Laser cooling and trapping of neutral particles has become a major area of research in atomic physics with the discovery of the first Bose-Einstein condensates (BECs) in 1995. These ultracold atomic vapors allow for study of fundamental quantum electromagnetic properties of atoms that are otherwise inaccessible due to large thermal energy fluctuations disrupting the quantum state. To this end, I have constructed and characterized a laser cooling system to be used to study spinor physics in a 41K BEC. In this thesis, I detail the major components of the laser cooling system that I worked on including the master external cavity diode laser (ECDL), tapered amplifier, laser frequency characterization subsystems, and saturated absorption spectroscopy lock. Additionally, I discuss the development of a novel passive magnetic field fluctuation-cancelling device that uses high temperature superconducting ribbon to take advantage of Lenz' Law. These components will serve as the backbone to the laser cooling apparatus needed to condense 41K into the quantum mechanical ground state.
Laser cooling and trapping of neutral particles has become a major area of research in atomic physics with the discovery of the first Bose-Einstein condensates (BECs) in 1995. These ultracold atomic vapors allow for study of fundamental quantum electromagnetic properties of atoms that are otherwise inaccessible due to large thermal energy fluctuations disrupting the quantum state. To this end, I have constructed and characterized a laser cooling system to be used to study spinor physics in a 41K BEC. In this thesis, I detail the major components of the laser cooling system that I worked on including the master external cavity diode laser (ECDL), tapered amplifier, laser frequency characterization subsystems, and saturated absorption spectroscopy lock. Additionally, I discuss the development of a novel passive magnetic field fluctuation-cancelling device that uses high temperature superconducting ribbon to take advantage of Lenz' Law. These components will serve as the backbone to the laser cooling apparatus needed to condense 41K into the quantum mechanical ground state.
Optical trapping as a viable means of exploring the physics of ultracold dilute atomic gases has revealed a new spectrum of physical phenomena. In particular, macroscopic and sudden occupation of the ground state below a critical temperature—-a phenomenon known as Bose-Einstein condensation—-has become an even richer system for the study of quantum mechanics, ultracold collisions, and many-body physics in general. Optical trapping liberates the spin degree of the BEC, making the order parameter vectorial (‘spinor BEC’), as opposed to the scalar order of traditional magnetically trapped condensates. The work described within is divided into two main efforts. The first encompasses the all-optical creation of a Bose-Einstein condensate in rubidium vapor. An all-optical path to spinor BEC (as opposed to transfer to an optical trap from a magnetic-trap condensate) was desired both for the simplicity of the experimental setup and also for the potential gains in speed of creation; evaporative cooling, the only known path to dilute-gas condensation, works only as efficiently as the rate of elastic collisions in the gas, a rate that starts out much higher in optical traps. The first all-optical BEC was formed elsewhere in 2001; the years following saw many groups worldwide seeking to create their own version. Our own all-optical spinor BEC, made with a single-beam dipole trap formed by a focused CO₂ laser, is described here, with particular attention paid to trap loading, measurement of trap parameters, and the use of a novel 780 nm high-power laser system. The second part describes initial experiments performed with the nascent condensate. The spinor properties of the condensate are documented, and a measurement is made of the density-dependent rate of spin mixing in the condensate. In addition, we demonstrate a novel dual-beam atom laser formed by outcoupling oppositely polarized components of the condensate, whose populations have been coherently evolved through spin dynamics. We drive coherent spin-mixing evolution through adiabatic compression of the initially weak trap. Such dual beams, nominally number-correlated through the angular momentum-conserving collision m=0 + m=0 ⇌ m=+1 + m=-1 have been proposed as tools to explore entanglement and squeezing in Bose-Einstein condensates.
In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field B. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field Bc, asymptotic values of n0 (relative atom number in mF=0 state) at large B and the phase diagram of n0. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" Ts and the ``kinetic temperature" Tk with Ts≪Tk, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.
