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Conference on Lasers and Electro-Optics

Efficient blue light production via coherent anti-Stokes conversion in gases

John J. Ottusch, Metin S. Mangir, David A. Rockwell

Published Apr 24, 1989• 0 citations
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Nonlinear optics and transformation of light in gases

Vasily G. Arkhipkin, A. K. Popov

Uspekhi Fizicheskih Nauk•Jan 1, 1987•7 citations
We experimentally demonstrate efficient Raman conversion to respective Stokes and anti-Stokes fields in both pulsed and continuous modes with a Rb-87 atomic vapor cell. The conversion efficiency is about 40-50% for the Stokes field and 20-30% for the anti-Stokes field, respectively. This efficient conversion process is realized with coherent feedback of both the Raman pump and the frequency-converted fields (Stokes or anti-Stokes). The experimental setup is simple and can be applied easily to produce light sources with larger frequency shifts using other Raman media with long coherence time. They may have potential applications in nonlinear optics, Raman spectroscopy and precision measurement.
We experimentally demonstrate efficient Raman conversion to respective Stokes and anti-Stokes fields in both pulsed and continuous modes with a Rb-87 atomic vapor cell. The conversion efficiency is about 40-50% for the Stokes field and 20-30% for the anti-Stokes field, respectively. This conversion process is realized with feedback of both the Raman pump and the frequency-converted fields (Stokes or anti-Stokes). The experimental setup is very simple and can be applied easily to produce the light source with larger frequency difference using other Raman media. They may have wide applications in nonlinear optics, atomic physics, quantum optics and precise measurement.
Molecular optomechanical cavities have recently emerged as a promising platform for frequency upconversion, enabling the quantum coherent conversion of infrared signal into the visible range. In a recent work [F. Zou et al., Phys. Rev. Lett. 132, 153602 (2024)], we proposed an amplification mechanism that can enhance the intensity of the upconverted infrared signals by a factor of 1000 or more within such a cavity under the ideal case without any noise. In this work, we employ the power spectrum method to investigate the noise added to the upconverted signal in a molecular optomechanical cavity along with the conversion efficiency from infrared signal into visible range. In the red-detuned regime, the anti-Stokes sideband achieves superior conversion efficiency relative to the Stokes sideband. Conversely, the Stokes sideband dominates under the blue-detuned condition, which amplifies the infrared signal. We further demonstrate the dependence of the added noise on the coupling strength and decay rates of the system. In particular, we find that when the infrared signal is amplified, the added noise approaches the quantum limit of one quantum.