The impact of lattice vibrations on the electric conductivity has been considered a settled issue since the proof of the Migdal theorem. The precondition for its validity is a higher velocity of electronic than phononic excitation modes. In some new materials, e. g. weakly coupled spin chains and heavy fermion systems, this precondition is not fulfilled. The heat conductivity of such systems is calculated by means of perturbation theory in this work. Another subject is the interplay of Umklapp scattering and weak disorder in spin chains and one-dimensional correlated metals. Hidden conservation laws lead to a strong coupling between heat current and charge or spin current, respectively. The transport properties are calculated perturbatively within the hydrodynamic memory matrix formalism, which gives a lower bound to the conductivies. To calculate the Lorenz number of one-dimensional metals, we model within this formalism also the influence of phonons, which in physical systems contribute substantially to the heat current. The introduction of ultracold quantum gases in optical lattices in the recent years provides a powerful tool for the modeling of many systems to solid state physics, in particular systems out of equilibrium. The relatively slow dynamics of the cold atoms allows for time resolved imaging of the atoms and thus opens up new perspectives. In the last part of this thesis, a recent experiment, which measures the expansion of a correlated atom cloud in an optical lattice, is compared to a lattice Boltzmann simulation. Depending on the local density, the problem is shown to be described by the crossover from diffusive to ballistic transport.
The impact of lattice vibrations on the electric conductivity has been considered a settled issue since the proof of the Migdal theorem. The precondition for its validity is a higher velocity of electronic than phononic excitation modes. In some new materials, e. g. weakly coupled spin chains and heavy fermion systems, this precondition is not fulfilled. The heat conductivity of such systems is calculated by means of perturbation theory in this work. Another subject is the interplay of Umklapp scattering and weak disorder in spin chains and one-dimensional correlated metals. Hidden conservation laws lead to a strong coupling between heat current and charge or spin current, respectively. The transport properties are calculated perturbatively within the hydrodynamic memory matrix formalism, which gives a lower bound to the conductivies. To calculate the Lorenz number of one-dimensional metals, we model within this formalism also the influence of phonons, which in physical systems contribute substantially to the heat current. The introduction of ultracold quantum gases in optical lattices in the recent years provides a powerful tool for the modeling of many systems to solid state physics, in particular systems out of equilibrium. The relatively slow dynamics of the cold atoms allows for time resolved imaging of the atoms and thus opens up new perspectives. In the last part of this thesis, a recent experiment, which measures the expansion of a correlated atom cloud in an optical lattice, is compared to a lattice Boltzmann simulation. Depending on the local density, the problem is shown to be described by the crossover from diffusive to ballistic transport.
The goal of this thesis is to study the transport properties and real-time dynamics of quantum magnets and ultra-cold atomic gases in one spatial dimension using numerical methods. The focus will be on the discussion of diffusive versus ballistic dynamics along with a detailed analysis of characteristic velocities in ballistic regimes. For the simulation of time-dependent density profiles we use the adaptive time-dependent density matrix renormalization group (DMRG). This numerical method allows for the simulation of time-dependent wave functions close to as well as far from equilibrium in a controlled manner. The studies of one-dimensional quantum magnets are partially motivated by the experimental evidence for a highly anisotropic and for insulators comparably high thermal conductivity of certain cuprates. We use linear response theory to study transport coefficients at arbitrary temperatures by diagonalizing small systems exactly and then calculating the current-current correlation functions. As first application we discuss the spin transport in the spin-1/2 Heisenberg chain with anisotropic exchange interactions (XXZ-chain). The second application of exact diagonalization, here in combination with time-dependent DMRG, is a discussion of the transverse components of the current-current correlation function. While usually only a Zeeman field is considered in the theory of transport coefficients, we here investigate the dynamic induced by an additional transverse magnetic field. We find that in this scenario the current-current correlation function exhibits coherent oscillations. In addition a second non-trivial frequency, different from the one expected from the usual Larmor precession, emerges and is studied varying temperature and field. Finally we calculate the frequency-dependent spin and heat conductivity of dimerized spin chains in a magnetic field. Motivated by the recent experimental studies of the phase diagram of C5H12N2CuBr4 we take the dimerized chain as a minimal model that exhibits features of the low-temperature region of the observed phase diagram. As a main result, the spin and heat conductivity obtained from linear response theory are enhanced in the field-induced gapless phase. The last application in the field of one-dimensional quantum magnets is the simulation of time-dependent energy-density wave-packets close to as well as far from equilibrium using the time-dependent density renormalization group. The main results are ballistic energy dynamics independently of how far out-of-equilibrium the initial state is and a detailed understanding of the average expansion velocity. The applications in the field of ultra-cold atomic gases focus on the sudden expansion of an initially trapped gas into an empty optical lattice. This setup was recently realized in an experiment performed by U. Schneider {\it et al.