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arXiv:2604.17882

Frequency upconversion of infrared signals via molecular optomechanical cavities

Fen Zou, Shu-Xian Quan, Yong Li, Hui Dong

quant-phSubmitted Apr 20, 2026• Announced Apr 21, 2026
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Abstract

Molecular optomechanical cavities have recently emerged as a promising platform for frequency upconversion, enabling the quantum coherent conversion of infrared signal into the visible range. In a recent work [F. Zou et al., Phys. Rev. Lett. 132, 153602 (2024)], we proposed an amplification mechanism that can enhance the intensity of the upconverted infrared signals by a factor of 1000 or more within such a cavity under the ideal case without any noise. In this work, we employ the power spectrum method to investigate the noise added to the upconverted signal in a molecular optomechanical cavity along with the conversion efficiency from infrared signal into visible range. In the red-detuned regime, the anti-Stokes sideband achieves superior conversion efficiency relative to the Stokes sideband. Conversely, the Stokes sideband dominates under the blue-detuned condition, which amplifies the infrared signal. We further demonstrate the dependence of the added noise on the coupling strength and decay rates of the system. In particular, we find that when the infrared signal is amplified, the added noise approaches the quantum limit of one quantum.

Journal reference
Commun. Theor. Phys. 78, 085503 (2026)
DOI
10.1088/1572-9494/ae70f1
Comments
10 pages, 6 figures

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Molecular optomechanical cavities have recently emerged as a promising platform for frequency upconversion, enabling the quantum coherent conversion of infrared signal into the visible range. In a recent work [F. Zou et al., Phys. Rev. Lett. 132, 153602 (2024)], we proposed an amplification mechanism that can enhance the intensity of the upconverted infrared signals by a factor of 1000 or more within such a cavity under the ideal case without any noise. In this work, we employ the power spectrum method to investigate the noise added to the upconverted signal in a molecular optomechanical cavity along with the conversion efficiency from infrared signal into visible range. In the red-detuned regime, the anti-Stokes sideband achieves superior conversion efficiency relative to the Stokes sideband. Conversely, the Stokes sideband dominates under the blue-detuned condition, which amplifies the infrared signal. We further demonstrate the dependence of the added noise on the coupling strength and decay rates of the system. In particular, we find that when the infrared signal is amplified, the added noise approaches the quantum limit of one quantum.
Molecular cavity optomechanical systems have recently emerged as a promising platform for enhancing infrared detection sensitivity, owing to their ability to up-convert low-frequency infrared (IR) photons to visible frequency range. Generally, under red-detuned pumping in such systems, the ideal conversion efficiency of the IR signal approaches 1. To overcome this efficiency constraint, we propose a scheme that incorporates gain into the infrared cavity of a molecular cavity optomechanical system comprising two cavities and an ensemble of N molecules. The upconversion process, which relies on IR absorption and Raman scattering associated with specific vibrational modes, is significantly amplified by the incorporation of gain under the red-detuned conditions. Moreover, our analysis demonstrates that the added noise is maintained near 0.5.
Abstract Adiabatic state conversion in optomechanical systems requires the evolution process to be very slow, which limits its application in quantum information processing. In this paper, we explicitly show that speeding up adiabatic state conversion in optomechanical systems can be implemented. For the case that each cavity is driven far from the red-detuned mechanical sideband, the high-efficiency population transfer between cavity modes is achieved via an additional Hamiltonian  a ( t ) , whereas the population of the mechanical resonator can be effectively inhibited. In the meanwhile, in the case of each cavity driven near the red-detuned mechanical sideband, the population transfers can be realized by varying the modified optomechanical couplings without an additional Hamiltonian. Numerical simulation demonstrates that the transfer is robust to the system decays.
High-gain amplifiers of electromagnetic signals operating near the quantum limit are crucial for quantum information systems and ultrasensitive quantum measurements.However, the existing techniques have a limited gain-bandwidth product and only operate with weak input signals.Here, we demonstrate a two-port optomechanical scheme for amplification and routing of microwave signals, a system that simultaneously performs high-gain amplification and frequency conversion in the quantum regime.Our amplifier, implemented in a two-cavity microwave optomechanical device, shows 41 dB of gain and has a high dynamic range, handling input signals up to 10 13 photons per second, 3 orders of magnitude more than corresponding Josephson parametric amplifiers.We show that although the active medium, the mechanical resonator, is at a high temperature far from the quantum limit, only 4.6 quanta of noise is added to the input signal.Our method can be readily applied to a wide variety of optomechanical systems, including hybrid optical-microwave systems, creating a universal hub for signals at the quantum level.
We propose and demonstrate a high efficiency broadband near infrared single-photon upconversion and detection with a broadband pump laser based on sum frequency conversion in the PPLN crystal. By using a pump laser centered at 1040 nm with a spectral bandwidth of 10 nm, the signal single-photons centered at 1562 nm with a broadband bandwidth up to 7.2 nm are frequency-converted from the near infrared to the visible regime. A maximum conversion efficiency of 18.8% is achieved, while the background noise is measured to be only 1.2 × 10−3 counts/pulse. The corresponding spectral linewidth of the upconverted photons is 0.2 nm. This scheme of broadband infrared single-photon upconversion and detection provides potential solutions in infrared laser ranging, broadband infrared imaging and quantum key distribution.
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Abstract The investigation of the ultimate limits imposed by quantum mechanics on amplification represents an important topic both on a fundamental level and from the perspective of potential applications. We discuss here a novel regime for bosonic linear amplifiers—beside phase-insensitive and phase-sensitive amplification—which we term here phase-mixing amplification. Furthermore, we show that phase-mixing amplification can be realised in a cavity optomechanical setup, constituted by a mechanical resonator which is dispersively coupled to an optomechanical cavity asymmetrically driven around both mechanical sidebands. While, in general, this amplifier is phase-mixing, for a suitable choice of parameters, the amplifier proposed here operates as a phase-sensitive amplifier. We show that both configurations allow amplification with an added noise below the quantum limit of (phase-insensitive) amplification in a parameter range compatible with current experiments in microwave circuit optomechanics. In particular, we show that introducing phase-mixing amplification typically allows for a significant reduction of the added noise.