mott insulator. This zero-temperature superfluid-insulator transition is studied via generalizations of the Josephson scaling relation for the superfluid density at the ordinary \ensuremath{\lambda} transition, highlighting the crucial role of quantum fluctuations. The transition is found to have a dynamic critical exponent z exactly equal to d and correlation length and order-parameter correlation exponents \ensuremath{\nu} and \ensuremath{\eta} which satisfy the bounds \ensuremath{\nu}\ensuremath{\ge}2/d and \ensuremath{\eta}\ensuremath{\le}2-d, respectively. It is argued that the superfluid-insulator transition in the presence of disorder may have an upper critical dimension dc which is infinite, but a perturbative renormalization-group calculation wherein the critical exponents have mean-field values for weak disorder above d=4 is also discussed. Many of these conclusions are verified by explicit calculations on a model of one-dimensional bosons in the presence of both random and periodic potentials. The general results are applied to experiments on 4He absorbed in porous media such as Vycor. Some measurable properties of the superfluid onset are predicted exactly [e.g., the exponent x relating the \ensuremath{\lambda} transition temperature to the zero-temperature superfluid density is found to be d/2(d-1)], while stringent bounds are placed on others. Analysis of preliminary data is consistent with these predictions.
Though most fermionic Mott insulators order at low temperatures, ordering is ancillary to their insulating behavior. Our emphasis here is on disentangling ordering from the intrinsic strongly correlated physics of a doped half-filled band. To this end, we focus on the two-dimensional Hubbard model. Because the charge gap arises from on-site correlations, we have been refining the nonperturbative approach of Matsumoto and Mancini [Phys. Rev. B 55, 2095 (1997)] which incorporates local physics. Crucial to this method is a self-consistent two-site dynamical cluster expansion which builds in the nearest-neighbor energy scale J. At half-filling, we find that the spectral function possesses a gap of order U and is devoid of any coherent quasiparticle peaks although ordering or charge fractionalization are absent. At low temperatures, local antiferromagnetic correlations emerge. In the doped case, we find that the Fermi surface exceeds the Luttinger volume. The breakdown of Luttinger's theorem in the underdoped regime is traced both to the dynamically generated Mott gap as well to a nonvanishing of the imaginary part of the self-energy at the Fermi level. Spectral weight transfer across the Mott gap also emerges as a ubiquitous feature of a doped Mott insulator and suggests that high- and low-energy scales are inseparable. Additionally in the underdoped regime, we find that a pseudogap exists in the single-particle density of states as well as in the heat capacity. The pseudogap (which is set by the energy scale t2/U) is argued to be a ubiquitous feature of a lightly doped Mott state and simply represents the fact that hole transport involves double occupancy. In analogy with the Mott gap and antiferromagnetism, we propose that ordering may also accompany the formation of a pseudogap. We suggest a current pattern within a one-band model that preserves translational but breaks time-reversal symmetry along the canonical x and y axes but not along $x=\ifmmode\pm\else\textpm\fi{}y$ that is consistent with the experimental observations. Finally, we show that the Hall coefficient in a doped Mott insulator must change sign at a doping level x<1/3. The sign change is tied to a termination of strong correlation physics in the doped Mott state.
We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon–doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon–doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott–Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of the fundamental physics of the Mott state, both in the antiferromagnetic insulator and at finite temperatures and dopings.