} and discussed in the context of electronic transport in the two-dimensional and the three-dimensional Fermi-Hubbard model. Here we investigate the sudden expansion of three different setups: For the expansion of a spin-balanced cloud of fermions, we identify the ballistic regime, and therein investigate the average expansion velocity of the cloud. As a main result the expansion velocity is determined by a small subset of the initial condition over a wide range of parameters. For instance, the Mott-insulating phase of the Hubbard model is characterized by a constant expansion velocity independently of the strength of the interaction. In the case of spinless bosons, we study the expansion from initial states that have a fixed particle number per lattice site and a certain concentration of defects. We study the expansion velocity as a function of interaction strength and investigate whether the time-dependent momentum distribution functions indicate a dynamical quasi-condensation. The last example is the sudden expansion of a spin-polarized gas of fermions in the presence of attractive interactions. This study is motivated by current effort to experimentally detect the Fulde-Ferrell-Larkin-Ovchinnikov state. Our results for the time-dependent momentum distribution functions and the wave-function of the pair condensate suggest that the signatures of the FFLO state vanish quickly, yet a stationary form of the momentum distribution also emerges fast. The latter is shown to be determined by the initial conditions, which might eventually allow for an indirect detection of the FFLO phase.
We set up a framework in which controlled lower bounds to conductivities of strongly correlated quantum systems may be calculated perturbatively in situations where the conductivities are infinite in the unperturbed model. This framework is then applied to study the transport properties of almost integrable systems, in general, and heat and spin conductivities in the integrable XXZ Heisenberg spin chain perturbed by various integrability breaking couplings, in particular. Furthermore, we systematically develop a microscopic description of the contribution of spin chains to experimentally measured heat conductivity in spin chain compounds, with an emphasis on the effect of weak disorder.
Cutting-edge technology needs small, ultrafast devices, operational in a wide range of regimes. This calls for solids with novel, unconventional and tailorable properties. Great progress is expected from materials in which electron-electron and electron-phonon correlations strongly affect the dynamics ( i.e. "unforeseen" useful properties are expected to be most likely found in systems with complex behavior). In spite of the potentially huge technological pay-off, our understanding of these systems is rather incomplete, especially in non-equilibrium. Often, with knowledge of systems or phenomena at an early stage, it is rewarding to resort to model, simplified descriptions. This strategy is used in this thesis, where we study several models lattice systems via density-functional theory. The latter is a well established approach (in fact, it is the current method of choice) for investigations of real materials. In our research, we focussed on little understood properties of interacting many-particle systems, such as the time-dependent conduction properties of electronic devices in the presence of interactions, disorder, and lattice vibrations, or the expansion of ultracold fermion clouds in 3D optical lattices. All these systems were described in terms of Hubbard-type interactions for the electrons, and Holstein-type electron-phonon interactions. Our results show interesting features due to the interactions which depend on dimensionality; they also show a dynamical crossover for several properties, due to the competition between disorder and interaction. Finally, when lattice vibrations are included, we showed how it is possible to manipulate in a controlled way the nuclear dynamics of molecular device via fast electronic external fields, of potential interest for technologies employing nanomolecular motors.
The study of collective behaviour in many-body systems often explores fundamentally new ideas absent from the mere constituents of such a system. A paradigmatic model for these studies is the spin-1/2 XXZ chain and its fermionic equivalent. This thesis can be broadly divided into the study of two fundamental aspects of this model. Firstly, we discuss localisation phenomena in one dimensional lattices as often experimentally realised in cold atom systems. Secondly, we investigate how disorder and symmetry influence heat transport in spin chains. More specifically, in the first part we consider a system of non-interacting fermions in one dimension subject to a single-particle potential consisting of a strong optical lattice, a harmonic trap, and uncorrelated on-site disorder. We investigate a global inhomogeneous quantum quench and present numerical and analytical results for static and dynamical properties. We show that the approach to the non-thermal equilibrium state is extremely slow and that it implies a sensitivity to disorder parametrically stronger than that expected from Anderson localisation. We also consider the above system in a strong non-uniform electric field. In the non-interacting case, due to Wannier-Stark localisation, the single-particle wave functions are exponentially localised without quenched disorder. We show that this system remains localised in the presence of nearest-neighbour interactions and exhibits physics analogous to models of conventional many-body localisation. The second part explores the hydrodynamics of the disordered XYZ spin chain. Using time-evolving block decimation on open chains of up to 400 spins attached to thermal baths, we probe the energy transport of this system. Our principal findings are as follows. For weak disorder there is a stable diffusive region that persists up to a critical disorder strength that depends on the XY anisotropy. Then, for disorder strengths above this critical value energy transport becomes increasingly subdiffusive.