The subject of this thesis is the use of BECs for atom interferometry. The standard way atom interferometry is today performed is by interrogating free falling samples of atoms. The employed samples are cold (but not condensed) to have high coherence, and dilute, not to interact significantly with each other. This technique represents nowadays an almost mature field of research in which the achievable interferometric sensitivity is bounded by the atomic shot noise. Until a few years ago the employment of BECs in such devices was strongly limited by the effect of the interactions between the condensed atoms. This obstacle is today removable exploiting interaction tuning techniques. The use of BECs would be advantageous for atom interferometry inasmuch they represents the matter analogue of the optical laser providing the maximum coherence allowed by quantum mechanics. Moreover, non-linear dynamic can be exploited in order to prepare entangled states of the system. The realization of entangled samples can lead to sub-shot noise sensitivity of the interferometers. At today very nice proof-of-principle experiments have been realized in this direction but a competitive device is still missing. This thesis work is inserted in a long term project whose goal is the realization of such a device. The basic operational idea of the project starts with the preparation of a BEC in a double well potential. By the effect of strong interactions the atomic system can be driven into an entangled state. Once the entangled state is prepared, interactions can be †switched off†and the interferometric sequence performed. This thesis begins with the description of the apparatus for the production of tunable BECs to be used in the interferometer. We chose to work with 39K atoms because this atomic species presents many convenient Feshabch resonances at easily accessible magnetic field values. The cooling of this particular atomic species presents many difficulties, both for the laser and evaporative cooling processes. For this reason, this was the last alkaline atom to be condensed. Its condensation up to now was only possible by employing sympathetic cooling with another species. In this thesis our solutions to the various cooling issues is reported. In particular we realized sub-Doppler cooling for the first time for this species and we achieved condensation via evaporation in an optical dipole trap taking advantage of a Feshbach resonance. In the last part of this work, are presented original calculations for the effects of thermal fluctuations on the coherence of a BEC in a double well, discussing the interplay between thermal fluctuations and interactions in this system. Estimations and feasibility studies regarding the double well trap to be realized are also reported.
Research on degenerate quantum gases of dilute atomic gases has become a well established field in modern physics and revealed many astonishing phenomena. The first experiments on Bose and Fermi gases at low temperatures aimed to prove the predictions of quantum mechanics on a macroscopic scale. Since then we make use of Bose and Fermi gases and mixtures of any combination to model other many body systems. A property of Bose Einstein condensates is superfluidity which we want to investigate further in toroidal potentials with a new apparatus which can produce an all-optical BEC. This means trapping thermal atoms in an optical dipole trap and cooling the sample by evaporation into the quantum degenerate regime. This new technique was first successfully demonstrated by M.D. Barrett et al. in 2001 and promises to be faster and simpler than the well established and common way of evaporation in magnetic traps. A new apparatus was built by the author and we report on the experimental details of the trapping of 87Rb atoms from a hot vapour and cooling them in a magneto-optical trap, and further evaporation to quantum degeneracy in a crossed optical dipole trap operating at a wavelength of l = 1064nm, with accurate control of the power in both beams via a feedback loop. The evaporation of neutral atoms of 87Rb in far red detuned optical dipole traps using linearly polarised laser light is spin independent, and mixed spinor condensates of the F=1 manifold can be formed. As an empirical technique we found by applying a magnetic gradient field during the final evaporation that we can selectively populate mF spin states or prepare mixtures. This intriguing mechanism was found earlier as well by M. S. Chang, but is yet not fully understood and subject of our future research. We can now routinely prepare an almost pure condensate containing up to 7000 atoms in the condensed phase purely in the mF = 0 spin state. This thesis contains the theoretical framework of Bose-Einstein condensation with in mean-field theory, the concepts of cooling of atoms in magneto-optical traps, the trapping and evaporation in optical dipole traps and the experimental realisation. In the future this experiment will be extended by a fast scanning dipole trap to apply arbitrary time averaged potentials of more complex geometries, such as toroidal traps to study the effects of superfluidity in a periodic potential. The production of toroidal traps and cold atoms in such a trap are outlined in this thesis.