In this thesis, several cases of non-equilibrium phenomena and quantum phase transitions in strongly correlated electron systems are analyzed. The unconventional critical behavior near magnetic quantum phase transitions in various heavy-fermion metals has triggered proposals on the breakdown of the Kondo effect at the critical point. In part I, we investigate, within one specific scenario, the fate of such a zero-temperature transition upon coupling of the electronic to lattice degrees of freedom. We study a Kondo-Heisenberg model with volume-dependent Kondo coupling � this model displays both Kondo volume collapse and Kondo-breakdown transitions. Within a large-N treatment, we find that the Kondo breakdown transition remains of second order except for very soft lattices. Finally, we relate our findings to current heavy-fermion experiments. Using non-equilibrium Green�s functions, we derive transport equations for the degrees of freedom participating in the quantum critical region of the Kondo breakdown transition. We discuss conditions under which the transport of electrical charge is described by the independent motion of conduction electrons and auxiliary bosons. Under these conditions, we derive a semiclassical transport equation for the bosons and quantitatively discuss the electrical conductivity of the whole system. Motivated by pressure experiments on FeAs-122 superconductors, in part II we propose a scenario based on local-moment physics to explain salient features at the magnetic phase boundary of CaFe2As2. In this scenario, the low-pressure magnetic phase derives from Fe moments, which become screened in the paramagnetic high-pressure phase. The quantum phase transition can be described as an orbital-selective Mott transition, which is rendered first order by coupling to the lattice. These ideas are illustrated by a suitable mean-field analysis of an Anderson lattice model. An analytical description of non-equilibrium phenomena in interacting quantum systems is rarely possible. In part III we present one example where such a description can be achieved, namely the ferromagnetic Kondo model. In equilibrium, this model is tractable via perturbative renormalization-group techniques. We employ a recently developed extension of the flow-equation method to calculate the non-equilibrium decay of the local magnetization at zero temperature. The flow equations admit analytical solutions which become exact at short and long times, in the latter case revealing that the system always retains a memory of its initial state. Finally, in part IV we analyze the Nernst effect resulting from normal state quasiparticles in the cuprates in presence of various types of translational symmetry breaking. In the electron-doped cuprates, the Nernst signal resulting from a reconstruction of the Fermi surface due to spin density wave order is discussed. An order parameter consistent with the reconstruction of the Fermi surface detected in electron-doped materials is shown to sharply enhance the Nernst signal close to optimal doping. Within a semiclassical treatment, the obtained magnitude and position of the enhanced Nernst signal agrees with Nernst measurements in electron-doped cuprates. In the hole-doped cuprates, we discuss relations between the normal-state Nernst effect and stripe order. We find that Fermi pockets caused by translational symmetry breaking lead to a strongly enhanced Nernst signal with a sign depending on the modulation period of the ordered state and other details of the Fermi surface. This implies differences between antiferromagnetic and charge-only stripes. We compare our findings with recent data from La1.6−xNd0.4SrxCuO4 and YBa2Cu3Oy.
Many strongly correlated electron systems fall outside the conventional quasiparticle paradigm. Their low-energy fermionic excitations need not be adiabatically connected to the bare electrons or appear as poles of the physical electron single-particle Green's function. This thesis investigates to what extent an effective quasiparticle description can nevertheless survive, and which emergent degrees of freedom provide the appropriate low-energy structure. First, the interaction-driven evolution from a quantum spin Hall insulator to a Mott insulator is studied using the dynamical cluster approximation. Dispersive zeros of the single-particle Green's function emerge near the Mott transition and retain a nontrivial topological character. When symmetry breaking is allowed, a nontopological excitonic insulator is found to intrude between quantum spin Hall and Mott insulators. Encoding both poles and zeros within a low-energy quasiparticle Hamiltonian provides a continuous one-body description of the three phases. On the Mott side, its gap evolution supports interpreting the soft excitonic mode as a bound state of quasiparticle and quasihole excitations tied to the Green's function zeros, rather than to the widely separated Hubbard bands. Second, the intrinsic anomalous Hall conductivity of a topological metal is analyzed within a multiband extension of Landau Fermi-liquid theory. Residual interactions among quasiparticles at the Fermi surface dress the dynamic current vertex and generate corrections to the Berry-curvature contribution obtained from the quasiparticle bands alone. Our result supports recent claims that the correct expressions for topological observables include vertex corrections besides the topological invariants built just upon the Green's function. It also demonstrates that such corrections are naturally accounted for by Landau Fermi-liquid theory. Extracting the relevant ingredients for an effective description of material-relevant correlated systems requires computational tools that remain reliable at low temperatures. To this end, a deterministic strong-coupling impurity solver for dynamical mean-field theory is discussed. By providing static, dynamical, and thermodynamic observables without stochastic sampling, it offers a promising route toward multiorbital and spin-orbit coupled problems where conventional Monte Carlo methods currently struggle. Finally, the auxiliary quasiparticle framework underlying the ghost-Gutzwiller Ansatz is investigated. On a model for correlated quantum spin Hall insulators, we show that the topology of the interacting state is encoded in the auxiliary one-body Hamiltonian. The resulting band-structure reveals topological Hubbard bands whose topological character can be tuned through a finite magnetization. When applied to the single-band t-J model, the same framework yields a fractionalized Fermi liquid (FL*). In this phase, dispersive neutral spinons, with vanishing physical-electron spectral weight, coexist with conventional quasiparticles forming a small hole-like Fermi surface, thus violating Luttinger's theorem. The corresponding temperature--doping phase diagram contains a low-doping FL*, a d-wave superconducting dome, and an overdoped conventional Fermi liquid, thereby reproducing key qualitative features of cuprate phenomenology.