Transport properties and nonequilibrium dynamics in strongly correlated materials are \ntypically difficult to calculate. This holds true even for minimalistic model Hamiltonians \nof these systems, such as the fermionic Hubbard model. \nUltracold atoms in optical lattices enable an alternative realization of the Hubbard \nmodel and have the advantage of being free of additional complications such as phonons, \nlattice defects or impurities. This way, cold atoms can be used as quantum simulators of \nstrongly interacting materials. Being thermally isolated systems, however, we show that \ncold atoms in optical lattices can also behave very differently from solids and can show a \nplethora of novel dynamic effects. \nIn this thesis, several out-of equilibrium processes involving interacting fermionic atoms \nin optical lattices are presented. We first analyze the expansion dynamics of an initially \nconfined atomic cloud in the lowest band of an optical lattice. While non-interacting atoms \nexpand ballistically, the cloud expands with a dramatically reduced velocity in the presence \nof interactions. Most prominently, the expansion velocity is independent of the attractive \nor repulsive character of the interactions, highlighting a novel dynamic symmetry of the \nHubbard model. \nIn a second project, we discuss the possibility of realizing negative absolute temperatures in optical lattices. Negative absolute temperatures characterize equilibrium states \nwith an inverted occupation of energy levels. Here, we propose a dynamical process to realize equilibrated Fermions at negative temperatures and analyze the time scales of global \nrelaxation to equilibrium, which are associated with a redistribution of energy and particles \nby slow diffusive processes. \nWe show that energy conservation has a major impact on the dynamics of an interacting \ncloud in an optical lattice, which is exposed to an additional weak linear (gravitational) \npotential. Instead of ‘falling downwards‘, the cloud diffuses symmetrically upwards and \ndownwards in the gravitational potential. Furthermore, we show analytically that the \nradius R grows with the time t according to R ∼ t^1/3, consistent with numerical simulations \nof the Boltzmann equation. \nFinally, we analyze the damping of Bloch oscillations by interactions. For a homogeneous system, we discuss the possibility of mapping the dynamics of the particle current to \na classical damped harmonic oscillator equation, thereby giving an analytic explanation for \nthe transition from weakly damped to over-damped Bloch oscillations. We show that the \ndynamics of a strongly Bloch oscillating and weakly interacting atomic cloud can be discribed in terms of a novel effective “stroboscopic” diffusion equation. In this approximation, \nthe cloud’s radius R grows asymptotically in time t according to R ∼ t^1/5 .
Modern quantum materials host a wide range of electronic phases in which transport properties are governed by strong interactions and collective effects. This thesis investigates charge, heat, and momentum transport in interacting electronic systems across different theoretical frameworks, ranging from Fermi liquid theory to strongly coupled strange metals.The first part of the thesis focuses on two-dimensional Fermi liquids at finite temperature, where rapid electron-electron scattering can give rise to hydrodynamic behavior. A kinetic-theory framework allowing an exact treatment of quasiparticle distribution functions beyond the asymptotic low-temperature regime is used to compute the full spectrum of collective modes, providing a detailed characterization of long-lived odd-parity excitations and the intermediate transport regime between ballistic and hydrodynamic flow. The same framework is employed to determine the shear viscosity of interacting electron liquids beyond conventional perturbative limits.The second part of the thesis concerns strongly interacting quantum systems where the quasiparticle picture breaks down.Holographic duality is used to study transport and thermoelectric response in quantum critical systems subject to periodic potentials, providing a controlled framework for momentum relaxation and magnetotransport in non-Fermi liquids. The thesis further develops holographic models of collective charge dynamics in systems with dynamical electromagnetism, including bulk plasmons and surface plasmon polaritons, and explores connections between Fermi surface physics and holographic gauge-field dynamics.