The possibility to mould and control pure quantum systems has been offered by the experimental observation of Bose-Einstein condensation, a unique phase of matter when macroscopic quantities of a gas occupy the lowest quantum state. Techniques for creating these degenerate gases vary from laboratory to laboratory; each offers an unique test bed for studying quantum physics on a macroscopic scale. This thesis reports on the experimental design, construction and performance of an apparatus to create two-component 87Rb and 41K condensates for studies of non-equilibrium dynamics. This thesis is broken down as follows. In Chapter 1, a brief overview of the history and status of Bose Einstein condensates is presented, to affirm the motivation behind our work. Chapter 2 then presents the fundamental theory and background information to understand how and why our experiment was built. Chapter 3 describes the bulk of the work undertaken at the beginning of this thesis. In particular it describes the design choices, construction and performance of the vacuum, and laser and magnetic coil systems that are the key structural elements of the apparatus. In particular the vacuum system is a two-component differentially pumped system designed to optimise the number and lifetime of trapped atoms. Another integral element of the vacuum chamber is the science cell that enables high optical access, and close physical, access to an atomic cloud. As a result, high resolution imaging, ≃ 980 nm resolution at 780 nm is expected with a commercial microscope objective lens. The laser system is carefully de- signed to best combine and deliver the seven different optical frequencies required to simultaneously trap and manipulate 87Rb and 41K atoms. The magnetic coil system also represents an integral component of the apparatus, responsible for trapping and transferring atoms in a quadrupole field. One pair of coils is able to have their current direction reversed in order to generate bias fields. This allows access to Feshbach resonances between the two species, once they have been condensed. The second part of this thesis, Chapter 4, describes the performance of the apparatus when used to simultaneously trap 41K and 87Rb in the 3D magneto- optical trap (MOT) and produce a condensate of 87Rb atoms. In particular 1 × 109 rubidium atoms are routinely trapped in the 3D-MOT and transferred to the science chamber. In the hybrid trap the atoms are evaporatively cooled via microwave radiation, later to be used to sympathetically cool 41K, and loaded into a hybrid optical dipole and magnetic trap. At this stage ≃ 5 × 106 atoms are evaporatively cooled, by lowering the trap depth of the optical dipole beam, until a condensate of 87Rb is formed, containing 1.5 × 105 atoms. Additionally we are able to produce 3D MOTs of 41K simultaneously with the 87Rb 3D MOTs.
The three experiments described in this thesis investigate fundamental properties of ultracold atoms. Using laser cooling and evaporative cooling, a dilute gas of sodium atoms is cooled to ~100 nK. Under these circumstances a Bose-Einstein condensate (BEC) forms, where millions of atoms collapse into the lowest energy state of the system and share a macroscopic wavefunction. The experiments are done in an ultrahigh vacuum and the atoms are manipulated remotely using laser beams, magnetic fields, and RF-fields. Using ultracold atoms allows unprecedented control over the internal and external degrees of freedom of the system, making it very suitable for precision measurements. Ultracold atoms also serve as a model system for more complicated or remote fields such as solid-state physics and cosmology. In the first experiment the refractive index of an ultracold bosonic gas is studied. The atomic clouds are analyzed for temperature and number of particles using nearly non-destructive phase-contrast imaging. After each pulse of probe light a small fraction of the atoms is lost, while the cloud is simultaneously slightly heated. This makes it possible to study the scattering rate as a function of temperature using only a single sample. It is observed that the scattering rate increases below the critical temperature for BEC by more than a factor of 3 compared to the classical value. This enhancement is in good agreement with the predictions by theoretical work that takes two-body correlation and the Lorentz-Lorenz correction into account. The method is also used to perform calorimetry on the Bose gas and directly measure the heat capacity of the BEC. The second chapter deals with magnetism in ultracold gases. When cooling an ultracold gas containing different spin components below the critical temperature for BEC, stable magnetic domains form. The appearance of these domains and the dynamics of the domain walls are studied. The spin mixture is prepared by performing an RF-sweep on ground state atoms in the presence of a magnetic field. Spin dynamics are induced by applying magnetic gradients. Spin drag, which is the transport coefficient responsible for damping spin currents, was measured in a two-component system. Furthermore a new method for spin resolved phase contrast imaging is presented, which is used to study time evolution in situ non-destructively. The last experiment focuses on spontaneous symmetry breaking. When passing a continuous phase transition, spontaneous symmetry breaking causes the development of domains with an independently chosen order parameter. The domains are separated by boundary defects. In this experiment the spontaneous creation of solitons was observed, which are boundary defects in the phase of the condensate, as well as magnetic domain walls, which are the boundary defects in the magnetization. Through the Kibble-Zurek mechanism it is possible to determine the critical exponents that characterize the phase transition. The critical exponents are predicted to be universal, i.e. do not depend on the microphysics of the system, so the results from our ultracold atoms lab can help answer universal questions for example from cosmology and from the early universe.